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We study the structure of the energy spectra along with the character of the states participating in optical transitions in colloidal CdS quantum dots (QDs) using the {\sl ab initio} accuracy charge patching method combined with the…

Materials Science · Physics 2009-11-11 D. O. Demchenko , Lin-Wang Wang

The photoluminescence spectra of spherical CdTe nanocrystals with zincblende structure are studied by size-selective spectroscopic techniques. We observe a resonant Stokes shift of 15 meV when the excitation laser energy is tuned to the red…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Perez-Conde , A. K. Bhattacharjee , M. Chamarro , P. Lavallard , V. D. Petrikov , A. A. Lipovskii

The mechanism of Stokes shift in semiconductor quantum dots is investigated by calculating the energy of the excitonic states. We have taken into account all possible contributions to the total electronic energy in the dot, i.e, dielectric…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Anjana Bagga , P. K. Chattopadhyay , Subhasis Ghosh

A transition from a cylindrical quantum dot to a highly elongated quantum dash is theoretically studied here with an atomistic approach combining empirical tight binding for single particle states and configuration interaction method for…

Mesoscale and Nanoscale Physics · Physics 2019-05-08 Michał Zieliński

Excitonic fine structure splitting in quantum dots is closely related to the lateral shape of the wave functions. We have studied theoretically the fine structure splitting in InAs quantum dots with a type-II confinement imposed by a GaAsSb…

Mesoscale and Nanoscale Physics · Physics 2015-12-02 Vlastimil Křápek , Petr Klenovský , Tomáš Šikola

We evaluate the optical gap and Stokes shift of several candidate 1 nm silicon nanocrystal structures using density functional and quantum Monte Carlo (QMC) methods. We find that the combination of absorption gap calculations and Stokes…

Although both epitaxial quantum dots (QDs) and colloidal nanocrystals (NCs) are quantum-confined semiconductor nanostructures, so far they have demonstrated dramatically-different exciton fine structure splittings (FSSs) at the cryogenic…

Mesoscale and Nanoscale Physics · Physics 2017-07-19 Chunyang Yin , Liyang Chen , Yan Lv , Fengrui Hu , Chun Sun , William W. Yu , Chunfeng Zhang , Xiaoyong Wang , Yu Zhang , Min Xiao

The energy levels and optical transitions of tetrahedral core/shell InP/ZnSe quantum dots (QDs) are investigated by means of multi-band k$\cdot$p theory. Despite the $\overline{T}_d$ symmetry relaxing spherical selection rules, the…

Mesoscale and Nanoscale Physics · Physics 2026-04-06 Josep Planelles , Juan I. Climente

Polariton emission from optical cavities integrated with various luminophores has been extensively studied recently due to the wide variety of possible applications in photonics, particularly promising in terms of fabrication of…

Mesoscale and Nanoscale Physics · Physics 2021-07-28 Dmitriy Dovzhenko , Maksim Lednev , Konstantin Mochalov , Ivan Vaskan , Pavel Samokhvalov , Yury Rakovich , Igor Nabiev

We report on stacked multiple quantum dots (QDs) formed inside inverted pyramidal recesses, which allow for the precise positioning of the QDs themselves. Specifically we fabricated double QDs with varying inter-dot distance and ensembles…

Mesoscale and Nanoscale Physics · Physics 2017-09-01 S. T. Moroni , T. H. Chung , G. Juska , A. Gocalinska , E. Pelucchi

We investigate theoretically the spin splitting of the exciton states in semiconductor coupled quantum dots (CQDs) containing a single magnetic ion. We find that the spin splitting can be switched on/off in the CQDs \textit{via} the…

Materials Science · Physics 2009-11-13 Xiaojing Li , Kai Chang

The exciton-exciton interaction energy of Tellurium doped CdSe colloidal quantum dots is experimentally investigated. The dots exhibit a strong Coulomb repulsion between the two excitons, which results in a huge measured biexciton blue…

Materials Science · Physics 2015-05-13 Assaf Avidan , Dan Oron

We study the size-dependent exciton fine structure in monolayer black phosphorus quantum dots (BPQDs) deposited on different substrates (isolated, Si and SiO$_2$) using a combination of tight-binding method to calculate the single-particle…

Mesoscale and Nanoscale Physics · Physics 2017-07-19 J. S. de Sousa , M. A. Lino , D. R. da Costa , A. Chaves , J. M. Pereira , G. A. Farias

Surface defects in colloidal quantum dots are a major source of nonradiative losses, yet the microscopic mechanisms underlying exciton trapping and recombination remain elusive. Here, we develop a model Hamiltonian based on atomistic…

Chemical Physics · Physics 2025-05-13 Bokang Hou , Salvatore Gatto , Samuel L. Rudge , Johan E. Runeson , Michael Thoss , Eran Rabani

The authors report that anisotropic confining potentials in laterally-coupled semiconductor quantum dots (QDs) have large impacts in optical transitions and energies of inter-shell collective electronic excitations. The observed…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Achintya Singha , Vittorio Pellegrini , Sokratis Kalliakos , Biswajit Karmakar , Aron Pinczuk , Loren N. Pfeiffer , Ken W. West

Colloidal quantum dots (QDs) of group III-V are considered as promising candidates for next-generation environmentally friendly light emitting devices, yet there appears to be only limited understanding of the underlying electronic and…

Materials Science · Physics 2019-12-11 Xiaoyu Ma , Jingjing Min , Zaiping Zeng , Christos S. Garoufalis , Sotirios Baskoutas , Yu Jia , Zuliang Du

Colloidal quantum dots (QDs) integrated with waveguide-coupled dielectric resonators are promising building blocks for compact on-chip light sources. However, deterministic placement of QDs with strong mode overlap at the desired location…

Hereby, we present a comprehensive experimental and theoretical study of the electronic structure and optical properties of excitonic complexes in strain-engineered InGaAs/GaAs quantum dots (QDs) grown by metal-organic chemical vapour…

We theoretically study the effects of bias-controlled interdot tunneling in vertically coupled quantum dots on the emission properties of spin excitons in various bias-controlled tunneling regimes. As a main result, for strongly coupled…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Hanz Y. Ramirez , Shun-Jen Cheng

Unique optical properties of colloidal semiconductor quantum dots (QDs), arising from quantum mechanical confinement of charge within these structures, present a versatile testbed for the study of how high electric fields affect the…

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