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Quantum fluctuations are expected to lead to highly entangled spin-liquid states in certain two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon spin relaxation rates in the copper-based…

Unlike conventional magnets where the magnetic moments are partially or completely static in the ground state, in a quantum spin liquid they remain in collective motion down to the lowest temperatures. The importance of this state is that…

Muon spin relaxation and rotation ($\mu$SR) experiments on single crystals of the structurally perfect triangular antiferromagnet YbMgGaO$_4$ indicate the absence of both static long-range magnetic order and spin freezing down to 0.048 K in…

Continuum of spin excitations observed in inelastic neutron scattering experiments are often considered as a strong evidence of quantum spin liquid formation. When quantum spin liquid is indeed the ground state of a disorder-free magnetic…

Strongly Correlated Electrons · Physics 2025-04-15 Jieming Sheng , Le Wang , Wenrui Jiang , Han Ge , Nan Zhao , Tiantian Li , Maiko Kofu , Dehong Yu , Wei Zhu , Jia-Wei Mei , Zhentao Wang , Liusuo Wu

A recent focus of quantum spin liquid (QSL) studies is how disorder/randomness in a QSL candidate affects its true magnetic ground state. The ultimate question is whether the QSL survives disorder or the disorder leads to a…

Strongly Correlated Electrons · Physics 2021-08-17 X. Rao , G. Hussain , Q. Huang , W. J. Chu , N. Li , X. Zhao , Z. Dun , E. S. Choi , T. Asaba , L. Chen , L. Li , X. Y. Yue , N. N. Wang , J. -G. Cheng , Y. H. Gao , Y. Shen , J. Zhao , G. Chen , H. D. Zhou , X. F. Sun

The simplest spin-orbital model can host a nematic spin-orbital liquid state on the triangular lattice. We provide clear evidence that the ground state of the SU(4) Kugel-Khomskii model on the triangular lattice can be well described by a…

Strongly Correlated Electrons · Physics 2022-03-31 Hui-Ke Jin , Rong-Yang Sun , Hong-Hao Tu , Yi Zhou

Magnetic, thermodynamic, neutron diffraction and inelastic neutron scattering are used to study spin correlations in the easy-axis XXZ triangular lattice magnet K2Co(SeO3)2. Despite the presence of quasi-2D "supersolid" magnetic order, the…

Strongly Correlated Electrons · Physics 2024-11-04 M. Zhu , V. Romerio , N. Steiger , S. D. Nabi , N. Murai , S. Ohira-Kawamura , K. Yu. Povarov , Y. Skourski , R. Sibille , L. Keller , Z. Yan , S. Gvasaliya , A. Zheludev

The quantum pyrochlore antiferromagnet is studied by perturbative expansions and exact diagonalization of small clusters. We find that the ground state is a spin-liquid state: The spin-spin correlation functions decay exponentially with…

Strongly Correlated Electrons · Physics 2009-10-31 Benjamin Canals , Claudine Lacroix

A quantum spin liquid (QSL) is a state of matter in which magnetic spins interact strongly, but quantum fluctuations inhibit long-range magnetic order even at zero temperature. A QSL has been predicted to have a host of exotic properties,…

Quantum spin liquids (QSLs) represent a novel state of matter in which quantum fluctuations prevent conventional magnetic order from being established, and the spins remain disordered even at zero temperature. There have been many…

Strongly Correlated Electrons · Physics 2018-10-11 Zhen Ma , Kejing Ran , Jinghui Wang , Song Bao , Zhengwei Cai , Shichao Li , Jinsheng Wen

A spin-1/2 triangular-lattice antiferromagnet is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between geometric spin frustration and quantum fluctuations. It can…

The cradle of quantum spin liquids, triangular antiferromagnets show strong proclivity to magnetic order and require deliberate tuning to stabilize a spin-liquid state. In this brief review, we juxtapose recent theoretical developments that…

Strongly Correlated Electrons · Physics 2020-03-13 Yuesheng Li , Philipp Gegenwart , Alexander A. Tsirlin

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

We report proximate quantum spin liquid behavior in K$_2$Co$_2$(SO$_4$)$_3$ with the magnetic Co$^{2+}$ ions embedded on a highly frustrated three-dimensional double trillium lattice. Single-crystal and high-resolution synchrotron powder…

We study quantum disordered ground states of the two dimensional Heisenberg-Kitaev model on the triangular lattice using a Schwinger boson approach. Our aim is to identify and characterize potential gapped quantum spin liquid phases that…

Strongly Correlated Electrons · Physics 2017-01-25 Pavel Kos , Matthias Punk

Motivated by the recent synthesis of $\beta$-Li$_2$IrO$_3$ -- a spin-orbit entangled $j=1/2$ Mott insulator with a three-dimensional lattice structure of the Ir$^{4+}$ ions -- we consider generalizations of the Kitaev model believed to…

Strongly Correlated Electrons · Physics 2014-06-03 M. Hermanns , S. Trebst

A spin liquid is a novel quantum state of matter with no conventional order parameter where a finite charge gap exists even though the band theory would predict metallic behavior. Finding a stable spin liquid in two or higher spatial…

Strongly Correlated Electrons · Physics 2012-12-20 Sandro Sorella , Yuichi Otsuka , Seiji Yunoki

We report results of magnetic susceptibility, specific heat, and muon spin relaxation ($\mu$SR) measurements on the polycrystalline Ba$_6$Nd$_2$Ti$_4$O$_{17}$, a disorder-free triangular-lattice antiferromagnet. The absence of long-range…

Strongly Correlated Electrons · Physics 2024-11-21 C. Y. Jiang , B. L. Chen , K. W. Chen , J. C. Jiao , Y. Wang , Q. Wu , N. Y. Zhang , M. Y. Zou , P. -C. Ho , O. O. Bernal , L. Shu

A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

Strongly Correlated Electrons · Physics 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin

We study in this paper quantum spin liquid states (QSLs) at the vicinity of metal-insulator transition. Assuming that the low energy excitations in the QSLs are labeled by "spinon" occupation numbers with the same Fermi surface structure as…

Strongly Correlated Electrons · Physics 2013-10-23 Yi Zhou , Tai-Kai Ng