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Polaritons are compositional light-matter quasiparticles that arise as a result of strong coupling between a vacuum field of a resonant optical cavity and electronic excitations in quantum emitters. Reaching such a regime is often hard, as…

The Raman response of the metallic glass Ni$_{67}$Zr$_{33}$ is measured as a function of polarization and temperature and analyzed theoretically. Unexpectedly, the intensity in the range up to 300\wn increases upon cooling, which is…

Disordered Systems and Neural Networks · Physics 2015-05-20 B. Muschler , I. Tüttő , A. Zawadowski , J. Balogh , R. Hackl

Phonon polaritons are hybrid states of light and matter that are typically realised when optically active phonons couple strongly to photons. We suggest a new approach to realising phonon polaritons, by employing a transverse-pumping Raman…

Mesoscale and Nanoscale Physics · Physics 2024-10-22 Alexander N. Bourzutschky , Benjamin L. Lev , Jonathan Keeling

Raman scattering is an excellent method for simultaneously determining the dynamics of lattice, spin, and charge degrees of freedom. Furthermore, polarization selection rules in Raman scattering enable momentum-resolved quasiparticle…

Strongly Correlated Electrons · Physics 2024-09-04 Reshma Kumawat , Shubham Farswan , Simranjeet Kaur , Smriti Bhatia , Kaushik Sen

The strong coupling of molecules with surface plasmons results in hybrid states which are part molecule, part surface-bound light. Since molecular resonances may acquire the spatial coherence of plasmons, which have mm-scale propagation…

Optics · Physics 2022-05-26 Marie S Rider , Rakesh Arul , Jeremy J Baumberg , William L Barnes

Strong coupling between light and matter is possible with a variety of organic materials. In contrast to the simpler inorganic case, organic materials often have a complicated spectrum, with vibrationally dressed electronic transitions.…

Mesoscale and Nanoscale Physics · Physics 2018-02-02 M. Ahsan Zeb , Peter G. Kirton , Jonathan Keeling

Room temperature cavity quantum electrodynamics with molecular materials in optical cavities offers exciting prospects for controlling electronic, nuclear and photonic degrees of freedom for applications in physics, chemistry and materials…

Quantum Physics · Physics 2025-01-15 Felipe Herrera , William L. Barnes

A theoretical model of resonant hyper-Raman scattering by an ensemble of spherical semiconductor quantum dots has been developed. The electronic intermediate states are described as Wannier-Mott excitons in the framework of the envelope…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 E. Menendez-Proupin , C. Trallero-Giner , A. Garcia-Cristobal

We formulate a scattering theory to study magnetic films in microwave cavities beyond the independent-spin and rotating wave approximations of the Tavis-Cummings model. We demonstrate that strong coupling can be realized not only for the…

Mesoscale and Nanoscale Physics · Physics 2015-03-26 Yunshan Cao , Peng Yan , Hans Huebl , Sebastian T. B. Goennenwein , Gerrit E. W. Bauer

It is shown that induced Raman scattering of electromagnetic waves in the strongly magnetized electron-positron plasma of pulsar magnetosphere may be important for wave propagation and as an effective saturation mechanism for…

Astrophysics · Physics 2009-10-30 Maxim Lyutikov

Molecular polaritons are the optical excitations which emerge when molecular transitions interact strongly with confined electromagnetic fields. Increasing interest in the hybrid molecular-photonic materials that host these excitations…

Mesoscale and Nanoscale Physics · Physics 2018-02-26 Raphael F. Ribeiro , Luis A. Martínez-Martínez , Matthew Du , Jorge Campos-Gonzalez-Angulo , Joel Yuen-Zhou

This review outlines several linear optical effects featured by molecular polaritons arising in the collective strong light-matter coupling regime. Under weak laser irradiation and when the single-molecule light-matter coupling can be…

Microcavity polaritons are strongly interacting hybrid light-matter quasiparticles, which are promising for the development of novel light sources and active photonic devices. Here, we report polariton lasing in the UV spectral range in…

As pioneering experiments have shown, strong vibrational coupling between molecular vibrations and light modes in an optical cavity can significantly alter molecular properties and even affect chemical reactivity. However, the current…

Chemical Physics · Physics 2024-07-26 Thomas Schnappinger , Markus Kowalewski

We present the effects of resonator birefringence on the cavity-enhanced interfacing of quantum states of light and matter, including the first observation of single photons with a time-dependent polarisation state that evolves within their…

Quantum Physics · Physics 2019-03-27 Thomas D. Barrett , Oliver Barter , Dustin Stuart , Ben Yuen , Axel Kuhn

Molecular polaritons are hybrid states of photonic and molecular character that form when molecules strongly interact with light. Strong coupling tunes energy levels and importantly, can modify molecular properties (e.g. photoreaction…

Chemical Physics · Physics 2023-02-14 Francesca Fassioli , Kyu Hyung Park , Sarah E. Bard , Gregory D. Scholes

There is an increasing scientific and technological interest on the design and implementation of nanoscale sources of quantum light. Here, we investigate the quantum statistics of the light scattered from a plasmonic nanocavity coupled to a…

Mesoscale and Nanoscale Physics · Physics 2019-03-14 R. Sáez-Blázquez , J. Feist , A. I. Fernández-Domínguez , F. J. García-Vidal

Vibrational Raman scattering -- a process where light exchanges energy with a molecular vibration through inelastic scattering -- is most fundamentally described in a quantum framework where both light and vibration are quantized. When the…

Quantum electrodynamics theory of the resonance Raman scattering is developed for an atom in a close proximity to a carbon nanotube. The theory predicts a dramatic enhancement of the Raman intensity in the strong atomic coupling regime to…

Mesoscale and Nanoscale Physics · Physics 2015-12-07 I. V. Bondarev

We present a detailed calculation of intensities of two-phonon and four-phonon Raman peaks in graphene. Writing the low-energy hamiltonian of the interaction of electrons with the crystal vibrations and the electromagnetic field from pure…

Materials Science · Physics 2009-11-13 D. M. Basko
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