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Due to the resource criticality of rare-earths (RE), an alternative to the well-known Nd$_2$Fe$_{14}$B magnets with a lower amount of critical elements is required. In this work, density functional theory (DFT) calculations to investigate…

Materials Science · Physics 2023-02-08 Stephan Erdmann

Emergent phenomena at polar-nonpolar oxide interfaces have been studied intensely in pursuit of next-generation oxide electronics and spintronics. Here we report the disentanglement of critical thicknesses for electron reconstruction and…

Nanomagnets with giant magnetic anisotropy energy and long coherence time are desired for various technological innovations such as quantum information procession and storage. Based on the first-principles calculations and model analyses,…

Materials Science · Physics 2020-08-26 Jie Li , Lei Gu , Ruqian Wu

The properties of the novel heavy fermion superconductor Ce$_3$PtIn$_{11}$ are investigated by thermodynamic and transport measurements at ambient and under hydrostatic pressure. At ambient pressure the compound exhibits two successive…

Strongly Correlated Electrons · Physics 2015-12-03 Jan Prokleška , Marie Kratochvílová , Klára Uhlířová , Vladimír Sechovský , Jeroen Custers

The electronic structures of the ferromagnetic superconductors $\mathrm{UGe}_2$ and $\mathrm{UCoGe}$ in the paramagnetic phase were studied by angle-resolved photoelectron spectroscopy using soft X-rays ($h\nu =400-500$). The quasi-particle…

We present electronic structure calculations for the one-dimensional magnetic chain compounds Ca_3CoRhO_6 and Ca_3FeRhO_6. The calculations are based on density functional theory and the local density approximation. We use the augmented…

Strongly Correlated Electrons · Physics 2008-01-26 V. Eyert , U. Schwingenschloegl , C. Hackenberger , T. Kopp , R. Fresard , U. Eckern

The structural properties of the uranium-encapsulated nano-cage U@Au14 are predicted using density functional theory. The presence of the uranium atom makes the Au14 structure more stable than the empty Au14-cage, with a triplet ground…

Atomic and Molecular Clusters · Physics 2013-12-30 Yang Gao , Xing Dai , Seung-gu Kang , Camilo Andres Jimenez Cruz , Minsi Xin , Yan Meng , Jie Han , Zhigang Wang , Ruhong Zhou

Neutron diffraction measurements on a high quality single crystal of CeAu2Ge2 reveal two new magnetic structures that coexist with commensurate long range antiferromagnetic order below the Neel temperature T_N ~ 14 K. The new magnetic…

Strongly Correlated Electrons · Physics 2012-09-03 D. K. Singh , A. Thamizhavel , J. W. Lynn , S. K. Dhar , T. Hermann

A family of magnetic halide double perovskites (HDPs) have recently attracted attention due to their potential to broaden application areas of halide double perovskites into e.g. spintronics. Up to date the theoretical modelling of these…

Materials Science · Physics 2022-11-30 Johan Klarbring , Utkarsh Singh , Sergei I. Simak , Igor A. Abrikosov

We investigate the magnetic structure of Mn3-xFexSn2 using neutron powder diffraction experiments and electronic structure calculations. These alloys crystallize in the orthorhombic Ni3Sn2 type of structure (Pnma) and comprise two…

Materials Science · Physics 2013-09-03 Q. Recour , V. Ban , Z. Gercsi , T. Mazet , M. Francois , B. Malaman

By means of first-principles calculations, the structural stability, mechanical properties and electronic structure of the newly synthesized incompressible Re2C, Re2N, Re3N and an analogous compound Re3C have been investigated. Our results…

Materials Science · Physics 2015-03-09 Naihua Miao , Baisheng Sa , Jian Zhou , Zhimei Sun , Rajeev Ahuja

The antiferromagnetic (AFM) state has been investigated in the three heavy-fermion compounds URu2Si2, UPd2Al3, and UNi2Al3 by measuring dV/dI(V) curves of point contacts at different temperatures (1.5-20 K) and magnetic fields (0-28 T). The…

Strongly Correlated Electrons · Physics 2009-11-07 Yu. G. Naidyuk , O. E. Kvitnitskaya , A. G. M. Jansen , C. Geibel , A. A. Menovsky , P. Wyder

We have performed a detailed analysis of the magnetic (collinear and noncollinear) order and atomic and the electron structures of UO2, PuO2 and UN on the basis of density functional theory with the Hubbard electron correlation correction…

Materials Science · Physics 2017-08-23 Denis Gryaznov , Eugene Heifets , David Sedmidubsky

Quaternary Heusler alloys Co$_2$Cr$_{1-x}$Fe$_{x}$Al with varying Cr to Fe ratio $x$ were investigated experimentally and theoretically. The electronic structure and spectroscopic properties were calculated using the full relativistic…

We report results of joint experimental and theoretical studies on magnetoelectric (ME) compounds Co4Nb2O9 and Co4Ta2O9. On the experimental side, we present results of the magnetization and dielectric permittivity measurements in the…

Materials Science · Physics 2016-09-23 I. V. Solovyev , T. V. Kolodiazhnyi

The electronic structures of four semiconductor compounds BaCu2S2, BaCu2Se2, BaAg2S2, and BaAg2Se2 are studied by density functional theory using both semi-local and hybrid functionals. The ionization energies and electron affinities were…

Materials Science · Physics 2013-09-13 Aditi Krishnapriyan , Phillip T. Barton , Maosheng Miao , Ram Seshadri

Correlation between geometry, electronic structure and magnetism of solids is both intriguing and elusive. This is particularly strongly manifested in small clusters, where a vast number of unusual structures appear. Here, we employ density…

Atomic and Molecular Clusters · Physics 2015-11-23 R. Logemann , G. A. de Wijs , M. I. Katsnelson , A. Kirilyuk

We report magnetic neutron-diffraction and electrical resistivity studies on single crystals of the heavy-fermion antiferromagnet CeRhIn$_{5}$ at pressures up to 2.3 GPa. These experiments show that the staggered moment of Ce and the…

The structural and magnetic properties of transition metal-doped Mn$_3$SnC are studied with an aim to understand the effect of transition metal atom on magnetostructural properties of the antiperovskite compound. The doped…

Materials Science · Physics 2020-04-03 V. N. Gaonkar , E. T. Dias , A. K. Nigam , K. R. Priolkar

We investigate the crystal structure, magnetic properties, and crystalline-electric field of tetragonal, $I4_1/amd$, NaCeO$_2$. In this compound, Ce$^{3+}$ ions form a tetragonally elongated diamond lattice coupled by antiferromagnetic…

Strongly Correlated Electrons · Physics 2021-01-26 Mitchell M. Bordelon , Joshua D. Bocarsly , Lorenzo Posthuma , Arnab Banerjee , Qiang Zhang , Stephen D. Wilson