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The phonon-induced dephasing dynamics in optically excited semiconductor quantum dots is studied within the frameworks of the independent Boson model and optimal control. We show that appropriate tailoring of laser pulses allows a complete…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Ulrich Hohenester , Georg Stadler

In this work, we extend the quantum optimal control theory of molecules subject to ultrashort laser pulses to the case of solvated systems, explicitly including the solvent dielectric properties in the system Hamiltonian. A reliable…

Chemical Physics · Physics 2019-12-23 Marta Rosa , Gabriel Gil , Stefano Corni , Roberto Cammi

A quantum memory is a system that enables transfer, storage, and retrieval of optical quantum states by ON/OFF switching of the control signal in each stages of the memory. In particular, it is known that, for perfect transfer of a…

Quantum Physics · Physics 2017-02-21 Hideaki Nakao , Naoki Yamamoto

Most quantum processors requires pulse sequences for controlling quantum states. Here, we present an alternative algorithm for computing an optimal pulse sequence in order to perform a specific task, being an implementation of a quantum…

Quantum Physics · Physics 2020-05-27 John P. S. Peterson , Roberto S. Sarthour , Raymond Laflamme

Optimally-shaped electromagnetic fields have the capacity to coherently control the dynamics of quantum systems and thus offer a promising means for controlling molecular transformations relevant to chemical, biological, and materials…

Quantum Physics · Physics 2021-06-08 Alicia B. Magann , Matthew D. Grace , Herschel A. Rabitz , Mohan Sarovar

Coherent control over photoelectron wavepackets, via the use of polarization-shaped laser pulses, can be understood as a time and polarization-multiplexed process. In this work, we investigate this multiplexing via computation of the…

Atomic Physics · Physics 2016-05-30 Paul Hockett , Matthias Wollenhaupt , Thomas Baumert

Controlling the wave function of free electrons is important to improve the spatial resolution of electron microscopes, the efficiency of electron interaction with sample modes of interest, and our ability to probe ultrafast materials…

Quantum Physics · Physics 2021-01-27 Valerio Di Giulio , F. Javier García de Abajo

Control of quantum systems is a central element of high-precision experiments and the development of quantum technological applications. Control pulses that are typically temporally or spatially modulated are often designed based on…

Quantum Physics · Physics 2021-01-04 Frederic Sauvage , Florian Mintert

We derive a generalized master equation for multiphoton pulses interacting with multiple emitters in a waveguide-quantum electrodynamics system where the emitter frequency can be modulated and the effects of non-guided modes can also be…

Quantum Physics · Physics 2020-11-06 Zeyang Liao , Yunning Lu , M. Suhail Zubairy

Photon emission and absorption by an individual qubit are essential elements for the quantum manipulation of light. Here we demonstrate the controllability of spontaneous emission of a qubit in various electromagnetic environments. The…

Quantum Physics · Physics 2019-07-10 Wai-Keong Mok , Jia-Bin You , Wenzu Zhang , Wan-Li Yang , Ching Eng Png

We investigate optimal control strategies for state to state transitions in a model of a quantum dot molecule containing two active strongly interacting electrons. The Schrodinger equation is solved nonperturbatively in conjunction with…

Quantum Physics · Physics 2016-08-14 R. Nepstad , L. Sælen , I. Degani , J. P. Hansen

A wide range of ultrafast phenomena in various atomic, molecular and condense matter systems is governed by electron dynamics. Therefore, the ability to image electronic motion in real space and real time would provide a deeper…

Atomic Physics · Physics 2018-02-27 Daria Popova-Gorelova

In this work, we study strategies for the optical control, within the dipole approximation, of a qubit encoded in the three-electron states of a triple quantum dot. The system is described by effective confining potentials, and its…

Mesoscale and Nanoscale Physics · Physics 2019-01-30 Diego S. Acosta Coden , Sergio S. Gomez , Rodolfo H. Romero , Omar Osenda , Alejandro Ferrón

In this report we review the present state of the art of the control of propagating quantum states at the single-electron level and its potential application to quantum information processing. We give an overview of the different approaches…

We study ultrafast ionization dynamics using orthogonally polarized two-color (OTC) laser pulses involving the resonant "first plus second" ($\omega+2\omega$) scheme. The scheme is illustrated by numerical simulations of the time-dependent…

Atomic Physics · Physics 2019-12-16 Hicham Agueny

Quantum controls realize the unitary or nonunitary operations employed in quantum computers, quantum simulators, quantum communications, and other quantum information devices. They implement the desired quantum dynamics with the help of…

Quantum Physics · Physics 2022-06-02 T S Mahesh , Priya Batra , M. Harshanth Ram

Semiconductor quantum dots embedded in optical cavities are promising on-demand sources of single photons. Here, we theoretically study single photon emission from an optically driven two-photon Raman transition between the biexciton and…

Using a quantum wave packet simulation including the nuclear and electronic degrees of freedom, we investigate the femtosecond and picosecond energy- and angle-resolved photoelectron spectra of the E($^1\Sigma_g^+$) electronic state of…

Chemical Physics · Physics 2019-04-04 R. Chamakhi , R. Puthumpally-Joseph , M. Telmini , E. Charron

The ability to characterise a Hamiltonian with high precision is crucial for the implementation of quantum technologies. In addition to the well-developed approaches utilising optimal probe states and optimal measurements, the method of…

Quantum Physics · Physics 2022-12-14 Shushen Qin , Marcus Cramer , Christiane P. Koch , Alessio Serafini

The energy and the angular distributions of photoelectrons are shown to be tunable by choosing the time and the spatial phase structure of the driving fields. These conclusions are derived from quantum mechanical calculations done within a…

Atomic Physics · Physics 2023-03-15 Jonas Wätzel , Johannes Hahn , Jamal Berakdar