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Numerical modelling of coherent spin relaxation in nanomagnets, formed by magnetic molecules of high spins, is accomplished. Such a coherent spin dynamics can be realized in the presence of a resonant electric circuit coupled to the magnet.…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 V. I. Yukalov , V. K. Henner , P. V. Kharebov

A scheme for decoupling and selectively recoupling large networks of dipolar-coupled spins is proposed. The scheme relies on a combination of broadband, decoupling pulse sequences applied to all the nuclear spins with a band-selective pulse…

Quantum Physics · Physics 2007-05-23 Fumiko Yamaguchi , Thaddeus D. Ladd , Cyrus P. Master , Yoshihisa Yamamoto , Navin Khaneja

The prospect of developing magnetic qubits is discussed. The first part of the article makes suggestions on how to achieve the coherent quantum superposition of spin states in small ferromagnetic clusters, weakly uncompensated…

Statistical Mechanics · Physics 2007-05-23 Eugene M. Chudnovsky

Based on a parametrization of pure quantum states we explicitly construct a sequence of (at most) $4N-5$ local time-continuous waveform controls to achieve a specified state transition for $N$-level quantum systems when sufficient controls…

Quantum Physics · Physics 2012-02-17 Ming Zhang , Jia-Hua Wei , Weiwei Zhou , Hong-Yi Dai , Zairong Xi , S. G. Schirmer

We demonstrate, numerically, the possibility of manipulating the spin states of molecular nanomagnets with shaped microwave pulses designed with quantum optimal control theory techniques. The state-to-state or full gate transformations can…

Quantum Physics · Physics 2021-12-01 Alberto Castro , Adrian Garcia Carrizo , David Zueco , Fernando Luis

Nuclear magnetic resonance (NMR) experiments can reveal local properties in materials, but are often limited by the low signal-to-noise ratio. Spin squeezed states have an improved resolution below the Heisenberg limit in one of the spin…

The dominant source of decoherence for an electron spin in a quantum dot is the hyperfine interaction with the surrounding bath of nuclear spins. The decoherence process may be slowed down by subjecting the electron spin to suitable…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Wenxian Zhang , V. V. Dobrovitski , Lea F. Santos , Lorenza Viola , B. N. Harmon

Nuclear magnetic resonance (NMR) spectroscopy provides unparalleled access to molecular structure and dynamics but is traditionally limited by weak signal strength, requiring large sample volumes and high magnetic fields. Here, we…

Applied Physics · Physics 2026-04-29 Dileep Singh , Riley W. Hooper , Christoph Findler , Utsab Banerjee , Dominik B. Bucher

Nuclear magnetic resonance (NMR) schemes can be applied to micron-, and nanometer-sized samples by the aid of quantum sensors such as nitrogen-vacancy (NV) color centers in diamond. These minute devices allow for magnetometry of nuclear…

Quantum Physics · Physics 2021-07-19 C. Munuera-Javaloy , R. Puebla , J. Casanova

Quantum sensors can show unprecedented sensitivities, provided they are controlled in a very specific, optimal way. Here, we consider a spin sensor of time-varying fields in the presence of dephasing noise, and we show that the problem of…

Quantum Physics · Physics 2024-07-10 S. Hernández-Gómez , F. Balducci , G. Fasiolo , P. Cappellaro , N. Fabbri , A. Scardicchio

Optimal control techniques provide a means to tailor the control pulses required to generate customized quantum gates, which helps to improve the resilience of quantum simulations to gate errors and device noise. However, the significant…

We study the interplay between rotating wave approximation and optimal control. In particular, we show that for a wide class of optimal control problems one can choose the control field such that the Hamiltonian becomes time-independent…

Quantum Physics · Physics 2016-03-21 Maximilian Keck , Matthias M. Müller , Tommaso Calarco , Simone Montangero

The Nitrogen-Vacancy (NV) defect in diamond is a unique quantum system that offers precision sensing of nanoscale physical quantities beyond the current state-of-the-art. Here we present a method to controllably encode the interactions in…

We study how to generate in minimum time special unitary transformations for a two-level quantum system under the assumptions that: (i) the system is subject to a constant drift, (ii) its dynamics can be affected by three independent,…

Quantum Physics · Physics 2015-11-18 Raffaele Romano

When probing nuclear spins in materials on the nanometer scale, random fluctuations of the spin polarization will exceed the mean Boltzmann polarization for sample volumes below about (100nm)^3. In this work, we use magnetic resonance force…

Mesoscale and Nanoscale Physics · Physics 2008-01-14 C. L. Degen , M. Poggio , H. J. Mamin , D. Rugar

Dynamical decoupling techniques are widely used to characterize and control the environments of solid-state quantum defects, enabling solid-state quantum memories and nanoscale quantum sensors. However, resolution is often limited by the…

The loss of coherence in quantum mechanical superposition states limits the time for which quantum information remains useful. Similarly, it limits the distance over which quantum information can be transmitted, resembling Anderson…

Quantum Physics · Physics 2010-06-11 Gonzalo A. Alvarez , Dieter Suter

The paper discusses various aspects of time-optimal control of quantum spin systems, modelled as right-invariant systems on a compact Lie group G. The main results are the reduction of such a system to an equivalent system on a homogeneous…

Quantum Physics · Physics 2007-05-23 Jan Swoboda

The loss of information about the relative phase between two quantum states, known as decoherence, strongly limits resolution in electron paramagnetic spectroscopy and hampers the use of molecules for quantum information processing. At low…

Quantum Physics · Physics 2025-04-28 Conor Ryan , Valerio Briganti , Cathal Hogan , Mark O'Neill , Alessandro Lunghi

Decoherence in Nature has become one of the most pressing problems in physics. Many applications, including quantum information processing, depend on understanding it; and fundamental theories going beyond quantum mechanics have been…

Mesoscale and Nanoscale Physics · Physics 2011-07-27 S. Takahashi , I. S. Tupitsyn , J. van Tol , C. C. Beedle , D. N. Hendrickson , P. C. E. Stamp
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