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Transition metal compounds with the $(t_{2g})^4$ electronic configuration are expected to be nonmagnetic atomic singlets both in the weakly interacting regime due to spin-orbit coupling, as well as in the Coulomb dominated regime with…

Strongly Correlated Electrons · Physics 2017-01-16 Christopher Svoboda , Mohit Randeria , Nandini Trivedi

Strong electronic correlations are often associated with the proximity of a Mott insulating state. In recent years however, it has become increasingly clear that the Hund's rule coupling (intra-atomic exchange) is responsible for strong…

Strongly Correlated Electrons · Physics 2013-03-20 Antoine Georges , Luca de' Medici , Jernej Mravlje

Based on density functional theory (DFT) calculations, we predict that a monolayer of OsCl$_3$---a layered material whose interlayer coupling is weaker than in graphite---possesses a quantum anomalous Hall (QAH) insulating phase generated…

Strongly Correlated Electrons · Physics 2017-05-10 Xian-Lei Sheng , Branislav K. Nikolic

The metal to insulator transition (MIT) in Mott-Hubbard systems is one of the most important discoveries in condensed matter physics, and results in abrupt orbital transitions from the insulating to metallic phases by elevating temperature…

Applied Physics · Physics 2019-04-02 Jikun Chen , Haiyang Hu , Takeaki Yajima , Jiaou Wang , Binghui Ge , Hongliang Dong , Yong Jiang , Nuofu Chen

We study a three-orbital Hubbard model with negative Hund coupling in infinite dimensions, combining dynamical mean-field theory with continuous time quantum Monte Carlo simulations. This model, which is relevant for the description of…

Superconductivity · Physics 2018-12-13 Kosuke Ishigaki , Joji Nasu , Akihisa Koga , Shintaro Hoshino , Philipp Werner

We study roles of electron correlations on topological insulators on the honeycomb lattice with the spin-orbit interaction. Accurate variational Monte Carlo calculations show that the increasing on-site Coulomb interactions cause a strong…

Strongly Correlated Electrons · Physics 2011-05-24 Youhei Yamaji , Masatoshi Imada

Using resonant x-ray diffraction, we observe an easy c-axis collinear antiferromagnetic structure for the bilayer Sr$_3$Ir$_2$O$_7$, a significant contrast to the single layer Sr$_2$IrO$_4$ with in-plane canted moments. Based on a…

Strongly Correlated Electrons · Physics 2012-12-11 J. W. Kim , Y. Choi , Jungho Kim , J. F. Mitchell , G. Jackeli , M. Daghofer , J. van den Brink , G. Khaliullin , B. J. Kim

We investigate the Hubbard model on two typical frustrated lattices in two dimensions, the kagome lattice and the anisotropic triangular lattice, by means of the cellular dynamical mean field theory. We show that the metallic phase is…

Strongly Correlated Electrons · Physics 2015-05-13 Takuma Ohashi , Tsutomu Momoi , Hirokazu Tsunetsugu , Norio Kawakami

Using density functional theory and LDA+U method, we investigate magnetic and electronic structure of Y$_{2}$Ir$_{2}$O$_{7}$ and rare-earth based pyrochlore iridates. Our study reveals that the ground state is a non-collinear magnetic…

Materials Science · Physics 2010-03-18 Xiangang Wan , Jinming Dong , Sergey Y. Savrasov

We study the non-equilibrium dynamics of a simple model for V2O3 that consists of a quarter-filled Hubbard model for two orbitals that are split by a weak crystal field. Peculiarities of this model are: (1) a Mott insulator whose gap…

Strongly Correlated Electrons · Physics 2015-05-05 Matteo Sandri , Michele Fabrizio

In Mott insulators with a half-filled $t_{2g}$ shell the Hund's rule coupling induces a spin-3/2 orbital-singlet ground state. The spin-orbit interaction is not expected to qualitatively impact low-energy degrees of freedom in such systems.…

Strongly Correlated Electrons · Physics 2023-08-28 Leonid V. Pourovskii

We study \textit{ab initio} a pyrochlore compound, CsW$_{2}$O$_{6}$, which exhibits a yet unexplained metal-insulator transition. We find that (1) the reported low-$T$ structure is likely inaccurate and the correct structure has a twice…

Superconductivity · Physics 2017-01-10 S. V. Streltsov , I. I. Mazin , R. Heid , K. -P. Bohnen

The periodic Anderson model (PAM) is studied within the framework of dynamical mean-field theory, with particular emphasis on the interaction-driven Mott transition it contains, and on resultant Mott insulators of both Mott-Hubbard and…

Strongly Correlated Electrons · Physics 2016-12-15 David E. Logan , Martin R. Galpin , Jonathan Mannouch

We report the low temperature properties of a new series of pyrochlore iridates R2Ir2O7 (R = rare-earth elements). We found that the compounds with R = Pr, Sm, Nd, and Eu exhibit metallic conductivity, whereas those with smaller rare-earth…

Strongly Correlated Electrons · Physics 2009-11-07 D. Yanagishima , Y. Maeno

In the presence of quenched disorder, the interplay between local magnetic-moment formation and Anderson localization for electrons at a zero-temperature, metal-insulator transition (MIT) remains a long unresolved problem. Here, we study…

Disordered Systems and Neural Networks · Physics 2024-10-17 Xinghai Zhang , Matthew S. Foster

Effects of spin-orbit interactions in condensed matter are an important and rapidly evolving topic. Strong competition between spin-orbit, on-site Coulomb and crystalline electric field interactions in iridates drives exotic quantum states…

Strongly Correlated Electrons · Physics 2018-02-27 Gang Cao , Pedro Schlottmann

A Mott insulator sometimes induces unconventional superconductivity in its neighbors when doped and/or pressurized. Because the phase diagram should be strongly related to the microscopic mechanism of the superconductivity, it is important…

Strongly Correlated Electrons · Physics 2019-05-14 Yoshitaka Kawasugi , Kazuhiro Seki , Satoshi Tajima , Jiang Pu , Taishi Takenobu , Seiji Yunoki , Hiroshi M. Yamamoto , Reizo Kato

The magnetic properties and Mott transition of the Hubbard model on the square lattice with frustration are studied at half-filling and zero temperature by the variational cluster approximation. When the on-site repulsion $U$ is large,…

Strongly Correlated Electrons · Physics 2015-06-15 A. Yamada , K. Seki , R. Eder , Y. Ohta

The moir\'e Hubbard model describes correlations in certain homobilayer twisted transition metal dichalcogenides. Using exact diagonalization and density matrix renormalization group methods, we find magnetic Mott insulating and metallic…

Strongly Correlated Electrons · Physics 2022-11-15 Alexander Wietek , Jie Wang , Jiawei Zang , Jennifer Cano , Antoine Georges , Andrew Millis

The Shastry-Sutherland lattice, one of the simplest systems with geometric frustration, which has an exact eigenstate by putting singlets on diagonal bonds, can be realized in a group of layered compounds and rises both theoretical and…

Strongly Correlated Electrons · Physics 2014-05-06 Hai-Di Liu , Yao-Hua Chen , Heng-Fu Lin , Hong-Shuai Tao , Wu-Ming Liu