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Chip-scale optical frequency combs can provide broadband spectroscopy for diagnosing complex organic molecules. They are also promising as miniaturized laser spectrometers in applications ranging from atmospheric chemistry to geological…

Mid-wave infrared (MWIR) frequency comb is expected to dramatically improve the precision and sensitivity of molecular spectroscopy. For high resolution application, high speed MWIR photodetector is one of the key components, however, the…

Applied Physics · Physics 2023-07-19 Jian Huang , Zhiyang Xie , Yaojiang Chen , John Bowers , Baile Chen

Frequency combs are powerful tools for many applications and high performances are achieved by stabilizing these lasers. For operation in the mid-infrared, quantum cascade lasers (QCL) are ideal candidates as they present numerous…

A femtosecond frequency comb provides a vast number of equidistantly spaced narrow band laser modes that can be simultaneously tuned and frequency calibrated with 15 digits accuracy. Our Vernier spectrometer utilizes all of theses modes in…

High-resolution ultrasound based imaging techniques like photoacoustic (PA) imaging that require fast detection of acoustic waves, are often coupled with an opto-mechanical sensor like a Fabry-Perot cavity (FPC) for enhanced sensitivity at…

Optical frequency combs based on semiconductor lasers are a promising technology for monolithic integration of dual-comb spectrometers. However, the stabilization of the offset frequency fceo remains a challenging feat due the lack of…

Vibrational spectroscopy is a cornerstone technique for molecular characterization and offers an ideal target for the computational investigation of molecular materials. Building on previous comprehensive assessments of efficient methods…

We demonstrate a high-accuracy dual-comb spectrometer centered at 3.4 \mu m. The amplitude and phase spectra of the P, Q, and partial R-branch of the methane {\nu}3 band are measured at 25 MHz to 100 MHz point spacing with ~kHz resolution…

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…

Supersonic engine development requires accurate and detailed measurements of fluidic and thermodynamic parameters to optimize engine designs and benchmark computational fluid dynamic (CFD) simulations. Here, we demonstrate that dual…

Si$_3$N$_4$ waveguides, pumped at 1550 nm, can provide spectrally smooth, broadband light for gas spectroscopy in the important 2 ${\mathrm{\mu}}$m to 2.5 ${\mathrm{\mu}}$m atmospheric water window, which is only partially accessible with…

Fourier-transform infrared spectroscopy (FTIR) is the golden standard of mid-infrared (MIR) molecular spectroscopic analysis through optically-encoded vibrational signatures. Michelson-type FTIR and MIR dual-comb spectrometers allow us to…

Optics · Physics 2025-05-06 Kazuki Hashimoto , Venkata Ramaiah Badarla , Takuro Ideguchi

Mid-infrared laser frequency combs are compelling sources for precise and sensitive metrology with applications in molecular spectroscopy and spectro-imaging. The infrared atmospheric window between 3-5.5 $\mu$m in particular provides vital…

Dual-comb spectroscopy is extended to the visible spectral range with a set-up based on two frequency-doubled femtosecond ytterbium-doped fiber lasers. The dense rovibronic spectrum of iodine around 19240 cm-1 is recorded within 12 ms at…

We extend the technique of multiplex coherent Raman spectroscopy with two femtosecond mode-locked lasers to oscillators of a pulse repetition frequency of 1 GHz. We demonstrate spectra of liquids, which span 1100 cm$^{-1}$ of Raman shifts.…

We demonstrate the advantages of THz frequency combs for high-resolution spectroscopy. This benefits from wide spectral coverage and the exact knowledge of the frequency position of each comb component. Heterodyne detection combined with a…

Instrumentation and Detectors · Physics 2024-12-03 Francis Hindle , Alexandra Khabbaz , Anthony Roucou , Jean-Francois Lampin , Gaël Mouret

Spectral imaging in the mid-infrared (MIR) range provides simultaneous morphological and chemical information of a wide variety of samples. However, current MIR technologies struggle to produce high-definition images over a broad spectral…

Optical frequency combs paved the way for fast and compact multi-component optical chemical analysis due to their broadband spectra. Dual-comb spectrometers embody this technology, but their design requires a pair of matched combs, adding…

Optics · Physics 2025-09-25 Ina Heckelmann , Davide Pinto , Uwe Schmitt , Mattias Beck , Jérôme Faist

We demonstrate balanced-detection dual-comb spectroscopy (DCS) using two free-running mechanical sharing dual-comb fiber lasers assisted by an all-computational digital phase correction algorithm. The mutual coherence between the combs…

The quest for extrasolar planets and their characterisation as well as studies of fundamental physics on cosmological scales rely on capabilities of high-resolution astronomical spectroscopy. A central requirement is a precise wavelength…