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By means of electronic transport, we study the transverse magnetic anisotropy of an individual Fe$_4$ single-molecule magnet (SMM) embedded in a three-terminal junction. In particular, we determine in situ the transverse anisotropy of the…

Mesoscale and Nanoscale Physics · Physics 2016-08-10 M. Misiorny , E. Burzurí , R. Gaudenzi , K. Park , M. Leijnse , M. R. Wegewijs , J. Paaske , A. Cornia , H. S. J. van der Zant

We have measured quantum transport through an individual Fe$_4$ single-molecule magnet embedded in a three-terminal device geometry. The characteristic zero-field splittings of adjacent charge states and their magnetic field evolution are…

Using first-principles methods we study theoretically the properties of an individual $\{Fe_4\}$ single-molecule magnet (SMM) attached to metallic leads in a single-electron transistor geometry. We show that the conductive leads do not…

Mesoscale and Nanoscale Physics · Physics 2014-07-01 J. F. Nossa , M. Fhokrul Islam , C. M. Canali , M. R. Pederson

We investigate how the electron-vibron coupling influences electron transport via an anisotropic magnetic molecule, such as a single-molecule magnet (SMM) Fe$_4$, by using a model Hamiltonian with parameter values obtained from…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Alexander McCaskey , Yoh Yamamoto , Michael Warnock , Enrique Burzuri , Herre S. J. van der Zant , Kyungwha Park

Spin-polarized transport through bistable magnetic adatoms or single-molecule magnets (SMMs), which exhibit both uniaxial and transverse magnetic anisotropy, is considered theoretically. The main focus is on the impact of transverse…

Mesoscale and Nanoscale Physics · Physics 2014-07-22 Maciej Misiorny , Józef Barnaś

We present a theoretical approach to calculate the molecular magnetic anisotropy parameters, $D_M$ and $E_M$ for single molecule magnets in any eigenstate of the exchange Hamiltonian, treating the anisotropy Hamiltonian as a perturbation.…

Strongly Correlated Electrons · Physics 2009-11-13 Rajamani Raghunathan , S. Ramasesha , Diptiman Sen

We analyze the electronic transport through a model spin-1 molecule as a function of temperature, magnetic field and bias voltage. We consider the effect of magnetic anisotropy, which can be generated experimentally by stretching the…

Strongly Correlated Electrons · Physics 2011-06-24 P. S. Cornaglia , P. Roura Bas , A. A. Aligia , C. A. Balseiro

We have theoretically studied the full counting statistics of electron transport through a single-molecule magnet (SMM) with an arbitrary angle between the applied magnetic field and the SMM's easy axis above the sequential tunneling…

Mesoscale and Nanoscale Physics · Physics 2011-04-21 Hai-Bin Xue , Y. -H. Nie , Z. -J. Li , J. -Q. Liang

We use an aluminium single electron transistor with a magnetic gate to directly quantify the chemical potential anisotropy of GaMnAs materials. Uniaxial and cubic contributions to the chemical potential anisotropy are determined from field…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 C. Ciccarelli , L. P. Zarbo , A. C. Irvine , R. P. Campion , B. L. Gallagher , J. Wunderlich , T. Jungwirth , A. J. Ferguson

Single-molecule transistors provide a unique experimental tool to investigate the coupling between charge transport and the molecular degrees of freedom in individual molecules. One interesting class of molecules for such experiments are…

We present a method for precisely measuring the tunnel splitting in single-molecule magnets using electron-spin resonance, and use these measurements to precisely and independently determine the underlying transverse anisotropy parameter,…

Mesoscale and Nanoscale Physics · Physics 2016-12-13 Charles A. Collett , Rafael A. Allão Cassaro , Jonathan R. Friedman

We report transport measurements through a single-molecule magnet, the Mn12 derivative [Mn12O12(O2C-C6H4-SAc)16(H2O)4], in a single-molecule transistor geometry. Thiol groups connect the molecule to gold electrodes that are fabricated by…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 H. B. Heersche , Z. de Groot , J. A. Folk , H. S. J. van der Zant , C. Romeike , M. R. Wegewijs , L. Zobbi , D. Barreca , E. Tondello , A. Cornia

We study linear electron transport through a single-molecule magnet (SMM) and the interplay of its anisotropic spin with quantized vibrational distortions of the molecule. We show that, despite the longitudinal anisotropy barrier and small…

Mesoscale and Nanoscale Physics · Physics 2011-02-15 F. May , M. R. Wegewijs , W. Hofstetter

To understand the effect of molecular environment on the electronic and magnetic properties of the single-molecule magnet (SMM) Mn$_{12}$, we explore two possible means for adding extra electrons to molecule. We explore both substitution of…

Materials Science · Physics 2009-11-10 Kyungwha Park , Mark R. Pederson

We study single-electron transport in a three-ion molecule with strong uniaxial anisotropy and in the presence of a transverse magnetic field. Two magnetic ions are connected to each other through a third, nonmagnetic ion. The magnetic ions…

Mesoscale and Nanoscale Physics · Physics 2014-05-12 Javier I. Romero , Eduardo R. Mucciolo

We theoretically analyze the spectrum of a magnetic molecule when its charge and spin can couple to the molecular vibrations. More specifically, we show that the interplay between charge-vibron and spin-vibron coupling leads to a…

Mesoscale and Nanoscale Physics · Physics 2018-07-04 Ahmed Kenawy , Janine Splettstoesser , Maciej Misiorny

Anisotropic magnetic molecules can be employed to manipulate charge transport in molecular nanojunctions. Charge transport through a molecular orbital connected to two leads and exchange-coupled with a precessing anisotropic molecular spin…

Mesoscale and Nanoscale Physics · Physics 2025-09-09 Milena Filipovic

This paper discusses transport methods for the investigation of the (Ga,Mn)As magnetic anisotropy. Typical magnetoresistance behaviour for different anisotropy types is discussed, focusing on an in depth discussion of the anisotropy…

Mesoscale and Nanoscale Physics · Physics 2008-03-03 K. Pappert , C. Gould , M. Sawicki , J. Wenisch , K. Brunner , G. Schmidt , L. W. Molenkamp

An electron transport is studied in the system which consists of scanning tunneling microscopy-single molecule magnet-metal. Due to quantum tunneling of magnetization in single-molecule magnet, linear response conductance exhibits stepwise…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Gwang-Hee Kim , Tae-Suk Kim

Spins in molecular magnets can experience both anisotropic exchange interactions and on-site magnetic anisotropy. In this paper we study the effect of exchange anisotropy on the molecular magnetic anisotropy both with and without on-site…

Materials Science · Physics 2018-12-12 Sumit Haldar , Rajamani Raghunathan , Jean-Pascal Sutter , S. Ramasesha
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