Related papers: Few-cycle pulse-driven excitation response of reso…
Coherent control with shaped ultrafast pulses is a powerful approach for steering nonlinear light-matter interactions. Previous studies in quantum control have shown that, beyond transform-limited pulses, those with antisymmetric spectral…
The correlated behavior of electrons determines the structure and optical properties of molecules, semiconductor and other systems. Valuable information on these correlations is provided by measuring the response to femtosecond laser…
We experimentally demonstrate a novel nonlinear effect in optical fibers: upconversion luminescence generation excited by multiphoton absorption of femtosecond infrared pulses. We directly estimate the average number of photons involved in…
Recent experimental work has demonstrated optical control of spin wave emission by tuning the shape of the optical pulse (Satoh et al.\ Nature Photonics, 6, 662 (2012)). We reproduce these results and extend the scope of the control by…
The interaction of coherent nonlinear structures (such as sub-cycle solitons, electron vortices and wake Langmuir waves) with a strong wake wave in a collisionless plasma can be exploited in order to produce ultra-short electromagnetic…
We show that the recently demonstrated technique for generating stationary pulses of light [Nature {\bf 426}, 638 (2003)] can be extended to localize optical pulses in all three spatial dimensions in a resonant atomic medium. This method…
We experimentally demonstrate coherent control of the nonlinear response of optical second harmonic generation in resonant nanostructures beyond the weak-field regime. Contrary to common perception, we show that maximizing the intensity of…
A dielectric material's response to light is macroscopically described by electric displacement fields due to polarization and susceptibility, but the atomistic origin is light-cycle-driven motion of electron densities in the restoring…
Nonlinear electron emission processes induced by surface plasmon oscillations have been studied both experimentally and theoretically. The measured above-threshold electron spectra extend up to energies whose appearance cannot be explained…
The interaction of optical fields sculpted on the nano-scale with matter may not be described by the dipole approximation since the fields vary appreciably across the molecular length scale. Rather than incrementally adding higher…
Calculation of the coherent nonlinear response of a system is essential to correctly interpret results from advanced techniques such as two-dimensional coherent spectroscopy (2DCS). Usually, even for the simplest systems, such calculations…
We study the propagation of few-cycle pulses in two-component medium consisting of nonlinear amplifying and absorbing two-level centers embedded into a linear and conductive host material. First we present a linear theory of propagation of…
We show that a laser pulse can always be found that induces a desired optical response from an arbitrary dynamical system. As illustrations, driving fields are computed to induce the same optical response from a variety of distinct systems…
Propagation of the extremely short electromagnetic pulse in non-linear dielectric media without the slowly varying envelope approximation is discussed. The models under consideration take into account both resonant and not-resonant…
Nonlinear optical responses provide a powerful way to understand the microscopic interactions between laser fields and matter. They are critical for plenty of applications, such as in lasers, integrated photonic circuits, biosensing and…
We investigate theoretically the ability of an optical centrifuge - a laser pulse whose linear polarization is rotating at an accelerated rate, to control molecular rotation in the regime when the rigid-rotor approximation breaks down due…
New phenomenon of temporal oscillations of nonlinear Faraday rotation in a driven four-level system is predicted. We show that in this system with one upper level, under the conditions of electromagnetically induced transparency created by…
A novel point of view on the phenomenon of self-pulsations is presented, which shows that they are a balanced state formed by two counteracting processes: beating of modes and bistable switching. A structure based on two coupled nonlinear…
Circularly-polarized light is well-known to induce, or flip the direction of, magnetization in solids. At its heart, this arises from time-reversal symmetry breaking by the vector potential, causing inverse-Faraday or analogous physical…
Intense multi-THz pulses are used to study the coherent nonlinear response of bulk InSb by means of field-resolved four-wave mixing spectroscopy. At amplitudes above 5 MV/cm the signals show a clear temporal substructure which is unexpected…