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Self-phoretic Janus particles move by inducing -- via non-equilibrium chemical reactions occurring on their surfaces -- changes in the chemical composition of the solution in which they are immersed. This process leads to gradients in…

Soft Condensed Matter · Physics 2018-01-30 W. E. Uspal , M. N. Popescu , M. Tasinkevych , S. Dietrich

Catalytically active Janus particles suspended in solution create gradients in the chemical composition of the solution along their surfaces, as well as along any nearby container walls. The former leads to self-phoresis, while the latter…

Soft Condensed Matter · Physics 2016-09-22 W. E. Uspal , M. N. Popescu , S. Dietrich , M. Tasinkevych

Micron-sized particles moving through solution in response to self-generated chemical gradients serve as model systems for studying active matter. Their far-reaching potential applications will require the particles to sense and respond to…

Soft Condensed Matter · Physics 2016-03-09 W. E. Uspal , M. N. Popescu , S. Dietrich , M. Tasinkevych

An interacting pair of chemotactic (anti-chemotactic) active colloids, that can rotate their axes of self-propulsion to align {parallel (anti-parallel)} to a chemical gradient, shows dynamical behaviour that varies from bound states to…

Biological Physics · Physics 2025-10-08 Suropriya Saha , Sriram Ramaswamy , Ramin Golestanian

Many biological microswimmers are capable of chemotaxis, i.e., they can sense an ambient chemical gradient and adjust their mechanism of motility to move towards or away from the source of the gradient. Synthetic active colloids endowed…

Soft Condensed Matter · Physics 2024-06-18 Viviana Mancuso , Mihail N. Popescu , William E. Uspal

Catalytically active colloids maintain non-equilibrium conditions in which they produce and deplete chemicals and hence effectively act as sources and sinks of molecules. While individual colloids that are symmetrically coated do not…

Soft Condensed Matter · Physics 2015-06-11 Rodrigo Soto , Ramin Golestanian

Various aspects of self-motility of chemically active colloids in Newtonian fluids can be captured by simple models for their chemical activity plus a phoretic slip hydrodynamic boundary condition on their surface. For particles of simple…

Soft Condensed Matter · Physics 2018-04-09 M. N. Popescu , W. E. Uspal , Z. Eskandari , M. Tasinkevych , S. Dietrich

Janus particles self-propel by generating local tangential concentration gradients along their surface. These gradients are present in a thin layer whose thickness is small compared to the particle size. Chemical asymmetry along the surface…

Soft Condensed Matter · Physics 2021-03-31 Prathmesh M. Vinze , Akash Choudhary , S. Pushpavanam

We study a mesoscopic model of a chemically active colloidal particle which on certain parts of its surface promotes chemical reactions in the surrounding solution. For reasons of simplicity and conceptual clarity, we focus on the case in…

Soft Condensed Matter · Physics 2017-07-25 G. Oshanin , M. N. Popescu , S. Dietrich

Chemotaxis, i.e. motion generated by chemical gradients, is a motility mode shared by many living species that has been developed by evolution to optimize certain biological processes such as foraging or immune response. In particular,…

Soft Condensed Matter · Physics 2023-05-24 Hugues Meyer , Heiko Rieger

The creation of synthetic systems that emulate the defining properties of living matter, such as motility, gradient-sensing, signalling and replication, is a grand challenge of biomimetics. Such imitations of life crucially contain active…

Soft Condensed Matter · Physics 2015-06-17 Suropriya Saha , Ramin Golestanian , Sriram Ramaswamy

Conspectus: The ability to navigate in chemical gradients, called chemotaxis, is crucial for the survival of microorganisms. It allows them to find food and to escape from toxins. Many microorganisms can produce the chemicals to which they…

Soft Condensed Matter · Physics 2018-10-03 Benno Liebchen , Hartmut Löwen

A heterogeneous and dilute suspension of catalytically active colloids is studied as a non-equilibrium analogue of ionic systems, which has the remarkable feature of action-reaction symmetry breaking. Symmetrically coated colloids are found…

Soft Condensed Matter · Physics 2015-06-16 Rodrigo Soto , Ramin Golestanian

Active particles with their characteristic feature of self-propulsion are regarded as the simplest models for motility in living systems. The accumulation of active particles in low activity regions has led to the general belief that…

Soft Condensed Matter · Physics 2021-05-26 Hidde D. Vuijk , Holger Merlitz , Michael Lang , Abhinav Sharma , Jens-Uwe Sommer

We consider a rigid assembly of two active Brownian particles, forming an active colloidal dimer, in a gradient of activity. We show analytically that depending on the relative orientation of the two particles the active dimer accumulates…

Soft Condensed Matter · Physics 2022-08-17 Hidde D. Vuijk , Sophie Klempahn , Holger Merlitz , Jens-Uwe Sommer , Abhinav Sharma

At the surfaces of autophoretic colloids, slip velocities arise from local chemical gradients that are many-body functions of particle configuration and activity. For rapid chemical diffusion, coupled with slip-induced hydrodynamic…

Soft Condensed Matter · Physics 2019-07-29 Rajesh Singh , R. Adhikari , M. E. Cates

While the behavior of active colloidal molecules is well studied by now for a constant activity, the effect of activity gradients is much less understood. Here we explore one of the simplest molecules in activity gradients, namely active…

Soft Condensed Matter · Physics 2022-10-19 Pietro Luigi Muzzeddu , Hidde Derk Vuijk , Hartmut Lowen , Jens-Uwe Sommer , Abhinav Sharma

We consider sedimented at a solid wall particles that are immersed in water containing small additives of photosensitive ionic surfactants. It is shown that illumination with an appropriate wavelength, a beam intensity profile, shape and…

The past two decades have seen a remarkable progress in the development of synthetic colloidal agents which are capable of creating directed motion in an unbiased environment at the microscale. These self-propelling particles are often…

Soft Condensed Matter · Physics 2023-02-10 Benno Liebchen , Aritra K. Mukhopadhyay

We study the diffusiophoretic self-propulsion of a colloidal catalytic particle due to a surface chemical reaction in a vicinity of a solid wall. Diffusiophoresis is a chemico-mechanical transduction mechanism in which a concentration…

Soft Condensed Matter · Physics 2016-06-22 Ali Mozaffari , Nima Sharifi-Mood , Joel Koplik , Charles Maldarelli
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