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A method is implemented to perform "fast" adiabatic variation of the spin Hamiltonian by imposing the constant adiabaticity condition. The method is applied to improve the performance of singlet-state Nuclear Magnetic Resonance (NMR)…

Coupled pairs of spin-1/2 nuclei support one singlet state and three triplet states. In many circumstances the nuclear singlet order, defined as the difference between the singlet population and the mean of the triplet populations, is a…

Quantum Physics · Physics 2022-10-19 Mohamed Sabba , Nino Wili , Christian Bengs , Lynda J. Brown , Malcolm H. Levitt

SABRE (Signal Amplification By Reversible Exchange) is a technique for enhancement of NMR (Nuclear Magnetic Resonance) signals, which utilizes parahydrogen (pH2, the H2 molecule in its nuclear spin state) as a source of non-thermal spin…

Dynamical polarization of nuclear spin ensembles is of central importance for magnetic resonance studies, precision sensing and for applications in quantum information theory. Here we propose a scheme to generate long-lived singlet pairs in…

Quantum Physics · Physics 2017-04-06 Johannes N. Greiner , D. D. Bhaktavatsala Rao , Jörg Wrachtrup

We provide a route to generate nematic order in a spin-1/2 system. Unlike the well-known magnon-binding mechanism, our spin nematics requires neigher the frustration effect nor a spin polarization in a high field or in the vicinity of a…

Strongly Correlated Electrons · Physics 2018-05-22 Yuto Yokoyama , Chisa Hotta

The interplay between unconventional superconductivity and altermagnetic order has attracted much attentions. In particular, whether spin-triplet superconductivity can be achieved by suppressing altermagnetism remains an open issue. We…

Superconductivity · Physics 2025-09-15 Xin Ma , Siqi Wu , Zilong Li , Lunhui Hu , Jianhui Dai , Chao Cao

Recently, Pang et al reported a novel polarization transfer scheme applicable to three-spin systems, whereby a rotating-frame NMR analogue of the cross effect could transfer polarization between; e.g., two 13Cs and an 15N in a single…

Quantum Physics · Physics 2026-04-21 Sundaresan Jayanthi , Adonis Lupulescu , Julia Grinshtein , Lucio Frydman

Quantum many-body phases offer unique properties and emergent phenomena, making them an active area of research. A promising approach for their experimental realization in model systems is to adiabatically follow the ground state of a…

Intramolecular spin alignment in pi-conjugated molecules is studied theoretically in a model of a Peierls-Hubbard chain coupled with two localized spins. By means of the exact diagonalization technique, we demonstrate that a spin singlet…

Materials Science · Physics 2009-11-10 Ping Huai , Yukihiro Shimoi , Shuji Abe

We present comprehensive high magnetic field studies of the alternating weakly coupled ferro-antiferromagnetic (FM-AFM) spin-$1/2$ chain compound Cu$_2$(OH)$_3$Br, with the structure of the natural mineral botallackite. Our measurements…

Strongly Correlated Electrons · Physics 2024-12-17 K. Yu. Povarov , Y. Skourskii , J. Wosnitza , D. E. Graf , Z. Zhao , S. A. Zvyagin

We report a successful measurement of the magnetic field-induced spin singlet-triplet transition in silicon-based coupled dot systems. Our specific experimental scheme incorporates a lateral gate-controlled Coulomb-blockaded structure in Si…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 S. D. Lee , S. J. Kim , J. S. Kang , Y. B. Cho , J. B. Choi , Sooa Park , S. -R. Eric Yang , S. J. Lee , T. H. Zyung

The nuclear spin singlet order involving coupled pairs of spins-1/2 may be used to store nuclear spin hyperpolarization in a room temperature liquid for a time much longer than the spin-lattice relaxation time $T_1$. There both are…

Quantum Physics · Physics 2021-06-02 Y. Yang , L. Zhou , Q. Chen

In quantum information science and sensing, electron spins are often purified into a specific polarisation through an optical-spin interface, a process known as optically-detected magnetic resonance (ODMR). Diamond-NV centres and transition…

Chemical Physics · Physics 2024-11-22 Yong Rui Poh , Joel Yuen-Zhou

Whereas there exists considerable evidence for the conversion of singlet Cooper pairs into triplet Cooper pairs in the presence of inhomogeneous magnetic fields, recent theoretical proposals have suggested an alternative way to exert…

Superconductivity · Physics 2018-06-06 N. Banerjee , J. A. Ouassou , Y. Zhu , N. A. Stelmashenko , J. Linder , M. G. Blamire

Electric-field switching of magnetic order is of significant physical interest and holds great potential for spintronic applications. However, it has rarely been reported in two-dimensional (2D) van der Waals (vdW) magnets due to the…

Materials Science · Physics 2025-02-06 Chengxi Huang , Jinzhe Han , Jing Wang , Jintao Jiang , Ziyang Qu , Fang Wu , Ang Li , Yi Wan , Kaiyou Wang , Erjun Kan

The influence of bond randomness on long range magnetic ordering in the weakly coupled S = 1/2 antiferromagnetic spin chain materials Cu(py)2(Cl1-xBrx)2 is studied by muon spin rotation and bulk measurements. Disorder is found to have a…

Strongly Correlated Electrons · Physics 2012-12-04 M. Thede , F. Xiao , Ch. Baines , C. Landee , E. Morenzoni , A. Zheludev

Coupled pairs of nuclear spins-1/2 support one singlet state and three triplet states. Transitions between the singlet state and one of the triplet states may be driven by an oscillating low-frequency magnetic field, in the presence of…

Quantum Physics · Physics 2021-10-27 Laurynas Dagys , Christian Bengs , Malcolm H. Levitt

A theoretical approach is proposed for quantitative modeling of SABRE (Signal Amplification By Reversible Exchange) experiments performed at a high magnetic field of an NMR spectrometer. SABRE is a method, which exploits the spin order of…

Chemical Physics · Physics 2019-05-01 Stephan Knecht , Konstantin L. Ivanov

A natural orbital functional for electronic systems with any value of the spin is proposed. This energy functional is based on a new reconstruction for the two-particle reduced density matrix (2RDM) of the multiplet, that is, of the mixed…

Chemical Physics · Physics 2019-10-02 Mario Piris

The pairing state and critical temperature (T$_c$) of a thin s-wave superconductor (S) on two or more ferromagnets (F) are controllable through the magnetization-alignment of the F layers. Magnetization misalignment can lead to…

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