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On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet…

Strongly Correlated Electrons · Physics 2016-03-02 M. Gomilsek , M. Klanjsek , M. Pregelj , F. C. Coomer , H. Luetkens , O. Zaharko , T. Fennell , Y. Li , Q. M. Zhang , A. Zorko

Quantum spin liquids provide paradigmatic examples of highly entangled quantum states of matter. Frustration is the key mechanism to favor spin liquids over more conventional magnetically ordered states. Here we propose to engineer…

Strongly Correlated Electrons · Physics 2021-11-29 Alessio Chiocchetta , Dominik Kiese , Carl Philipp Zelle , Francesco Piazza , Sebastian Diehl

The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…

A spin liquid is a new state of matter with topological order where the spin moments continue to fluctuate coherently down to the lowest temperatures rather than develop static long-range magnetic order as found in conventional magnets. For…

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was predicted for the Ising antiferromagnetic triangular model more than half a century…

Strongly Correlated Electrons · Physics 2022-11-15 T. Arh , B. Sana , M. Pregelj , P. Khuntia , Z. Jagličić , M. D. Le , P. Biswas , A. Ozarowski , A. Zorko

The interplay of electronic interactions and frustration in crystalline systems leads to a panoply of correlated phases, including exotic Mott insulators with non-trivial patterns of entanglement. Disorder introduces additional quantum…

Strongly Correlated Electrons · Physics 2025-01-03 Sunghoon Kim , Mohammad Saad , Dan Mao , Adhip Agarwala , Debanjan Chowdhury

This article is an introductory review of the physics of quantum spin liquid (QSL) states. Quantum magnetism is a rapidly evolving field, and recent developments reveal that the ground states and low-energy physics of frustrated spin…

Strongly Correlated Electrons · Physics 2017-04-21 Yi Zhou , Kazushi Kanoda , Tai-Kai Ng

Cs2CuCl4 is known to possess a quantum spin liquid phase with antiferromagnetic interaction below 2.8 K. We report the observation of a new metastable magnetic phase of the triangular frustrated quantum spin system Cs2CuCl4 induced by the…

Strongly Correlated Electrons · Physics 2017-12-18 Hyeong-Jin Kim , C. R. S. Haines , C. Liu , Sae Hwan Chun , Kee Hoon Kim , H. T. Yi , Sang-Wook Cheong , Siddharth S. Saxena

Quantum spin liquids (QSLs) represent a novel state of matter in which quantum fluctuations prevent conventional magnetic order from being established, and the spins remain disordered even at zero temperature. There have been many…

Strongly Correlated Electrons · Physics 2018-10-11 Zhen Ma , Kejing Ran , Jinghui Wang , Song Bao , Zhengwei Cai , Shichao Li , Jinsheng Wen

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

Strongly Correlated Electrons · Physics 2019-07-02 A. Zorko , M. Pregelj , M. Klanjšek , M. Gomilšek , Z. Jagličić , J. S. Lord , J. A. T. Verezhak , T. Shang , W. Sun , J. -X. Mi

The search for novel phases of matter is a central theme of modern physics, with some of the most intriguing examples provided by the spin liquids found in magnets with competing, or "frustrated" interactions. Ca$_{10}$Cr$_7$O$_{28}$, a…

Strongly Correlated Electrons · Physics 2025-04-11 Rico Pohle , Han Yan , Nic Shannon

Recent years have witnessed the emergence of spin supersolids in frustrated quantum magnets, establishing a material-based platform for supersolidity beyond its original context in solid helium. A spin supersolid is characterized by the…

Strongly Correlated Electrons · Physics 2026-05-26 Yixuan Huang , Seiji Yunoki , Sadamichi Maekawa

In a quantum spin liquid, the magnetic moments of the constituent electron spins evade classical long-range order to form an exotic state that is quantum entangled and coherent over macroscopic length scales [1-2]. Such phases offer…

There have been tremendous experimental and theoretical efforts toward discovery of quantum spin liquid phase in honeycomb-based-lattice materials with strong spin-orbit coupling. Here the bond-dependent Kitaev interaction between local…

Strongly Correlated Electrons · Physics 2016-12-23 Heung-Sik Kim , Yong Baek Kim , Hae-Young Kee

Frustration in magnetic materials arising from competing exchange interactions can prevent the system from adopting long-range magnetic order and can instead lead to a diverse range of novel quantum and topological states with exotic…

Strongly Correlated Electrons · Physics 2023-11-16 J. Khatua , B. Sana , A. Zorko , M. Gomilšek , K. Sethupathi M. S. Ramachandra Rao , M. Baenitz , B. Schmidt , P. Khuntia

Quantum spin liquids are exotic states of matter which form when strongly frustrated magnetic interactions induce a highly entangled quantum paramagnet far below the energy scale of the magnetic interactions. Three-dimensional cases are…

Quantum spin-1/2 kagome Heisenberg antiferromagnet is the representative frustrated system possibly hosting a spin liquid. Clarifying the nature of this elusive topological phase is a key challenge in condensed matter, however, even…

Strongly Correlated Electrons · Physics 2015-06-16 Satoshi Nishimoto , Naokazu Shibata , Chisa Hotta

A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

Strongly Correlated Electrons · Physics 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin
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