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High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

Using one-dimensional simulations analyzed through the lens of open quantum systems, we study the photoelectron's strong-field dynamics from an atom surrounded by a scattering environment stochastically structured. We theoretically…

Quantum Physics · Physics 2026-05-21 Simon His , Camille Lévêque , Jérémie Caillat , Richard Taïeb , Jonathan Dubois

The first scheme for quasi-phase-matching high harmonic generation of circularly polarized radiation is proposed: optical rotation quasi-phase-matching (ORQPM). In ORQPM propagation of the driving radiation in a system exhibiting circular…

Optics · Physics 2013-03-19 Lewis Z. Liu , Kevin O'Keeffe , Simon M. Hooker

Present photoionization experiments cannot measure molecular frame photoelectron angular distributions (MFPAD) from the outermost valence electrons of molecules. We show that details of the MFPAD can be retrieved with high-order harmonics…

Atomic Physics · Physics 2009-05-24 Anh-Thu Le , R. R. Lucchese , M. T. Lee , C. D. Lin

High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…

In present paper we develop an analytic theory for the harmonic generation of symmetric diatomic molecular ions beyond two-level model, emphasizing the influence of charge-resonance (CR) states those are strongly coupled to electromagnetic…

Atomic Physics · Physics 2009-11-13 Yanjun Chen , Jing Chen , Jie Liu

We study the Cooper minimum in high harmonic generation from argon atoms using long wavelength laser pulses. We find that the minimum in high harmonic spectra is systematically shifted with respect to total photoionization cross section…

We report on high-order harmonic generation in the two-band superconductor MgB$_2$ driven by intense terahertz electromagnetic pulses. Third- and fifth-order harmonics are resolved in time domain and investigated as a function of…

The interaction of matter with a quantized electromagnetic mode is considered. Representing a strong exciting field, the mode is assumed to contain a large number of photons. As a result, the material response is highly nonlinear: the…

Quantum Physics · Physics 2020-01-17 Ákos Gombkötő , Sándor Varró , Péter Mati , Péter Földi

In strong field laser physics it is a common practice to use the high-order harmonic cutoff to estimate the laser intensity of the pulse that generates the harmonic radiation. Based on the semiclassical arguments it is possible to find a…

Atomic Physics · Physics 2015-06-11 T. Shaaran , M. F. Ciappina , M. Lewenstein

We study the process of resonant generation of high-order harmonics in a closed cavity in the model of vacuum nonlinear electrodynamics. Concretely, we study the possibility of resonant generation of the third harmonic induced by a single…

Quantum Physics · Physics 2023-07-12 Ilia Kopchinskii , Petr Satunin

We investigated the high-order harmonic generation (HHG) process of diatomic molecular ion $\mathrm{H}_2^+$ in non-Born-Oppenheimer approximations. The corresponding three-dimensional time-dependent Schr\"odinger equation is solved with…

Atomic Physics · Physics 2017-02-28 Mu-Zi Li , Guang-Rui Jia , Xue-Bin Bian

We derive a simple theory for high-order harmonic generation due to pumping a noninteracting metal with a large amplitude oscillating electric field. The model assumes that the radiated light field arises from the acceleration of electrons…

Optics · Physics 2015-01-12 J. K. Freericks , A. Y. Liu , A. F. Kemper , T. P. Devereaux

We study the ellipticity of high-order harmonics emitted from CO$_2$ molecule driven by linearly polarized laser fields using numerical simulations within the time-dependent density functional theory. We find that the overall ellipticity of…

Atomic and Molecular Clusters · Physics 2024-09-17 Andres Mora , Lauren Bauerle , Yuqing Xia , Agnieszka Jaron

A method is proposed for arbitrarily engineering the high-order harmonic generation phase achieved by shaping a laser pulse and employing xuv light or x rays for ionization. This renders the production of bandwidth-limited attosecond pulses…

Atomic Physics · Physics 2011-02-25 Markus C. Kohler , Christoph H. Keitel , Karen Z. Hatsagortsyan

We study high-order harmonic generation by optically driven one- and two-dimensional hydrogenlike atoms formed by Coulomb imurities in graphene. The time-dependent Dirac equations with Coulomb plus time-periodic monochromatic field…

Mesoscale and Nanoscale Physics · Physics 2025-04-07 S. Rakhmanov , K. Matchonov , H. Yusupov , K. Nasriddinov , D. Matrasulov

Symmetries essentially provide conservation rules in nonlinear light-matter interactions, that facilitate control and understanding of photon conversion processes or electron dynamics. Since anisotropic solids have rich symmetries, they are…

We study the high harmonic generation with vortex beams beyond the dipole approximation. To do so we employ the full minimal coupling approach to account for multipolar coupling without truncation and describe the full spatio-temporal…

Atomic Physics · Physics 2026-01-21 Esra Ilke Albar , Valeriia P. Kosheleva , Heiko Appel , Angel Rubio , Franco P. Bonafé

High-harmonic generation by a highly non-linear interaction of infrared laser fields with matter allows for the generation of attosecond pulses in the XUV spectral regime. This process, well established for atoms, has been recently extended…

High harmonic generation (HHG) is a highly nonlinear emission process in which systems driven by intense laser pulses emit integer multiples (harmonics) of the driving field. This feature is considered universal to all occurrences of HHG.…