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We present an inelastic neutron scattering (INS) study of the excitation spectrum of a model S = 1/2 equilateral Heisenberg trimer, Cu_3(O_2C_16H_23)_6.1.2C_6H_12. Earlier measurements were interpreted on the basis of a spin ground state…

Strongly Correlated Electrons · Physics 2007-05-23 M. B. Stone , F. Fernandez-Alonso , D. T. Adroja , N. S. Dalal , D. Villagran , F. A. Cotton , S. E. Nagler

We theoretically examine the orbital excitations coupled to the spin degree of freedom in the parent state of the iron-arsenide superconductor, based on the calculation in a five-band itinerant model. The calculated Fe $L_3$-edge resonant…

Strongly Correlated Electrons · Physics 2011-08-04 E. Kaneshita , K. Tsutsui , T. Tohyama

Mechanism of unconventional superconductivity in FeSe has been intensely scrutinized recently because of a variety of exotic properties unprecedented for other iron-based superconductors. A central unanswered question concerns the origin of…

Recent STM experiments and theoretical considerations have highlighted the role of interaction-driven orbital selectivity in FeSe, and its role in generating the extremely anisotropic superconducting gap structure in this material. We study…

Superconductivity · Physics 2019-01-08 Andreas Kreisel , Brian M. Andersen , P. J. Hirschfeld

Using first-principles calculations, we demonstrate that the magnetic exchange interaction and the magnetocrystalline anisotropy of biatomic Fe chains grown in the trenches of the 5x1 reconstructed Ir(001) surface depend sensitively on the…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Yuriy Mokrousov , Alexander Thiess , Stefan Heinze

By substituting S into single-layer FeSe/SrTiO3, chemical pressure is applied to tune its paramagnetic state that is modeled as an incoherent superposition of spin-spiral states. The resulting electronic bands resemble an ordered…

Superconductivity · Physics 2023-10-10 Qiang Zou , Basu Dev Oli , Huimin Zhang , Tatsuya Shishidou , Daniel Agterberg , Michael Weinert , Lian Li

We use polarized inelastic neutron scattering to study low-energy spin excitations and their spatial anisotropy in electron-overdoped superconducting BaFe$_{1.85}$Ni$_{0.15}$As$_{2}$ ($T_c=14$ K). In the normal state, the imaginary part of…

Superconductivity · Physics 2012-06-26 Mengshu Liu , C. Lester , Jiri Kulda , Xingye Lu , Huiqian Luo , Meng Wang , Stephen M. Hayden , Pengcheng Dai

We investigate the re-entrant tetragonal phase in the iron-based superconductor Ba0 .76K0.24Fe2As2 by DC magnetization and thermoelectrical measurements. The reversible magnetization confirms by a thermodynamic method that the spin…

We present a detailed study of the ground-state magnetic structure of ultrathin Fe films on the surface of fcc Ir(001). We use the spin-cluster expansion technique in combination with the relativistic disordered local moment scheme to…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 A. Deák , L. Szunyogh , B. Ujfalussy

The fluctuations of the magnetic order parameter, or longitudinal spin excitations, are investigated theoretically in the ferromagnetic Fe and Ni as well as in the antiferromagnetic phase of the pnictide superconductor FeSe. The charge and…

Strongly Correlated Electrons · Physics 2020-07-01 Paweł Buczek , Nadine Buczek , Giovanni Vignale , Arthur Ernst

We study the crystalline and electronic properties of the $\textrm{Fe}_{1-x}\textrm{Co}_x\textrm{Se}$ system ($x=0$, 0.25, 0.5, 0.75, and 1.0) using X-ray diffraction, X-ray spectroscopy and density functional theory. We show that the…

Superconductivity · Physics 2014-07-22 I. Perez , J. A. McLeod , R. J. Green , R. Escamilla , V. Ortiz , A. Moewes

Magnetism in the orthorhombic metal CaFe$_4$As$_3$ was examined through neutron diffraction for powder and single crystalline samples. Incommensurate (${\bm q}_{\rm m}\approx (0.37-0.39)\times{\bm b}^{\ast}$) and predominantly…

We report a comprehensive study of the spin ladder compound BaFe$_2$S$_{2.5}$Se$_{0.5}$ using neutron diffraction, inelastic neutron scattering, high pressure synchrotron diffraction, and high pressure transport techniques. We find that…

Neutron scattering measurements were performed to investigate magnetic excitations in a single-crystal sample of the ternary iron arsenide BaFe2As2, a parent compound of a recently discovered family of Fe-based superconductors. In the…

Strongly Correlated Electrons · Physics 2009-02-28 K. Matan , R. Morinaga , K. Iida , T. J. Sato

We employ a five-orbital tight-binding model to develop the mean field solution for various possible spin density wave states in the iron-chalcogenides. The quasiparticle interference (QPI) technique is applied to detect signatures of these…

Superconductivity · Physics 2016-05-09 Bhaskar Kamble , Alireza Akbari , Ilya Eremin

Iron telluride (FeTe), a relative of the iron based high temperature superconductors, displays unusual magnetic order and structural transitions. Here we explore the idea that strong correlations may play an important role in these…

Materials Science · Physics 2013-05-29 Ari M. Turner , Fa Wang , Ashvin Vishwanath

Over the past few years Fe chalcogenides (FeSe/Te) have advanced to the forefront of Fe-based superconductors (FeBS) research. The most intriguing results thus far are for intercalated and monolayer FeSe, however experimental studies are…

Superconductivity · Physics 2015-11-10 J. K. Glasbrenner , I. I. Mazin , Harald O. Jeschke , P. J. Hirschfeld , Roser Valentí

A Raman scattering study covering the entire substitution range of the FeSe$_{1-x}$S$_x$ solid solution is presented. Data were taken as a function of sulfur concentration $x$ for $0\le x \le 1$, of temperature and of scattering symmetry.…

Normal state spin dynamics of the recently discovered iron-pnictide superconductors is discussed by calculating spin structure factor S(q, omega) in an itinerant five-band model within RPA approximation. Due to the characteristic Fermi…

Strongly Correlated Electrons · Physics 2009-04-15 Toshikaze Kariyado , Masao Ogata

Fe3-xGeTe2 is an itinerant ferromagnet composed of two-dimensional layers weakly connected by van der Waals bonding that shows a variety of intriguing phenomena. Inelastic neutron scattering measurements on bulk single crystals of…

Strongly Correlated Electrons · Physics 2019-03-27 S. Calder , A. I. Kolesnikov , A. F. May