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Using time-dependent density functional theory, high-harmonic generation (HHG) is studied in one-dimensional structures of sizes from a single nucleus up to hundreds of nuclei. The HHG cutoff is observed to extent linearly with the system…

Atomic Physics · Physics 2018-04-27 Kenneth K. Hansen , Dieter Bauer , Lars Bojer Madsen

An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…

The interaction of relativistically strong tailored laser pulses with an atomic system is considered. Due to a special tailoring of the laser pulse, the suppression of the relativistic drift of the ionized electron and a dramatic…

Atomic Physics · Physics 2007-05-23 M. Klaiber , K. Z. Hatsagortsyan , C. H. Keitel

High-harmonic generation (HHG) is a coherent optical process in which the incident photon energy is up-converted to the multiples of its initial energy. In solids, under the influence of a strong laser field, electron-hole (e-h) pairs are…

High-order harmonic generation (HHG) in solids has emerged as a versatile platform for exploring ultrafast and quantum-coherent phenomena in condensed matter. Recent advances reveal Berry-phase and topological effects in harmonic emission,…

Optics · Physics 2025-10-20 Marcelo F. Ciappina

The combination of high-order harmonic generation (HHG) with resonant XUV excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process is investigated theoretically. In this setup, the…

Atomic Physics · Physics 2023-01-10 Christian Buth , Markus C. Kohler , Joachim Ullrich , Christoph H. Keitel

High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated…

Atomic Physics · Physics 2008-11-14 Y. J. Chen , J. Liu , Bambi Hu

High harmonic generation (HHG) from semiconductors and insulators has become a very active area of research due to its great potential for developing compact HHG devices. Here we show that by growing monolayers (ML) of insulators on…

Atomic Physics · Physics 2016-12-28 Néstor F. Aguirre , Fernando Martín

High order harmonic generation from clusters is a controversial topic: conflicting theories exist, with different explanations for similar experimental observations. From an experimental point of view, separating the contributions from…

Atomic and Molecular Clusters · Physics 2015-06-12 H. Ruf , C. Handschin , R. Cireasa , N. Thiré , A. Ferré , S. Petit , D. Descamps , E. Mével , E. Constant , V. Blanchet , B. Fabre , Y. Mairesse

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

Optics · Physics 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

We present studies of high-order harmonic generation (HHG) at laser intensities well above saturation. We use driving laser pulses which present a particular electron dynamics in the turn-on stage. Our results predict an increasing on the…

Atomic Physics · Physics 2015-06-19 J. A. Pérez-Hernández , M. F. Ciappina , M. Lewenstein , A. Zaïr , L. Roso

We report a study of high harmonic generation from noble gas clusters of xenon atoms in a gas jet. Harmonic spectra were investigated as a function of backing pressure, showing spectral shifts due to the nanoplasma electrons in the…

Atomic Physics · Physics 2016-02-17 M. Aladi , R. Bolla , P. Rácz , I. B. Földes

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

Optics · Physics 2020-05-20 Jonas Wätzel , Jamal Berakdar

Acting as a highly nonlinear response to the strong laser field, high harmonic generation (HHG) naturally contains the fingerprints of atomic and electronic properties of materials. Electronic properties of a solid such as band structure…

Materials Science · Physics 2023-04-20 Shi-Qi Hu , Hui Zhao , Xin-Bao Liu , Da-Qiang Chen , Sheng Meng

We present a study of the possibility to significantly enhance the efficiency of high-order harmonic generation (HHG) using few-cycle optical waveforms obtained by superposing two laser pulses of different color delayed optimally relative…

Optics · Physics 2024-12-11 O. V. Meshkov , M. Yu. Emelin , M. Yu. Ryabikin

Preparation of nonclassical light with special quantum properties is essential for quantum technologies. High-harmonic generation (HHG) is a process which not only enables the creation of attosecond pulses but also has the potential to…

Quantum Physics · Physics 2026-03-03 Ákos Gombkötő , Péter Ádám , David Theidel , Tamás Kiss