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Trirutile-type LiFe$_2$F$_6$ is a charge-ordered material with Fe$^{2+}$/Fe$^{3+}$ configuration. Here its physical properties, including magnetism, electronic structure, phase transition, and charge ordering, are studied theoretically. On…

Materials Science · Physics 2017-12-11 Ling-Fang Lin , Qiao-Ru Xu , Yang Zhang , Jun-Jie Zhang , Yan-Ping Liang , Shuai Dong

Competing interactions and geometric frustration provide favourable conditions for exotic states of matter. Such competition often causes multiple phase transitions as a function of temperature and can lead to magnetic structures that break…

The coupling between magnetic order and ferroelectricity has been under intense investigation in a wide range of transition-metal oxides. The strongest coupling is obtained in so-called magnetically-induced multiferroics where…

Materials Science · Physics 2015-05-13 V. S. Zapf , M. Kenzelmann , F. Wolff-Fabris , F. Balakirev , Y. Chen

We describe a mechanism by which both ferroelectric polarization and magnetization can be created in nonpolar, nonmagnetic materials. Using a combination of phenomenological modeling and first-principles calculations, we demonstrate that…

Materials Science · Physics 2024-04-26 Carolina Paiva , Michael Fechner , Dominik M. Juraschek

With a combined ab initio density functional and model Hamiltonian approach we establish that in the recently discovered multiferroic phase of the manganite Sr$_{1/2}$Ba$_{1/2}$MnO$_{3}$ the polar distortion of Mn and O ions is stabilized…

Materials Science · Physics 2015-03-09 Gianluca Giovannetti , Sanjeev Kumar , Carmine Ortix , Massimo Capone , Jeroen van den Brink

Controlling magnetism using voltage is highly desired for applications, but remains challenging due to fundamental contradiction between polarity and magnetism. Here we propose a mechanism to manipulate magnetic domain walls in…

Materials Science · Physics 2021-03-22 Jun Chen , Shuai Dong

The electric field effect on magnetism was examined in the multiferroic conical magnet Mn$_2$GeO$_4$, which shows a strong coupling between ferromagnetic and ferroelectric order parameters. The systematic evaluation of the electric…

Strongly Correlated Electrons · Physics 2020-08-12 Jonas K. H. Fischer , Hiroki Ueda , Tsuyoshi Kimura

We propose a microscopic theory for magnetic switching of electric polarization (P) in the spin-spiral multiferroics by taking TbMnO3 and DyMnO3 as examples. We reproduce their phase diagrams under a magnetic field H_ex by Monte-Carlo…

Strongly Correlated Electrons · Physics 2010-10-29 Masahito Mochizuki , Nobuo Furukawa

Using first principles calculations, we study the microscopic origin of ferroelectricity (FE) induced by magnetic order in the orthorhombic HoMnO3. We obtain the largest ferroelectric polarization observed in the whole class of improper…

Materials Science · Physics 2009-11-13 Silvia Picozzi , Kunihiko Yamauchi , Biplab Sanyal , Ivan A. Sergienko , Elbio Dagotto

By means of first-principles simulations, we unambiguously show that improper ferroelectricity in magnetite in the low-temperature insulating phase is driven by charge-ordering. An accurate comparison between monoclinic ferroelectric Cc and…

Materials Science · Physics 2015-05-13 Kunihiko Yamauchi , Tetsuya Fukushima , Silvia Picozzi

Spin-driven multiferroics exhibit strong magnetoelectric coupling, with notable polarization changes under a magnetic field, but these effects are usually limited to high-Z magnetic insulators with low electronic polarization. In this work,…

Materials Science · Physics 2024-12-31 Ranquan Cao , Ruizhi Dong , Ruixiang Fei , Yugui Yao

A collective excitation of the spin structure in a magnetic insulator can transmit spin-angular momentum with negligible dissipation. This quantum of a spin wave, introduced more than nine decades ago, has always been manipulated through…

All-electrical and programmable manipulations of ferromagnetic bits are highly pursued for the aim of high integration and low energy consumption in modern information technology. Methods based on the spin-orbit torque switching in heavy…

Magnetoelectric crystals have the interesting property that they allow electric fields to induce magnetic polarizations, and vice versa, magnetic fields to generate ferroelectric polarizations. Having such a magnetoelectric coupling usually…

Mesoscale and Nanoscale Physics · Physics 2024-01-08 Carmine Ortix , Jeroen van den Brink

Despite remarkable progress in developing multifunctional materials, spin-driven ferroelectrics featuring both spontaneous magnetization and electric polarization are still rare. Among such ferromagnetic ferroelectrics are conical spin…

Strongly Correlated Electrons · Physics 2017-06-09 T. Honda , J. S. White , A. B. Harris , L. C. Chapon , A. Fennell , B. Roessli , O. Zaharko , Y. Murakami , M. Kenzelmann , T. Kimura

The chiral components in the magnetic order in multiferroic MnWO4 have been studied by neutron diffraction using spherical polarization analysis as a function of temperature and of external electric field. We show that sufficiently close to…

Strongly Correlated Electrons · Physics 2009-07-31 T. Finger , D. Senff , K. Schmalzl , W. Schmidt , L. P. Regnault , P. Becker , L. Bohaty , M. Braden

The olivine compound Mn2GeO4 is shown to feature both a ferroelectric polarization and a ferromagnetic magnetization that are directly coupled and point along the same direction. We show that a spin spiral generates ferroelectricity (FE),…

Materials Science · Physics 2012-08-07 J. S. White , T. Honda , K. Kimura , T. Kimura , Ch. Niedermayer , O. Zaharko , A. Poole , B. Roessli , M. Kenzelmann

Composite multiferroics, heterostructures of ferromagnetic (FM) and ferroelectric (FE) materials, are characterized by a remarkable magnetoelectric effect at the interface. Previous work has supported the ferromagnetic structure with…

Mesoscale and Nanoscale Physics · Physics 2016-04-01 Zidong Wang , Malcolm J. Grimson

Magnetoelectric and magnetoelastic phenomena correlated with a phase transition into noncollinear magnetic phase have been investigated for single crystals of CuFeO2 with a frustrated triangular lattice. CuFeO2 exhibits several…

Strongly Correlated Electrons · Physics 2009-11-11 T. Kimura , J. C. Lashley , A. P. Ramirez

The effects of high magnetic fields applied perpendicular to the spontaneous ferroelectric polarization on single crystals of BiFeO$_3$ were investigated through magnetization, magnetostriction, and neutron diffraction measurements. The…

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