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Variational algorithms for strongly correlated chemical and materials systems are one of the most promising applications of near-term quantum computers. We present an extension to the variational quantum eigensolver that approximates the…

Quantum Physics · Physics 2020-08-26 William J. Huggins , Joonho Lee , Unpil Baek , Bryan O'Gorman , K. Birgitta Whaley

The technological performances of metallic compounds are largely influenced by atomic ordering. Although there is a general consensus that successful theories of metallic systems should account for the quantum nature of the electronic glue,…

Materials Science · Physics 2015-05-13 Ezio Bruno , Francesco Mammano , Beniamino Ginatempo

We conduct a numerical investigation of structural order in the shifted-force Lennard-Jones system by calculating metrics of translational and bond-orientational order along various paths in the phase diagram covering equilibrium solid,…

Statistical Mechanics · Physics 2009-11-07 Jeffrey R. Errington , Pablo G. Debenedetti , Salvatore Torquato

Many methods for computing electronic correlation effects at finite temperature are related to many-body perturbation theory in the grand-canonical ensemble. In most applications, however, the average number of electrons is known rather…

Materials Science · Physics 2022-10-21 Felix Hummel

Quantum entanglement is a particularly useful characterization of topological orders which lack conventional order parameters. In this work, we study the entanglement in topologically ordered states between two arbitrary spatial regions,…

Strongly Correlated Electrons · Physics 2023-08-01 Chao Yin , Shang Liu

We suggest two metrics for assessing the quality of atomistic configurations of disordered materials, both of which are based on quantifying the orientational distribution of neighbours around each atom in the configuration. The first…

Materials Science · Physics 2012-11-20 Matthew J. Cliffe , Andrew L. Goodwin

This paper focuses on systems of nonlinear second-order stochastic differential equations with multi-scales. The motivation for our study stems from mathematical physics and statistical mechanics, for examples, Langevin dynamics and…

Probability · Mathematics 2024-04-08 Nhu N. Nguyen , George Yin

In pursuit of a minimal basis for systems with non-ideal bond angles, in this work we try to pinpoint the exact orientation of the major overlapping orbitals along the nearest neighbouring coordination segments in a given system such that…

Materials Science · Physics 2022-09-14 Joydev De , Sujith N S , Manoar Hossain , Joydeep Bhattacharjee

Predictive high-fidelity finite element simulations of human cardiac mechanics co\-mmon\-ly require a large number of structural degrees of freedom. Additionally, these models are often coupled with lumped-parameter models of hemodynamics.…

Computational Engineering, Finance, and Science · Computer Science 2020-02-18 Martin R. Pfaller , Maria Cruz Varona , Johannes Lang , Cristóbal Bertoglio , Wolfgang A. Wall

Three-parametric Lenard-Jones and Morse interatomic potentials are the simplest ones, which that can be used to obtain thermophysical properties of the liquid and solid substances. Upon adjusting the model parameters to real substance…

Materials Science · Physics 2022-09-29 A. A. Likhachev , Yu. N. Koval , T. G. Sych , V. A. Tatarenko

The stability of antiferromagnetic long-range order against quenched disorder is considered. A simple model of an antiferromagnet with a spatially varying Neel temperature is shown to possess a nontrivial fixed point corresponding to…

Statistical Mechanics · Physics 2009-10-28 T. R. Kirkpatrick , D. Belitz

Phase diagrams exhibiting extended solid-solution and lens-like melting are often reproduced using ideal solutions, where ideal mixing considers a fully random configurational entropy of mixing. In the field of irreversible thermodynamics,…

Materials Science · Physics 2024-02-06 Jonathan Paras , Antoine Allanore

We consider various incommensurate (IC) order parameters for electrons on a square lattice which reduce to $d_{x^2-y^2}$-density wave (DDW) order when the ordering wavevector ${\bf Q}\to (\pi,\pi)$. We describe the associated charge and…

Superconductivity · Physics 2007-05-23 Ivailo Dimov , Chetan Nayak

We investigate the nature of quantum entanglement in long-range orders and spontaneous symmetry breaking. It is shown that diminishing of entanglement between the condensate mode and the rest of the system underlies off-diagonal long-range…

Condensed Matter · Physics 2009-11-07 Yu Shi

A new notion is introduced of matrix order indices which relate the matrix norm and its trace. These indices can be defined for any given matrix. They are especially important for matrices describing many-body systems, equilibrium as well…

Condensed Matter · Physics 2009-11-07 V. I. Yukalov

We model two-dimensional crystals by a configuration space in which every admissible configuration is a hard disk configuration and a perturbed version of some triangular lattice with side length one. In this model we show that, under the…

Mathematical Physics · Physics 2014-05-14 Alexisz Tamás Gaál

In the present paper, we have studied atomic structure of nitrogenous austenite. High precision ab-initio calculation was utilized for the calculation of the pair potentials of interatomic interactions N-N in FCC Fe lattice. These…

Atomic and Molecular Clusters · Physics 2011-12-01 A. N. Timoshevskii , S. O. Yablonovskii

Variations with oxygen concentration of titanium lattice parameters are obtained by means of ab initio calculations, considering the impact of oxygen ordering. The quasiharmonic approximation is used to take into account the thermal…

We describe a Monte Carlo scheme which, in a single simulation, yields a measurement of the chemical potential of a crystalline solid. Within the isobaric ensemble, this immediately provides an estimate of the system free energy, with…

Statistical Mechanics · Physics 2015-06-11 Nigel B. Wilding , Peter Sollich

A model subspace configuration interaction method is developed to obtain chemically accurate electron correlations by diagonalising a very compact effective Hamiltonian of realistic molecule. The construction of the effective Hamiltonian is…

Chemical Physics · Physics 2022-10-18 Jiasheng Li , Jun Yang