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The dream of room temperature superconductors has inspired intense research effort to find routes for enhancing the superconducting transition temperature (Tc). Therefore, single-layer FeSe on a SrTiO3 substrate, with its extraordinarily…

Superconductivity · Physics 2019-03-12 Q. Song , T. L. Yu , X. Lou , B. P. Xie , H. C. Xu , C. H. P. Wen , Q. Yao , S. Y. Zhang , X. T. Zhu , J. D. Guo , R. Peng , D. L. Feng

In a recent experiment the superconducting gap of a single unit cell thick FeSe film on SrTiO$_3$ substrate is observed by scanning tunneling spectroscopy and angle-resolved photoemission spectroscopy. The value of the superconducting gap…

Superconductivity · Physics 2012-10-09 Fa Wang , Yuan-Yuan Xiang , Da Wang , Qiang-Hua Wang , Dung-Hai Lee

We show that electron-phonon coupling can induce strong electron pairing in an FeSe monolayer on a SrTiO3 substrate (experimental indications for superconducting Tc are between 65 and 109K). The role of the SrTiO3 substrate in increasing…

Superconductivity · Physics 2015-07-27 Sinisa Coh , Marvin L. Cohen , Steven G. Louie

We examine the impact of interfacial phonons on the superconducting state of FeSe/SrTiO$_3$ developing a material's specific multiband, full bandwidth, and anisotropic Eliashberg theory for this system. Our self-consistent calculations…

Superconductivity · Physics 2018-02-07 Alex Aperis , Peter M. Oppeneer

While a predictive theory for unconventional superconductivity in Fe-based superconductors remains elusive, an extensively debated aspect is the interaction between phonons and strongly correlated electrons, and its potential role in the…

Strongly Correlated Electrons · Physics 2025-06-30 Qiang Zou , Antik Sihi , Basu Dev Oli , Mercè Roig , Daniel Agterberg , Michael Weinert , Lian Li , Subhasish Mandal

Observation of replica bands in the ARPES spectra of the single-layer FeSe on strontium titanate substrate revealed a phonon component among mechanisms behind high Tc superconductivity there. We study the interaction of the in-layer FeSe…

Superconductivity · Physics 2016-02-24 Lev P. Gor'kov

Mono- and multilayer FeSe thin films grown on SrTiO$_\mathrm{3}$ and BiTiO$_\mathrm{3}$ substrates exhibit a greatly enhanced superconductivity over that found in bulk FeSe. A number of proposals have been advanced for the mechanism of this…

Superconductivity · Physics 2016-05-04 Y. Wang , K. Nakatsukasa , L. Rademaker , T. Berlijn , S. Johnston

The discovery of high-temperature (Tc) superconductivity in monolayer FeSe on SrTiO3 raised a fundamental question whether high Tc is commonly realized in monolayer iron-based superconductors. Tetragonal FeS is a key material to resolve…

The interface-enhanced superconductivity in monolayer iron selenide (FeSe) films on SrTiO3 has been actively pursued in the past decade. Although a synergistic effect between interfacial charge transfer and interfacial electron-phonon…

The significant role of interfacial coupling on the superconductivity enhancement in FeSe films on SrTiO3 has been widely recognized. But the explicit origination of this coupling is yet to be identified. Here by surface phonon measurements…

Monolayer FeSe/TiO$_x$ and FeSe/FeO$_x$ interfaces exhibit significant superconductivity enhancement compared to bulk FeSe, with interfacial electron-phonon coupling (EPC) playing a crucial role. However, the reduced dimensionality in…

Distinctive superconducting behaviors between bulk and monolayer FeSe make it challenging to obtain a unified picture of all FeSe-based superconductors. We investigate the ultrafast quasiparticle (QP) dynamics of an intercalated…

Superconductivity · Physics 2020-09-08 Q. Wu , H. X. Zhou , Y. L. Wu , L. L. Hu , S. L. Ni , Y. C. Tian , F. Sun , F. Zhou , X. L. Dong , Z. X. Zhao , Jimin Zhao

Alkali-metal (potassium) adsorption on FeSe thin films with thickness from two unit cells (UC) to 4-UC on SrTiO3 grown by molecular beam epitaxy is investigated with a low-temperature scanning tunneling microscope. At appropriate potassium…

It was observed recently (K. Shigekawa et al, PNAS 116, 2470 (2019)) that while monolayer iron chalcigenide FeSe on SrTiO3 (STO) substrate has a very high critical temperature, its chemical and structural "twin" material FeS=STO has a very…

Superconductivity · Physics 2021-06-23 Baruch Rosenstein , B. Ya. Shapiro

The mechanism of enhanced superconductivity in the one unit-cell (1UC) FeSe film on a SrTiO3 (STO) substrate has stimulated significant research interest but remains elusive. Using low-temperature, voltage-gated Raman spectroscopy and…

A subtle balance between competing interactions in strongly correlated systems can be easily tipped by additional interfacial interactions in a heterostructure. This often induces exotic phases with unprecedented properties, as recently…

The pairing mechanism in iron-based superconductors is believed to be unconventional, i.e. not phonon-mediated. The achieved transition temperatures Tc in these superconductors are still significantly below those of some of the cuprates,…

We study the effect of combining spin fluctuations and forward scattering electron-phonon ({\eph}) coupling on the superconductivity in the FeSe/SrTiO$_3$ system modeled by a phenomenological two-band Hubbard model with long-range {\eph}…

Superconductivity · Physics 2021-04-14 Louk Rademaker , Gustavo Alvarez-Suchini , Ken Nakatsukasa , Yan Wang , Steven Johnston

The quasiparticle relaxation dynamics of the iron-based superconductor CsCa$_2$Fe$_4$As$_4$F$_2$ ($T_c$ $\sim$ 29 K) were investigated using ultrafast optical spectroscopy. A pseudogap ($\Delta_{PG}$ $\approx$ 3.3 meV) was observed to open…

We use ultrafast optical spectroscopy to study the nonequilibrium quasiparticle relaxation dynamics of the iron-based superconductor KCa$_2$Fe$_4$As$_4$F$_2$ with $T_c=33.5$ K. Our results reveal a possible pseudogap ($\Delta_{PG}$ = 2.4…

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