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We describe a coherent mid-infrared continuum source with 700 cm-1 usable bandwidth, readily tuned within 600 - 2500 cm-1 (4 - 17 \mum) and thus covering much of the infrared "fingerprint" molecular vibration region. It is based on…

Quantum Physics · Physics 2015-06-04 Fritz Keilmann , Sergiu Amarie

Optical frequency combs have had a remarkable impact on precision spectroscopy. Enabling this technology in the x-ray domain is expected to result in wide-ranging applications, such as stringent tests of astrophysical models and quantum…

Frequency combs, specialized laser sources emitting multiple equidistant frequency lines, have revolutionized science and technology with unprecedented precision and versatility. Recently, integrated frequency combs are emerging as scalable…

Mid-infrared (mid-IR) spectroscopy provides a way to study structures and dynamics of complicated molecules in condensed phases. Therefore, developing compact and broadband mid-IR spectrometer has been a long-standing challenge. Here, we…

Optics · Physics 2020-01-16 Noh Soo Han , JunWoo Kim , Tai Hyun Yoon , Minhaeng Cho

A femtosecond frequency comb provides a vast number of equidistantly spaced narrow band laser modes that can be simultaneously tuned and frequency calibrated with 15 digits accuracy. Our Vernier spectrometer utilizes all of theses modes in…

Frequency combs are a spectrum of equally spaced frequency components with very high time-frequency accuracy, which have been widely used in the optical and microwave frequency ranges. We propose the realization of a frequency comb…

Mesoscale and Nanoscale Physics · Physics 2026-03-31 Xiyin Ye , Tao Yu

Electro-optic frequency combs with tooth spacings as low as 100 Hz were employed to probe electromagnetically induced transparency (EIT) and hyperfine pumping in rubidium and potassium vapor cells. From the potassium EIT transition we were…

Atomic Physics · Physics 2018-12-27 David A. Long , Adam J. Fleisher , Joseph T. Hodges

Coherent dual-comb spectroscopy (DCS) enables high-resolution measurements at high speeds without the trade-off between resolution and update rate inherent to mechanical delay scanning approaches. However, high system complexity and limited…

We have built a frequency chain which enables to measure the absolute frequency of a laser emitting in the 28-31 THz frequency range and stabilized onto a molecular absorption line. The set-up uses an optical frequency comb and an…

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

Optical frequency combs have revolutionized precision measurement, time-keeping, and molecular spectroscopy. A substantial effort has developed around "microcombs": integrating comb-generating technologies into compact, reliable photonic…

Mid-infrared frequency comb spectroscopy enables measurement of molecular at megahertz spectral resolution, sub-hertz frequency accuracy and microsecond acquisition speed. However, the widespread adoption of this technique has been hindered…

Precise measurements of the geometrical thickness of a sample and its refractive index are important for materials science, engineering, and medical diagnosis. Among the possible non-contact evaluation methods, optical interferometric…

We show how two frequency combs $\mathcal{E}_1$, $\mathcal{E}_2$ can be used to measure single-photon, two-photon absorption (TPA), and Raman resonances in a molecule with three electronic bands, by detecting the radio frequency modulation…

Chemical Physics · Physics 2014-08-12 Rachel Glenn , Shaul Mukamel

Dual-comb spectroscopy is a rapidly developing technique that enables moving parts-free, simultaneously broadband and high-resolution measurements with microseconds of acquisition time. However, for high sensitivity measurements and…

Instrumentation and Detectors · Physics 2019-08-14 Lukasz A. Sterczewski , Jonas Westberg , Gerard Wysocki

Tunable mid-infrared lasers are essential for optical sensing and imaging. Existing technologies, however, face challenges in simultaneously achieving broadband spectral tunability and ultra-rapid scan rates, limiting their utility in…

Optics · Physics 2025-01-20 Xiaoshuai Ma , Tianjian Lv , Xudong Zhu , Ming Yan , Heping Zeng

We report a precision realization of photonic thermometry using dual-comb spectroscopy to interrogate a $\pi$-phase-shifted fiber Bragg grating. We achieve read-out stability of 7.5 mK at 1 s and resolve temperature changes of similar…

A theoretical analysis is carried out for the recently developed three-pulse photon echo spectroscopy employing dual frequency combs (DFC) as the light sources. In this method, the molecular sample interacts with three pulse trains derived…

Chemical Physics · Physics 2020-01-08 Jonggu Jeon , JunWoo Kim , Tai Hyun Yoon , Minhaeng Cho

We demonstrate ultra-broadband optoelectronic mixing of frequency combs that provides phase-coherent detection of a repetition frequency up to 500 GHz, using a high-speed modified uni-traveling carrier (MUTC) photodiode. Nonlinear…

Optics · Physics 2024-10-30 Jizhao Zang , Jesse S. Morgan , Andreas Beling , Scott B. Papp

The advent of the laser frequency comb as the wavelength calibration unit allows us to measure the radial velocity at $cm\ s^{-1}$ precision level with high stability in long-term, which enable the possibility of the detection of…

Instrumentation and Methods for Astrophysics · Physics 2018-10-15 Zhao Fei , Zhao Gang , Liu Yujuan , Wang Liang , Wang Huijuan , Li Hongbin , Ye Huiqi , Hao Zhibo , Xiao Dong , Zhang Junbo , Kellermann Hanna , Grupp Frank