Related papers: Nonlinear light-matter interaction at terahertz fr…
The interplay of electric charge, spin, and orbital polarizations, coherently driven by picosecond long oscillations of light fields in spin-orbit coupled systems, is the foundation of emerging terahertz spintronics and orbitronics. The…
The induced terahertz response of semiconductor systems is investigated with a microscopic theory. In agreement with recent terahertz experiments, the developed theory fully explains the ultrafast build up of the plasmon resonance and the…
The dynamic control of novel states of matter beyond thermodynamic equilibrium is a fundamental pursuit in condensed matter physics. Intense terahertz fields have enabled metal-insulator transitions, superconductivity, quantum paraelectric…
Metasurfaces represent a new frontier in materials science paving for unprecedented methods of controlling electromagnetic waves, with a range of applications spanning from sensing to imaging and communications. For pulsed terahertz…
Modern laser sources nowadays deliver ultrashort light pulses reaching few cycles in duration, high energies beyond the Joule level and peak powers exceeding several terawatt (TW). When such pulses propagate through optically-transparent…
The feasibility to generate correlated photon pairs at variable frequencies is investigated. For this purpose, we consider the interaction of an off-resonant laser field with a two-level system possessing broken inversion symmetry. We show…
Recently developed terahertz (THz) two-dimensional coherent spectroscopy (2DCS) is a powerful technique to obtain materials information in a fashion qualitatively different from other spectroscopies. Here, we utilized THz 2DCS to…
Excitation of coherent optical phonons in solids provides a pathway for ultrafast modulation of light on a sub-ps timescale. Here, we report on efficient 3.6 THz modulation of light reflected from hybrid metal/semiconductor plasmonic…
We theoretically investigate photo-excitation of electron-hole pairs and high harmonic generation in the bulk of zinc oxide (ZnO) subjected to intense femto-second laser pulses with mid-infrared wavelength. The main microscopic mechanism of…
Many applications in photonics require all-optical manipulation of plasma waves, which can concentrate electromagnetic energy on sub-wavelength length scales. This is difficult in metallic plasmas because of their small optical…
The recent observation of a transmitted Thz pulse oscillating at three times the frequency of the incident light paves the way to a new protocol to access resonant excitations in a superconductor. Here we show that this non-linear optical…
Ultra-intense laser-matter interactions are often difficult to predict from first principles because of the complexity of plasma processes and the many degrees of freedom relating to the laser and target parameters. An important approach to…
Coherent control of quantum materials has progressed along two major fronts: nonlinear phononics, which reshapes lattices to induce emergent states, and Floquet engineering, which tailors electronic band reconstruction via time-periodic…
To explore the capabilities of metallic spintronic thin-film stacks as a source of intense and broadband terahertz electromagnetic fields, we excite a W/CoFeB/Pt trilayer on a large-area glass substrate (diameter of 7.5 cm) by a femtosecond…
Adoption of terahertz technologies is hindered by the lack of cost-effective THz sources. Here we demonstrate a fundamentally new way to generate and control THz radiation, via spatio-temporal emissivity modulation. By patterning the…
The brightness of a light source defines its applicability to nonlinear phenomena in science. Bright low frequency terahertz (< 5THz) radiation confined to a diffraction-limited spot size is a present hurdle due to the broad bandwidth and…
A free electron can temporarily gain a very significant amount of energy if it is overrun by an intense electromagnetic wave. In principle, this process would permit large enhancements in the center-of-mass energy of electron-electron,…
We refine the method towards extraction of sub-cycle transients in the 0.1-1 THz frequency (mm-wavelength) range from optical rectification in lithium niobate using tilted pulse fronts. Our scheme exploits previously unexplored…
Irradiation of solid surfaces with intense ultrashort laser pulses represents a unique way of depositing energy into materials. It allows to realize states of extreme electronic excitation and/or very high temperature and pressure, and to…
Self-phase modulation (SPM) of light pulses is found to occur strongly, at low incident intensities, in the coupling of light with superconductors. We develop a theory from a synthesis of the time-dependent Ginzburg-Landau (TDGL) equation…