Related papers: Two-Photon Absorption Spectroscopy using Intense P…
Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…
We consider ramifications of the use of high speed light modulators to questions of correlation and measurement of time-energy entangled photons. Using phase modulators, we find that temporal modulation of one photon of an entangled pair,…
Traditionally, spectroscopy is performed by examining the position of absorption lines. However, at frequencies near the transition frequency, additional information can be obtained from the phase shift. In this work we consider the…
The authors demonstrate a form of two-photon-counting interferometry by measuring the coincidence counts between single-photon-counting detectors at an output port of a Mach-Zehnder Interferometer (MZI) following injection of broad-band…
We consider a scheme of multiplexed cold atomic ensembles that generate a frequency-entangled biphoton state with controllable entropy of entanglement. The biphoton state consists of a telecommunication photon (signal) immediately followed…
Joint spectral measurements are a powerful tool for characterising biphoton spectral correlation, which is crucial for quantum information and communication technologies. In these applications, highly pure biphoton states are essential in…
We use a non-perturbative theoretical approach to the parametric down-conversion (PDC) process, which generates entangled-photon field for an arbitrarily strong pump-pulse. This approach can be used to evaluate multi-point field correlation…
We investigate how entanglement can enhance two-photon absorption in a three-level system. First, we employ the Schmidt decomposition to determine the entanglement properties of the optimal two-photon state to drive such a transition, and…
Entangled photon pairs have been promised to deliver a substantial quantum advantage for two-photon absorption spectroscopy. However, recent work has challenged the previously reported magnitude of quantum enhancement in two-photon…
Spectroscopy with entanglement has shown great potential to break limitations of traditional spectroscopic measurements, yet the role of entanglement in spectroscopic multi-parameter joint measurement, particularly in the infrared optical…
Quantum entanglement offers an incredible resource for enhancing the sensing and spectroscopic probes. Here we develop a microscopic theory for the stimulated Raman scattering (SRS) using entangled photons. We demonstrate that the…
We experimentally demonstrate shaping of the two-photon wavefunction of entangled photon-pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the two-photon wavefunction exactly like a…
Quantum-intensity-correlated twin beams of light can be used to measure absorption with precision beyond the classical shot-noise limit. The degree to which this can be achieved with a given estimator is defined by the quality of the…
We propose a novel quantum diffraction imaging technique whereby one photon of an entangled pair is diffracted off a sample and detected in coincidence with its twin. The image is obtained by scanning the photon that did not interact with…
Quantum entanglement has emerged as a great resource for interactions between molecules and radiation. We propose a new paradigm of stimulated Raman scattering with entangled photons. A quantum ultrafast Raman spectroscopy is developed for…
We report on an experiment demonstrating entanglement swapping of time-frequency entangled photons. We perform a frequency-resolved Bell-state measurement on the idler photons from two independent entangled photon pairs, which projects the…
We investigate experimentally the nonlocal phase modulation of multiple-frequency-mode, continuous-variable entangled twin beams. We use a pair of electro-optical phase modulators to modulate the entangled probe and conjugate light beams…
We observe that a weak guided light field transmitted through an ensemble of atoms coupled to an optical nanofiber exhibits quadrature squeezing. From the measured squeezing spectrum we gain direct access to the phase and amplitude of the…
Spectroscopy of gases under high-pressure conditions is of interest in various fields such as plasma physics and astrophysics. Recently, it has also been proposed to utilize a high-pressure noble gas environment as a thermalization medium…
We demonstrate theoretical and experimentally how it is possible to manipulate an entangled angular spectrum of twin beams, in order to reconstruct correlated images with coincidence detection. The entangled angular spectrum comes from the…