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The radiative recombination of a free electron into an excited state of a bare, high-Z ion is studied, together with its subsequent decay, within the framework of the density matrix theory and Dirac's relativistic equation. Special…

Atomic Physics · Physics 2010-11-29 A. V. Maiorova , A. Surzhykov , S. Tashenov , V. M. Shabaev , S. Fritzsche , G. Plunien , Th. Stoehlker

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

With a semiclassical quasi-static model we achieve an insight into the complex dynamics of two correlated electrons under the combined influence of a two-center Coulomb potential and an intense laser field. The model calculation is able to…

Atomic and Molecular Clusters · Physics 2009-11-13 J. Liu , D. F. Ye , J. Chen , X. liu

We report on the unambiguous observation of the sub-cycle ionization bursts in sequential strong-field double ionization of H$_2$ and their disentanglement in molecular frame photoelectron angular distributions. This observation was made…

We address nonsequential double ionization induced by strong, linearly polarized laser fields of only a few cycles, considering a physical mechanism in which the second electron is dislodged by the inelastic collision of the first electron…

Atomic Physics · Physics 2009-11-10 C. Figueira de Morisson Faria , X. Liu , A. Sanpera , M. Lewenstein

It was recently shown that the exact potential driving the electron's dynamics in enhanced ionization of H$_2^+$ can have large contributions arising from dynamical electron-nuclear correlation, going beyond what any electrostatics-based…

Atomic and Molecular Clusters · Physics 2017-06-07 E. Khosravi , A. Abedi , A. Rubio , N. T. Maitra

Microscopically understanding competing orders in strongly correlated systems is a key challenge in modern quantum many-body physics. For example, the study of magnetic polarons and their relation to pairing in the Fermi-Hubbard model in…

Strongly Correlated Electrons · Physics 2024-10-02 Henning Schlömer , Ulrich Schollwöck , Annabelle Bohrdt , Fabian Grusdt

Quantum phase transition at the saturation field is studied for a class of frustrated quantum antiferromagnets. The considered models include (i) the $J_1$-$J_2$ frustrated square-lattice antiferromagnet with $J_2={1/2}J_1$ and (ii) the…

Strongly Correlated Electrons · Physics 2007-05-23 G. Jackeli , M. E. Zhitomirsky

An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…

Atomic Physics · Physics 2020-06-26 Bar Ezra , Shimshon Kallush , Ronnie Kosloff

We consider the final stage of double ionization of $\rm O_2$ molecules by short linearly polarized laser pulses. The saddles of the effective adiabatic potential energy close to which simultaneous escape of electrons from a molecule takes…

Atomic Physics · Physics 2007-05-23 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

Chemical Physics · Physics 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

We theoretically study the inelastic electron-H($2s$) scattering in a linearly polarized laser field in the domain of high scattering energies and moderate field intensities. We investigate the angular distributions and the resonance…

Atomic Physics · Physics 2023-09-04 Gabriela Buica

A single-atom 'double-slit' experiment is realized by photo-ionizing Rubidium atoms using two independent low power lasers. The photoelectron wave of well-defined energy recedes to the continuum either from the 5P or 6P states in the same…

Atomic Physics · Physics 2019-01-17 James Pursehouse , Andrew James Murray , Jonas Wätzel , Jamal Berakdar

When a diatomic molecule is ionized by an intense laser field, the ionization rate depends very strongly on the inter-nuclear separation. That dependence exhibits a pronounced maximum at the inter-nuclear separation known as the critical…

Chemical Physics · Physics 2015-04-21 Han Xu , Feng He , D. Kielpinski , R. T. Sang , I. V. Litvinyuk

We report on the fragmentation dynamics of triply charged, diatomic, molecular ions of NO and CO. Dissociative fragmentation after multiple ionization of NO and CO is studied under the impact of 200 keV proton beam using recoil-ion momentum…

Atomic Physics · Physics 2022-09-23 Avijit Duley , Narendra Nath Dutta , C. Bagdia , L. C. Tribedi , C. P. Safvan , A. H. Kelkar

We present the results of experimental studies of photon-negative ion interactions involving the dynamics of two electrons. Resonances associated with doubly excited states of Li^- and He^- have been observed using laser photodetachment…

Atomic Physics · Physics 2015-06-26 D. Hanstorp , G. Haeffler , A. E. Klinkmueller , U. Ljungblad , U. Berzinsh , I. Yu. Kiyan , D. J. Pegg

We present state-selective measurements on the NH$_2^{+}$ + H$^{+}$ and NH$^{+}$ + H$^{+}$ + H dissociation channels following single-photon double ionization at 61.5 eV of neutral NH$_{3}$, where the two photoelectrons and two cations are…

We formulate a three-dimensional semi-classical model to address triple and double ionization in three-electron atoms driven by intense infrared laser pulses. During time propagation, our model fully accounts for the Coulomb singularities,…

Atomic Physics · Physics 2022-04-20 M. B. Peters , G. P. Katsoulis , A. Emmanouilidou

Random quenched dilution of the triangular-lattice antiferromagnetic Ising model locally relieves frustration, leading to ordering phenomena. We have studied this system, under such dilution of one sublattice, using hard-spin mean-field…

Statistical Mechanics · Physics 2009-10-31 Huseyin Kaya , A. Nihat Berker

We theoretically investigate the laser wavelength dependence of asymmetric dissociation of H$_2^+$. It is found that the electron localization in molecular dissociation is significantly manipulated by varying the wavelength of the driving…

Atomic and Molecular Clusters · Physics 2015-06-03 Kunlong Liu , Weiyi Hong , Qingbin Zhang , Peixiang Lu
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