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Mott insulators with localized magnetic moments will exhibit a quantum spin liquid (QSL) state when the quantum fluctuations are strong enough to suppress the ordering of the spins. Such an entangled state will give rise to collective…

Strongly Correlated Electrons · Physics 2025-04-17 Haiyang Chen , Fo-Hong Wang , Qiang Gao , Xue-Jian Gao , Zhenhua Chen , Yaobo Huang , Kam Tuen Law , Xiao Yan Xu , Peng Chen

Understanding the interplay between charge, nematic, and structural ordering tendencies in cuprate superconductors is critical to unraveling their complex phase diagram. Using pump-probe time-resolved resonant x-ray scattering on the (0 0…

Molecular absorption and photo-electron spectra can be efficiently predicted with real-time time-dependent density-functional theory (TDDFT). We show here how these techniques can be easily extended to study time-resolved pump-probe…

Atomic and Molecular Clusters · Physics 2013-01-10 Umberto De Giovannini , Gustavo Brunetto , Alberto Castro , Jessica Walkenhorst , Angel Rubio

Within the framework of the density matrix method, general formulas obtained that are convenient for describing fast pulsed photoemission that occurs in a time less than or on the order of the times of relaxation processes inside the…

Mesoscale and Nanoscale Physics · Physics 2022-01-12 Yu. G. Peisakhovich , A. A. Shtygashev

Time-resolved electron dynamics in coupled quantum dots is directly observed by a pulsed-gate technique. While individual gate voltages are modulated with periodic pulse trains, average charge occupations are measured with a nearby quantum…

Mesoscale and Nanoscale Physics · Physics 2010-11-12 D. Harbusch , S. Manus , H. P. Tranitz , W. Wegscheider , S. Ludwig

Photoexcitation is a powerful means in distinguishing different interactions and manipulating the states of matter, especially in complex quantum systems. As a well-known charge density wave (CDW) material, 1T-TaS2 has been widely studied…

Strongly Correlated Electrons · Physics 2019-10-02 Jin Zhang , Chao Lian , Mengxue Guan , Wei Ma , Huixia Fu , Sheng Meng

Pump-probe experiments with femtosecond time resolution allow to disentangle the electronic dynamics from the lattice response and thus provide valuable insights into the non-equilibrium behavior of correlated materials. In Cr-doped…

Strongly Correlated Electrons · Physics 2024-07-15 Jiyu Chen , Francesco Petocchi , Viktor Christiansson , Philipp Werner

We study the doping of a Mott insulator in the presence of quenched frustrating disorder in the magnetic exchange. A low doping regime $\delta<J/t$ is found, in which the quasiparticle coherent scale is low : $\epsilon_F^* = J…

Strongly Correlated Electrons · Physics 2016-08-31 Olivier Parcollet , Antoine Georges

We investigate a photoinduced insulator-metal transition in the Falicov-Kimball model with the dynamical mean-field theory (DMFT) extended to nonequilibrium systems in periodic modulations in time. When the photon energy of the pump light…

Strongly Correlated Electrons · Physics 2015-05-13 Naoto Tsuji , Takashi Oka , Hideo Aoki

Time-dependent electron transport through a quantum dot and double quantum dot systems in the presence of polychromatic external periodic quantum dot energy-level modulations is studied within the time evolution operator method for a…

Mesoscale and Nanoscale Physics · Physics 2010-03-12 T. Kwapinski , S. Kohler , P. Hanggi

The use of ultrafast pump-probe conductivity (PPC) for studies of photoelectron dynamics in nonpolar molecular liquids has been based upon the perturbation of geminate recombination dynamics of trapped electrons by their laser…

Chemical Physics · Physics 2007-05-23 Ilya A. Shkrob , Leonid Ryzhik

Utilizing the time-dependent density-matrix renormalization group technique, we numerically prove photoinduced pairing states in the extended Falicov-Kimball model (EFKM) at half filling, both with and without internal SU(2) symmetry. In…

Strongly Correlated Electrons · Physics 2022-06-24 Satoshi Ejima , Florian Lange , Holger Fehske

Using the emission of the positively charged exciton as a probe, we analyze the dynamics of the optical pumping and the dynamics of the relaxation of a Mn spin exchange-coupled with a confined hole spin in a II-VI semiconductor quantum dot.…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 B. Varghese , H. Boukari , L. Besombes

Recent theoretical studies showed that the electronic structure of 1$T$-TaS$_2$ in the low-temperature commensurate charge density wave phase exhibits a nontrivial interplay between band-insulating and Mott insulating behavior. This has…

Strongly Correlated Electrons · Physics 2023-04-19 Francesco Petocchi , Jiyu Chen , Jiajun Li , Martin Eckstein , Philipp Werner

We report on the dynamics of optically induced nuclear spin polarization in individual CdTe/ZnTe quantum dots loaded with one electron by modulation doping. The fine structure of the hot trion (charged exciton $X^-$ with an electron in the…

Mesoscale and Nanoscale Physics · Physics 2012-06-18 C. Le Gall , A. Brunetti , H. Boukari , L. Besombes

The interaction between ultrashort light pulses and non-absorbing materials is dominated by Impulsive Stimulated Raman Scattering (ISRS). The description of ISRS in the context of pump\&probe experiments is based on effective classical…

Femtosecond optical pump-probe technique is used to study charge carrier dynamics in few-layer MoS2 samples fabricated by mechanical exfoliation. An ultrafast pump pulse excites carriers and differential reflection of a probe pulse tuned to…

Mesoscale and Nanoscale Physics · Physics 2011-11-01 Rui Wang , Brian A. Ruzicka , Nardeep Kumar , Matthew Z. Bellus , Hsin-Ying Chiu , Hui Zhao

We compute the time-resolved photoemission spectrum after photo-doping in a two-dimensional Mott-Hubbard insulator. We find that the relaxation rate of high-energy photo-doped electrons in the paramagnetic phase scales with the strength of…

Strongly Correlated Electrons · Physics 2016-02-26 Martin Eckstein , Philipp Werner

We provide provide a detailed study of biasless coherent transport of singlet electron pairs in one-dimensional (1D) channels induced by electron-electron interactions that are time-varying in certain spatially localized regions of the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Kunal K. Das

We study the dynamics of a quantum dot embedded in a three-dimensional microcavity in the strong coupling regime in which the quantum dot exciton has an energy close to the frequency of a confined cavity mode. Under the continuous pumping…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 J. I. Perea , D. Porras , C. Tejedor