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Layered two-dimensional (2D) semiconductors such as molybdenum disulfide (MoS2) have recently attracted remarkable attention because of their unique physical properties. Here, we use photoluminescence (PL) and Raman spectroscopy to study…

Two-dimensional Transition-Metal Dichalcogenides (TMDs) are of great interest for second harmonic (SH) generation due to their large second-order susceptibility, atomically thin structure, and relaxed phase-matching conditions. TMDs are…

In many-cycle plane waves at intermediate intensities, the nonlinear trident process can be well-approximated by the two sequential steps of nonlinear Compton scattering of a polarised real photon followed by its transformation into an…

High Energy Physics - Phenomenology · Physics 2023-05-11 S. Tang , B. King

Topology-driven nonlinear light-matter effects open up new paradigms for both topological photonics and nonlinear optics. Here, we propose to achieve high-efficiency second-harmonic generation in a second-order photonic topological…

Optics · Physics 2021-12-02 Yafeng Chen , Zhihao Lan , Jensen Li , Jie Zhu

We employ transformation optics to optimize the generic nonlinear wave interaction of second-harmonic generation from a pair of touching metallic wires. We demonstrate a 10 orders of magnitude increase in the second-harmonic scattering…

Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…

Mesoscale and Nanoscale Physics · Physics 2020-07-03 E. A. Stepanov , S. V. Semin , C. R. Woods , M. Vandelli , A. V. Kimel , K. S. Novoselov , M. I. Katsnelson

In moir\'e crystals resulting from the stacking of twisted two-dimensional (2D) layered materials, a subtle adjustment in the twist angle surprisingly gives rise to a wide range of correlated optical and electrical properties. Herein, we…

Transition metal dichalcogenides (TMDs) are layered materials which show excellent potential for nanoelectronic and optoelectronic applications. However, as many of the exciting features of these materials are controlled by the anharmonic…

Materials Science · Physics 2021-08-13 Suvodeep Paul , Saheb Karak , Annie Mathew , Ankita Ram , Surajit Saha

Atomically thin two dimensional (2D) layered materials have emerged as a new class of material for nanoelectromechanical systems (NEMS) due to their extraordinary mechanical properties and ultralow mass density. Among them, graphene has…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 C. Samanta , P. R. Yasasvi Gangavarapu , A. K. Naik

Due to the absence of interlayer coupling and inversion symmetry, transition metal dichalcogenide (MX$_2$) semiconductor monolayers exhibit novel properties that are distinctly different from their bulk crystals such as direct optical band…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Chung-Yu Wang , Guang-Yu Guo

The bulk photovoltaic effect in noncentrosymmetric materials is an intriguing physical phenomenon that holds potential for high-efficiency energy harvesting. Here, we study the shift current bulk photovoltaic effect in the transition metal…

Materials Science · Physics 2021-01-28 Aaron M. Schankler , Lingyuan Gao , Andrew M. Rappe

Two-dimensional (2D) layered transition metal dichalcogenides (TMDs) have emerged as promising materials for electronic, optoelectronic, and valleytronic applications. Recent work suggests drastic changes of the band gap and exciton binding…

Mesoscale and Nanoscale Physics · Physics 2017-08-02 Eric Parzinger , Martin Hetzl , Ursula Wurstbauer , Alexander W. Holleitner

Light modulation is an essential operation in photonics and optoelectronics. With existing and emerging technologies increasingly demanding compact, efficient, fast and broadband optical modulators, high-performance light modulation…

Optics · Physics 2016-05-04 Zhipei Sun , Amos Martinez , Feng Wang

Using Time-Dependent Density Functional Theory (TDDFT) nonlinear nonperturbative response of the molecular system is studied for photoisomerization reaction. The 1,3-cyclohexadiene photoisomerization is probed by the high-harmonic…

Chemical Physics · Physics 2024-08-06 Lauren Bauerle , Agnieszka Jaron

We study the properties of a tunable nonlinear metamaterial operating at microwave frequencies. We fabricate the nonlinear metamaterial composed of double split-ring resonators and wires where a varactor diode is introduced into each…

Nonlinear optical (NLO) phenomena such as harmonic generation, Kerr, and Pockels effects are of great technological importance for lasers, frequency converters, modulators, switches, etc. Recently, two-dimensional (2D) materials have drawn…

Nonlinear optical processes associated with even-order nonlinear susceptibilities are critical for both classical and quantum technologies. Inversion symmetry, however, prevents nonlinear optical responses mediated by even-order…

Optics · Physics 2022-02-24 Davis M. Welakuh , Prineha Narang

We have studied on optical second harmonic generations (SHGs) from atomically thin MoTe2 flakes with 2H and 1T' phases. From 2H-MoTe2 samples with odd (even) numbers of layers, strong (negligible) SHGs are observed due to the…

Optics · Physics 2018-05-25 Yu Song , Ruijuan Tian , Jiulong Yang , Rui Yin , Jianlin Zhao , Xuetao Gan

Since the discovery of the laser, optical parametric nonlinearities have been at the core of efficient light conversion sources. Typically, thick transparent crystals or quasi-phase matched waveguides, are utilized in conjunction with…

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…