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Nanoporous carbon-based supercapacitors store electricity through adsorption of ions from the electrolyte at the surface of the electrodes. Room temperature ionic liquids, which show the largest ion concentrations among organic liquid…

Molecular dynamics simulations were used to explain the origin and properties of electrical double-layer capacitance in short graphene nanochannels with width below 2 nm. The results explain the previously reported experimental result on…

Chemical Physics · Physics 2017-04-06 Yinghua Qiu , Yunfei Chen

In the recent experiments [Chmiola et al, Science 313, 1760 (2006); Largeot et al, J. Am. Chem. Soc. 130, 2730 (2008)] an anomalous increase of the capacitance with a decrease of the pore size of a carbon-based porous electric double-layer…

Soft Condensed Matter · Physics 2015-03-17 S. Kondrat , A. Kornyshev

Supercapacitors, based on the fast ion transportation, are specialized to provide high power, long stability, and efficient energy storage with highly porous electrode materials. However, their low energy density and specific capacitance…

Materials Science · Physics 2013-11-07 Hao Yang , Santhakumar Kannappan , Amaresh S. Pandian , Jae-Hyung Jang , Yun Sung Lee , Wu Lu

Supercapacitors are energy storage devices able to deliver electricity with a high power. They consist of porous carbon electrodes in a concentrated electrolyte. Charged is stored by the adsorption of ions at the electrode surface.…

Chemical Physics · Physics 2018-11-26 Benjamin Rotenberg , Mathieu Salanne , Patrice Simon

Carbon nanotubes are excellent nano-electromechanical systems, combining high resonance frequency, low mass, and large zero-point motion. At cryogenic temperatures they display high mechanical quality factors. Equally they are outstanding…

Mesoscale and Nanoscale Physics · Physics 2024-03-06 N. Hüttner , S. Blien , P. Steger , A. N. Loh , R. Graaf , A. K. Hüttel

With the ability to selectively control ionic flux, biological protein ion channels perform a fundamental role in many physiological processes. For practical applications that require the functionality of a biological ion channel, graphene…

In recent experiments, unprecedentedly large values for the conductivity of electrolytes through carbon nanotubes (CNTs) have been measured, possibly owing to flow slip and a high pore surface charge density whose origin is still unknown.…

Soft Condensed Matter · Physics 2023-07-25 Théo Hennequin , Manoel Manghi , Adrien Noury , Francois Henn , Vincent Jourdain , John Palmeri

Carbon-carbon supercapacitors are high power electrochemical energy storage systems which store energy through reversible ion adsorption at the electrode-electrolyte interface. Due to the complex structure of the porous carbons used as…

Materials Science · Physics 2024-06-19 El Hassane Lahrar , Patrice Simon , Céline Merlet

Owing to its peculiar energy dispersion, the quantum capacitance property of graphene can be exploited in a two-dimensional layered capacitor configuration. Using graphene and boron nitride respectively as the electrodes and the insulating…

Quantum Physics · Physics 2017-05-19 Sina Khorasani , Akshay Koottandavida

Nanoporous supercapacitors are an important player in the field of energy storage that fill the gap between dielectric capacitors and batteries. The key challenge in the development of supercapacitors is the perceived trade-off between…

Materials Science · Physics 2016-06-22 Alpha A Lee , Dominic Vella , Alain Goriely , Svyatoslav Kondrat

Quantum dots are nanostructures made of semiconducting materials that are engineered to hold a small amount of electric charge (a few electrons) that is controlled by external gate and may hence be considered as tunable artificial atoms. A…

Strongly Correlated Electrons · Physics 2019-01-07 Rok Zitko

We have investigated the quantum capacitance ($C_Q$) in functionalized graphene, modified with ad-atoms from different groups in the periodic table. Changes in the electronic band structure of graphene upon functionalization and…

Materials Science · Physics 2019-06-17 Sruthi T , Kartick Tarafder

When an ionic liquid adsorbs onto a porous electrode, its ionic arrangement is deeply modified due to a screening of the Coulombic interactions by the metallic surface and by the confinement imposed upon it by the electrode's morphology. In…

Quantum interference has dramatic effects on electronic transport through nanotube contacts. In optimal configuration the intertube conductance can approach that of a perfect nanotube ($4e^2/h$). The maximum conductance increases rapidly…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Calin Buia , Alper Buldum , Jian Ping Lu

During the dielectric breakdown process of thin solid-state nanopores, the application of high voltages may cause the formation of multi-nanopores on one chip, which number and sizes are important for their applications. Here, simulations…

Chemical Physics · Physics 2024-10-30 Yinghua Qiu , Long Ma , Zhe Liu , Hongwen Zhang , Bowen Ai , Xinman Tu

The interplay between electronic properties and optical response enables the realization of novel types of materials with tunable responses. Superconductors are well known to exhibit profound changes in the electronic structure related to…

Optics · Physics 2021-06-23 Kaveh Delfanazari , Otto L. Muskens

Ionic transport in nanopores or nanochannels is key to many cellular processes and is now being explored as a method for DNA/polymer sequencing and detection. Although apparently simple in its scope, the study of ionic dynamics in confined…

Mesoscale and Nanoscale Physics · Physics 2013-06-13 Andrew Meyertholen , Massimiliano Di Ventra

Ion transport through nanopores permeates through many areas of science and technology, from cell behavior to sensing and separation to catalysis and batteries. Two-dimensional materials, such as graphene, molybdenum disulfide (MoS$_2$),…

Mesoscale and Nanoscale Physics · Physics 2019-07-19 Subin Sahu , Michael Zwolak

For a capacitor made of a semiconducting carbon nanotube (CNT) suspended above a metallic gate, Coulomb correlations between individual electrons can lead to a capacitance that is much larger than the geometric capacitance. We argue that…

Strongly Correlated Electrons · Physics 2015-04-22 Han Fu , B. I. Shklovskii , Brian Skinner
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