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The phenomenon of spatial (polar) asymmetry of produced photoelectron emission due to strong-field multiphoton process of above-threshold ionization (ATI) in atoms irradiated by a linearly polarized two-color (bichromatic) laser field…

Atomic Physics · Physics 2017-06-19 P. E. Pyak , E. A. Andreeva , V. I. Usachenko

Photoelectron-photoion coincidence momentum imaging has been performed to investigate excitation processes on dissociative ionization of OCS, OCS $\to$ OCS$^+$ + e$^-$ $\to$ OC + S$^+$ + e$^-$, in phase-locked $\omega + 2\omega$ intense…

Atomic Physics · Physics 2026-02-18 Tomoyuki Endo , Tomohito Otobe , Ryuji Itakura

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

Atomic Physics · Physics 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

We use three dimensional time-dependent Schr\"odinger equation (3D--TDSE) to calculate angular electron momentum distributions and photoelectron spectra of atoms driven by spatially inhomogeneous fields. An example for such inhomogeneous…

Atomic Physics · Physics 2013-06-26 M. F. Ciappina , J. A. Pérez-Hernández , T. Shaaran , L. Roso , M. Lewenstein

Understanding the microscopic spatio-temporal dynamics of nonequilibrium charge carriers in heterosystems promises optimization of process and device design towards desired energy transfer. Hot electron transport is governed by scattering…

We present numerical simulations of ultrafast multiphoton ionization dynamics in a two-dimensional atomic model driven by co- and counterrotating circularly polarized single-color and bichromatic carrier envelope phase (CEP) stable…

Atomic Physics · Physics 2020-07-15 T. Bayer , Ch. Philipp , K. Eickhoff , M. Wollenhaupt

Photoelectron momentum distributions from strong-field ionization of carbonyl sulfide with 800 nm central-wavelength laser pulses at various peak intensities from $4.6$ to $13\times10^{13}$ W/cm$^2$ were recorded and analyzed regarding…

We present theoretical studies of above threshold ionization (ATI) produced by spatially inhomogeneous fields. This kind of field appears as a result of the illumination of plasmonic nanostructures and metal nanoparticles with a short laser…

Recent experimental techniques in multicolor waveform synthesis allow the temporal shaping of strong femtosecond laser pulses with applications in the control of quantum mechanical processes in atoms, molecules, and nanostructures.…

Atomic Physics · Physics 2017-10-11 Janne Solanpää , Marcelo F. Ciappina , Esa Räsänen

We present a time-dependent density-functional method able to describe the photoelectron spectrum of atoms and molecules when excited by laser pulses. This computationally feasible scheme is based on a geometrical partitioning that…

Atomic Physics · Physics 2012-06-28 U. De Giovannini , D. Varsano , M. A. L. Marques , H. Appel , E. K. U. Gross , A. Rubio

Coherent control of interfering one- and two-photon processes has for decades been the subject of research to achieve the redirection of photocurrent. The present study develops two-pathway coherent control of ground state helium atom…

Atomic Physics · Physics 2021-06-02 Yimeng Wang , Chris H. Greene

We investigate plasmon-assisted photoelectron emission using a one-dimensional time-dependent density-functional theory (TDDFT) model. Photoelectron spectra are computed with the time-dependent surface-flux (t-SURFF) method. In addition to…

Quantum Physics · Physics 2025-10-14 Mikhail Bednov , Waqas Pervez , Ingo Barke , Dieter Bauer

Phase-of-the-phase spectroscopy using two-color colinearly polarized laser pulses has been introduced and experimentally applied to strong-field tunneling ionization in S. Skruszewicz et al., Phys. Rev. Lett. 115, 043001 (2015) and recently…

Atomic Physics · Physics 2018-12-05 V. Tulsky , M. A. Almajid , D. Bauer

By measuring energy spectra of the electron emission from a sharp tungsten tip induced by few-cycle laser pulses, the laser-field dependence of the emission mechanism was investigated. In strong laser fields, we confirm the appearance of…

We present the results of a systematic study of photoelectron emission from gasphase dielectric nanoparticles (SiO2) irradiated by intense 25 fs, 780 nm linearly polarized laser pulses as a function of particle size (20 nm to 750 nm in…

Laser fields can be shaped on a subwavelength scale as to have a specific distribution in spin angular momentum, orbital structure, or topology. We study how these various features affect the strongly nonlinear electron dynamics.…

Quantum Physics · Physics 2020-12-30 Jonas Wätzel , Jamal Berakdar

We study nondipole effects in multiphoton ionization of a two-dimensional hydrogen-like atom by a flat-top laser pulse of varied intensity. For this purpose, we solve numerically a two-dimensional Schr\"odinger equation treating a…

Atomic Physics · Physics 2024-12-25 J. Z. Kamiński , K. Krajewska

Strong-field ionization of polar molecules contains rich dynamical processes such as tunneling, excitation, and Stark shift. These processes occur on a sub-cycle time scale and are difficult to distinguish in ultrafast measurements. Here,…

Atomic Physics · Physics 2021-12-15 Jia-Yin Che , Chao Chen , Shang Wang , Guo-Guo Xin , Yan-Jun Chen

The operation of photoemission electron sources with wavelengths near the photoemission threshold has been shown to dramatically decrease the minimum achievable photocathode emittance, but at the cost of significantly reduced quantum…

Accelerator Physics · Physics 2018-08-22 Jai Kwan Bae , Ivan Bazarov , Pietro Musumeci , Siddharth Karkare , Howard Padmore , Jared Maxson

We investigate the process of phase-controlled high-order above-threshold photoemission from sharp metallic nanotips under bichromatic laser fields. Experimental photoelectron spectra resulting from two-color excitation with a moderately…

Atomic Physics · Physics 2018-07-04 Lennart Seiffert , Timo Paschen , Peter Hommelhoff , Thomas Fennel