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We study the dynamical decay of the van Hove function of Brownian hard spheres using event-driven Brownian dynamics simulations and dynamic test particle theory. Relevant decays mechanisms include deconfinement of the self particle, decay…

Soft Condensed Matter · Physics 2022-04-20 Lucas L. Treffenstädt , Thomas Schindler , Matthias Schmidt

We demonstrate that the time evolution of the van Hove dynamical pair correlation function is governed by adiabatic forces that arise from the free energy and by superadiabatic forces that are induced by the flow of the van Hove function.…

Soft Condensed Matter · Physics 2021-02-24 Lucas L. Treffenstädt , Matthias Schmidt

Using Brownian dynamics computer simulations we investigate the dynamics of the one-body density and one-body current in a one-dimensional system of particles that interact with a repulsive Gaussian pair potential. We systematically split…

Soft Condensed Matter · Physics 2016-08-05 Elias Bernreuther , Matthias Schmidt

Superadiabatic dynamical density functional theory (superadiabatic-DDFT), a first-principles approach based on the inhomogeneous two-body correlation functions, is employed to investigate the response of interacting Brownian particles to…

Soft Condensed Matter · Physics 2023-06-23 S. M. Tschopp , H. D. Vuijk , J. M. Brader

Using dynamical density functional theory (DDFT), we theoretically study Brownian self-diffusion and structural relaxation of hard disks and compare to experimental results on quasi two-dimensional colloidal hard spheres. To this end, we…

Soft Condensed Matter · Physics 2018-04-04 Daniel Stopper , Alice Thorneywork , Roel Dullens , Roland Roth

We show that one may view the self and the distinct part of the van Hove dynamic correlation function of a simple fluid as the one-body density distributions of a binary mixture that evolve in time according to dynamical density functional…

Soft Condensed Matter · Physics 2011-11-09 Andrew J. Archer , Paul Hopkins , Matthias Schmidt

For classical many-body systems subject to Brownian dynamics we develop a superadiabatic dynamical density functional theory (DDFT) for the description of inhomogeneous fluids out-of-equilibrium. By explicitly incorporating the dynamics of…

Soft Condensed Matter · Physics 2022-12-20 S. M. Tschopp , J. M. Brader

Two-time correlations are a crucial tool to probe the dynamics of many-body systems. We use these correlation functions to study the dynamics of dissipative quantum systems. Extending the adiabatic elimination method, we show that the…

Quantum Gases · Physics 2015-06-11 Bruno Sciolla , Dario Poletti , Corinna Kollath

Active Brownian particles display self-propelled movement, which can be modelled as arising from a one-body force. Although their interparticle interactions are purely repulsive, for strong self propulsion the swimmers phase separate into…

Soft Condensed Matter · Physics 2021-03-25 Sophie Hermann , Daniel de las Heras , Matthias Schmidt

Theoretical approaches to nonequilibrium many-body dynamics generally rest upon an adiabatic assumption, whereby the true dynamics is represented as a sequence of equilibrium states. Going beyond this simple approximation is a notoriously…

Soft Condensed Matter · Physics 2014-10-15 Andrea Fortini , Daniel de las Heras , Joseph M. Brader , Matthias Schmidt

Based on Brownian Dynamics (BD) simulations, we study the dynamical self-assembly of active Brownian particles with dipole-dipole interactions, stemming from a permanent point dipole at the particle center. The propulsion direction of each…

Soft Condensed Matter · Physics 2021-06-09 Guo-Jun Liao , Carol K. Hall , Sabine H. L. Klapp

Transport properties of a hard-sphere colloidal fluid are investigated by Brownian dynamics simulations. We implement a novel algorithm for the time-dependent velocity-autocorrelation function (VACF) essentially eliminating the noise of the…

Soft Condensed Matter · Physics 2020-04-23 Suvendu Mandal , Lukas Schrack , Hartmut Löwen , Matthias Sperl , Thomas Franosch

We study the dynamics of colloidal suspensions of hard spheres that are subject to Brownian motion in the overdamped limit. We obtain the time evolution of the self and distinct parts of the van Hove function by means of dynamical density…

Soft Condensed Matter · Physics 2018-01-16 Daniel Stopper , Kevin Marolt , Hendrik Hansen-Goos , Roland Roth

We describe a test particle approach based on dynamical density functional theory (DDFT) for studying the correlated time evolution of the particles that constitute a fluid. Our theory provides a means of calculating the van Hove…

Soft Condensed Matter · Physics 2011-03-17 Paul Hopkins , Andrea Fortini , Andrew Archer , Matthias Schmidt

The Active Brownian Particle (ABP) model has become a prototype of self-propelled particles. ABPs move persistently at a constant speed $V$ along a direction that changes slowly by rotational diffusion, characterized by a coefficient $\Dr$.…

Soft Condensed Matter · Physics 2025-03-11 Rodrigo Soto

We study structural relaxation of colloidal hard spheres undergoing Brownian motion using dynamical density functional theory. Contrary to the partial linearization route [Stopper {\em et al.}, Phys. Rev. E {\bf 92}, 022151 (2015)] which…

Soft Condensed Matter · Physics 2018-01-16 Daniel Stopper , Roland Roth , Hendrik Hansen-Goos

The superadiabatic dynamical density functional theory (superadiabatic-DDFT) is a promising new method for the study of colloidal systems out-of-equilibrium. Within this approach the viscous forces arising from interparticle interactions…

Soft Condensed Matter · Physics 2024-06-10 S. M. Tschopp , J. M. Brader

Dynamic particle-scale numerical simulations are used to show that the shear thickening observed in dense colloidal, or Brownian, suspensions is of a similar nature to that observed in non-colloidal suspensions, i.e., a stress-induced…

Soft Condensed Matter · Physics 2015-12-04 Romain Mari , Ryohei Seto , Jeffrey F. Morris , Morton M. Denn

We investigate a model for colloidal network formation using Brownian Dynamics computer simulations. Hysteretic springs establish transient bonds between particles with repulsive core. If a bonded pair is separated by a cutoff distance, the…

Soft Condensed Matter · Physics 2016-04-20 Philip Krinninger , Andrea Fortini , Matthias Schmidt

We derive a dynamic Ornstein-Zernike equation for classical fluids undergoing overdamped Brownian motion and driven out of equilibrium. Inhomogeneous two-time correlation functions are obtained from functional differentiation of the…

Soft Condensed Matter · Physics 2013-10-31 Joseph M. Brader , Matthias Schmidt
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