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We study the ability to implement unitary maps on states of the $I=9/2$ nuclear spin in \textsuperscript{87}Sr, a $d=10$ dimensional (qudecimal) Hilbert space, using quantum optimal control. Through a combination of nuclear spin-resonance…

Quantum Physics · Physics 2022-11-30 Sivaprasad Omanakuttan , Anupam Mitra , Michael J. Martin , Ivan H Deutsch

Nuclear spins are highly coherent quantum objects. In large ensembles, their control and detection via magnetic resonance is widely exploited, e.g. in chemistry, medicine, materials science and mining. Nuclear spins also featured in early…

Zero-field nuclear magnetic resonance (NMR) provides complementary analysis modalities to those of high-field NMR and allows for ultra-high-resolution spectroscopy and measurement of untruncated spin-spin interactions. Unlike for the…

Quantum Physics · Physics 2022-03-01 Min Jiang , Teng Wu , John W. Blanchard , Guanru Feng , Xinhua Peng , Dmitry Budker

We develop energy efficient, continuous microwave schemes to couple electron and nuclear spins, using phase or amplitude modulation to bridge their frequency difference. These controls have promising applications in biological systems,…

Quantum Physics · Physics 2019-01-14 J. Casanova , E. Torrontegui , M. B. Plenio , J. J. García-Ripoll , E. Solano

For the implementation of a quantum computer it is necessary to exercise complete control over the Hamiltonian of the used physical system. For NMR quantum computing the effectively acting Hamiltonian can be manipulated via pulse sequences.…

Quantum Physics · Physics 2009-11-07 Marcus Stollsteimer , Guenter Mahler

Nuclear magnetic resonance (NMR) is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities -…

The nuclear spin is a prime candidate for quantum information applications due to its weak coupling to the environment and inherently long coherence times. However, this weak coupling also challenges the addressability of the nuclear spin.…

Quantum Physics · Physics 2025-12-15 Hester G. Vennema , Cristina Mier , Evert W. Stolte , Leonard Edens , Jinwon Lee , Sander Otte

Quantum sensors have recently achieved to detect the magnetic moment of few or single nuclear spins and measure their magnetic resonance (NMR) signal. However, the spectral resolution, a key feature of NMR, has been limited by relaxation of…

Decoherence-protected spins associated with nitrogen-vacancy color centers in diamond possess remarkable long coherence time, which make them one of the most promising and robust quantum registers. The current demand is to explore practical…

Quantum Physics · Physics 2024-02-27 Jiazhao Tian , Haibin Liu , Roberto Sailer , Liantuan Xiao , Fedor Jelezko , Ressa S. Said

Optimizing the controls of quantum systems plays a crucial role in advancing quantum technologies. The time-varying noises in quantum systems and the widespread use of inhomogeneous quantum ensembles raise the need for high-quality quantum…

Quantum Physics · Physics 2025-05-06 Xinyu Fei , Lucas T. Brady , Jeffrey Larson , Sven Leyffer , Siqian Shen

We propose a quantum algorithm for inferring the molecular nuclear spin Hamiltonian from time-resolved measurements of spin-spin correlators, which can be obtained via nuclear magnetic resonance (NMR). We focus on learning the anisotropic…

We study the decay of multiple quantum (MQ) NMR coherences in systems with the large number of equivalent spins. As being created on the preparation period of MQ NMR experiment, they decay due to the dipole-dipole interactions (DDI) on the…

Quantum Physics · Physics 2011-01-25 S. I. Doronin , E. B. Fel'dman , A. I. Zenchuk

We present a new formulation of monotonically convergent algorithms which allows to optimize both the control duration and the field fluence. A standard algorithm designs a control field of fixed duration which both brings the system close…

Quantum Physics · Physics 2012-03-13 M. Lapert , J. Salomon , D. Sugny

We propose a method for enacting the unitary time propagation of two interacting neutrons at leading order of chiral effective field theory by efficiently encoding the nuclear dynamics into a single multi-level quantum device. The emulated…

Mechanical resonators operating in the megahertz range have become a versatile platform for fundamental and applied quantum research. Their exceptional properties, such as low mass and high quality factor, make them also appealing for force…

Mesoscale and Nanoscale Physics · Physics 2026-04-20 Diego A. Visani , Letizia Catalini , Christian L. Degen , Alexander Eichler , Javier del Pino

The article considers a two-level open quantum system whose dynamics is driven by a combination of coherent and incoherent controls. Coherent control enters into the Hamiltonian part of the dynamics whereas incoherent control enters into…

Quantum Physics · Physics 2019-09-24 Oleg V. Morzhin , Alexander N. Pechen

Characterizing noisy quantum devices requires methods for learning the underlying quantum Hamiltonian which governs their dynamics. Often, such methods compare measurements to simulations of candidate Hamiltonians, a task which requires…

Quantum Physics · Physics 2021-10-13 Assaf Zubida , Elad Yitzhaki , Netanel H. Lindner , Eyal Bairey

Quantum optimal control is a technique for controlling the evolution of a quantum system and has been applied to a wide range of problems in quantum physics. We study a binary quantum control optimization problem, where control decisions…

Quantum Physics · Physics 2024-10-15 Xinyu Fei , Lucas T. Brady , Jeffrey Larson , Sven Leyffer , Siqian Shen

Fifty years of developments in nuclear magnetic resonance (NMR) have resulted in an unrivaled degree of control of the dynamics of coupled two-level quantum systems. This coherent control of nuclear spin dynamics has recently been taken to…

Quantum Physics · Physics 2015-06-26 Lieven M. K. Vandersypen , Isaac L. Chuang

A new class of cost functionals for optimal control of quantum systems which produces controls which are sparse in frequency and smooth in time is proposed. This is achieved by penalizing a suitable time-frequency representation of the…

Optimization and Control · Mathematics 2016-07-15 Gero Friesecke , Felix Henneke , Karl Kunisch