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We report the successful synthesis of single-crystals of the layered iridate, (Na$_{1-x}$Li$_{x}$)$_2$IrO$_3$, $0\leq x \leq 0.9$, and a thorough study of its structural, magnetic, thermal and transport properties. The new compound allows a…

Strongly Correlated Electrons · Physics 2014-01-07 G. Cao , T. F. Qi , L. Li , J. Terzic , V. S. Cao , S. J. Yuan , M. Tovar , G. Murthy , R. K. Kaul

We consider electrons on a honeycomb or triangular lattice doped to the saddle point of the bandstructure. We assume system parameters are such that spin density wave (SDW) order emerges below a temperature $T_N$ and investigate the nature…

Strongly Correlated Electrons · Physics 2013-05-15 Rahul Nandkishore , Gia-Wei Chern , Andrey V. Chubukov

Hexagonally deformed Fermi surfaces and strong nesting, found in topological insulators (TIs) such as $Bi_2Se_3$ and $Bi_2Te_3$, have led to several predictions of the existence of Density Wave order in these systems. Recent evidence for…

We use neutron scattering to study the spin and lattice structures of single crystal and powder samples of Na$_{1-\delta}$FeAs ($T_c = 23$ K). On cooling from room temperature, the system goes through a series of phase transitions: first…

Superconductivity · Physics 2009-07-10 Shiliang Li , Clarina de la Cruz , Q. Huang , G. F. Chen , T. -L. Xia , J. L. Lou , N. L. Wang , Pengcheng Dai

The layered honeycomb lattice iridate Cu$_2$IrO$_3$ is the closest realization of the Kitaev quantum spin liquid, primarily due to the enhanced interlayer separation and nearly ideal honeycomb lattice. We report pressure-induced structural…

A new honeycomb lattice iridate (La,Na)IrO$_3$ ($\approx$ LaNaIr$_2$O$_6$) is successfully synthesized from the spin-orbit coupled Mott insulator Na$_2$IrO$_3$ by replacing the interlayer Na$^+$ ions with La$^{3+}$ ions. (La,Na)IrO$_3$…

Strongly Correlated Electrons · Physics 2024-06-06 Yuya Haraguchi , Hiroko Aruga Katori

Transition-metal dichalcogenide IrTe2 has attracted attention because of striped lattice, charge ordering and superconductivity. We have investigated the surface structure of IrTe2, using low energy electron diffraction (LEED) and scanning…

Materials Science · Physics 2017-04-05 Chen Chen , Jisun Kim , Yifan Yang , Guixin Cao , Rongying Jin , E. W. Plummer

Direct experimental investigations of the low-energy electronic structure of the Na$_2$IrO$_3$ iridate insulator are sparse and draw two conflicting pictures. One relies on flat bands and a clear gap, the other involves dispersive states…

The silver ruthenium oxide AgRuO$_3$ consists of honeycomb [Ru$_2^{5+}$O$_6^{2-}$] layers, and can be considered an analogue of SrRu$_2$O$_6$ with a different intercalation stage. We present measurements of magnetic susceptibility and…

Li2MnO3 with a S=3/2 two-dimensional Mn honeycomb lattice has a Neel-type antiferromagnetic transition at TN=36 K with a broad maximum in the magnetic susceptibility at TM=48 K. We have investigated site percolation effects by replacing Mn…

Strongly Correlated Electrons · Physics 2015-06-22 Sanghyun Lee , Junghwan Park , Jiyeon Kim , Kun-Pyo Hong , Youngmi Song , Je-Geun Park

We investigated the crystal structure, magnetic behavior, and optical properties of the layered honeycomb compound Na2Cu2TeO6. X-ray and neutron diffraction confirmed a monoclinic structure, with Cu ions arranged in dimerized chains.…

Strongly Correlated Electrons · Physics 2025-08-25 Shubham Patil , S. D. Kaushik

We use low energy optical spectroscopy and first principles LDA+DMFT calculations to test the hypothesis that the anomalous transport properties of strongly correlated metals originate in the strong temperature dependence of their…

Strongly Correlated Electrons · Physics 2014-12-09 Xiaoyu Deng , Aaron Sternbach , Kristjan Haule , D. N. Basov , Gabriel Kotliar

The magnetic structure of honeycomb iridate Na$_2$IrO$_3$ is of paramount importance to its exotic properties. The magnetic order is established experimentally to be zigzag antiferromagnetic. However, the previous assignment of ordered…

Materials Science · Physics 2015-10-20 Kaige Hu , Fa Wang , Ji Feng

We consider the quasi-two-dimensional pseudo-spin-1/2 Kitaev - Heisenberg model proposed for A2IrO3 (A=Li, Na) compounds. The spin-wave excitation spectrum, the sublattice magnetization, and the transition temperatures are calculated in the…

Strongly Correlated Electrons · Physics 2016-08-24 A. A. Vladimirov , D. Ihle , N. M. Plakida

Cu$_2$IrO$_3$ has attracted recent interest due to its proximity to the Kitaev quantum spin liquid state and the complex structural response observed at high pressures. We use x-ray spectroscopy and scattering as well as electrical…

Single crystals of a honeycomb lattice antiferromagnet, Tb$_2$Ir$_3$Ga$_9$ were synthesized, and the physical properties have been studied. From magnetometry, a long-range antiferromagnetic ordering at $\approx$12.5 K with highly…

Mesoscale and Nanoscale Physics · Physics 2019-11-27 Mojammel A. Khan , Qiang Zhang , Jin-Ke Bao , Randy S. Fishman , Antia S. Botana , Y. Choi , G. Fabbris , D. Haskel , John Singleton , John F. Mitchell

We studied the effect of external pressure on the electrodynamic properties of $\alpha$-Li$_2$IrO$_3$ single crystals in the frequency range of the phonon modes and the Ir $d$-$d$ transitions. The abrupt hardening of several phonon modes…

Strongly Correlated Electrons · Physics 2019-06-14 V. Hermann , J. Ebad-Allah , F. Freund , A. Jesche , A. A. Tsirlin , P. Gegenwart , C. A. Kuntscher

We study the effect of isoelectronic doping and external pressure in tuning the ground state of the honeycomb iridate Na$_2$IrO$_3$ by combining optical spectroscopy with synchrotron x-ray diffraction measurements on single crystals. The…

Strongly Correlated Electrons · Physics 2018-01-31 V. Hermann , J. Ebad-Allah , F. Freund , I. M. Pietsch , A. Jesche , A. A. Tsirlin , J. Deisenhofer , M. Hanfland , P. Gegenwart , C. A. Kuntscher

We derive and study a spin one-half Hamiltonian on a honeycomb lattice describing the exchange interactions between Ir$^{4+}$ ions in a family of layered iridates $A_2$IrO$_3$ ($A$=Li,Na). Depending on the microscopic parameters, the…

Strongly Correlated Electrons · Physics 2014-11-20 Jiri Chaloupka , George Jackeli , Giniyat Khaliullin

Quantum magnets based on honeycomb lattices with low-coordination number offer a viable ground to realize exotic emergent quantum excitations and phenomena arising from the interplay between competing magnetic interactions, spin…

Strongly Correlated Electrons · Physics 2024-11-14 J. Khatua , M. Gomilsek , Kwang-Yong Choi , P. Khuntia