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Chemical imaging enabled by Raman processes is crucial to investigating biological and chemical samples in a label-free manner. Stimulated Raman spectroscopy (SRS) overcomes the key limitation associated with low signal levels in…

Optics · Physics 2026-03-25 Florian M. Schweizer , Hannah Terrasa , Manish Garg

Cavity-enhanced direct frequency comb spectroscopy combines broad spectral bandwidth, high spectral resolution, precise frequency calibration, and ultrahigh detection sensitivity, all in one experimental platform based on an optical…

Optics · Physics 2009-11-13 Michael J. Thorpe , Jun Ye

Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of…

Dual-comb spectroscopy is a rapidly developing technique enabling ultraprecise broadband optical diagnostics of atoms and molecules. This powerful tool typically requires two phase-locked femtosecond lasers, yet it has been shown that it…

The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…

Optics · Physics 2026-02-17 John J. McCauley , DylanP. Tooley , R. Jason Jones

We devise a new detection technique for mid-infrared multi-heterodyne spectroscopy. As an experimental implementation, mid-infrared light interrogates a gas sample in the 3-$\mu$m region of the fundamental CH, OH, NH stretch in molecules…

Optics · Physics 2020-03-17 Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

The femtosecond laser frequency comb has enabled the 21st century revolution in optical synthesis and metrology. A particularly compelling technique that relies on the broadband coherence of two laser frequency combs is dual-comb…

Optics · Physics 2023-07-19 Vicente Duran , Santiago Tainta , Victor Torres-Company

Computational techniques have gained significant traction in photonics, enabling the co-design of hardware and data processing algorithms to drastically simplify optical system architectures and improve their performance. However, their…

Optics · Physics 2026-01-19 J. J. Navarro-Alventosa , A. Aupart-Acosta , V. Duran

Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…

Optics · Physics 2020-06-04 A. V. Muraviev , D. Konnov , K. L. Vodopyanov

An electro-optic dual comb system based on chirped-pulse waveforms is used to simultaneously acquire temporally magnified rapid passage signals and normal spectral line shapes from the back-transformation to the time domain.…

Optics · Physics 2022-08-10 Jasper R. Stroud , David F. Plusquellic

Integrated Kerr micro-combs, a powerful source of many wavelengths for photonic RF and microwave signal processing, are particularly useful for transversal filter systems. They have many advantages including a compact footprint, high…

Applied Physics · Physics 2021-03-08 Mengxi Tan , Xingyuan Xu , Jiayang Wu , David J. Moss

We demonstrate the advantages of THz frequency combs for high-resolution spectroscopy. This benefits from wide spectral coverage and the exact knowledge of the frequency position of each comb component. Heterodyne detection combined with a…

Instrumentation and Detectors · Physics 2024-12-03 Francis Hindle , Alexandra Khabbaz , Anthony Roucou , Jean-Francois Lampin , Gaël Mouret

Dissipative Kerr-microresonator soliton combs (hereafter called soliton combs) are promising to realize chip scale integration of full soliton comb systems providing high precision, broad spectral coverage and a coherent link to the…

Dual-comb spectroscopy (DCS) utilizes a pair of broadband mutually coherent laser frequency combs to enable high-resolution, high-accuracy spectroscopic measurements with atomic-clock-level frequency referencing, and rapid, multiplexed…

Optics · Physics 2025-10-01 D. Konnov , A. Muraviev , K. L. Vodopyanov

Optical frequency combs, named for their comb-like peaks in the spectrum, are essential for various sensing applications. As the technology develops, its performance has reached the standard quantum limit dictated by the quantum…

Quantum Physics · Physics 2026-05-25 Haowei Shi , Quntao Zhuang

Dual THz comb spectroscopy has the potential to be used as universal THz spectroscopy with high spectral resolution, high spectral accuracy, and broad spectral coverage; however, the requirement for dual stabilized femtosecond lasers…

Instrumentation and Detectors · Physics 2019-08-06 Guoqing Hu , Tatsuya Mizuguchi , Ryo Oe , Kazuki Nitta , Xin Zhao , Takeo Minamikawa , Ting Li , Zheng Zheng , Takeshi Yasui

Optical frequency combs are key to optical precision measurements. While most frequency combs operate in the near-infrared regime, many applications require combs at mid-infrared, visible or even ultra-violet wavelengths. Frequency combs…

We explore the advantages of a free-form dual-comb spectroscopy (DCS) platform based on time-programmable frequency combs for real-time, penalty-free apodized scanning. In traditional DCS, the fundamental spectral resolution, which equals…

Frequency-modulated (FM) combs are produced by mode-locked lasers in which the electric field has a linearly chirped frequency and nearly constant amplitude. This regime of operation occurs naturally in certain laser systems and constitutes…

We have carried out dual-comb spectroscopy and observed in a simultaneous acquisition a 140-THz-wide spectrum from 1.0 to 1.9 {\mu}m using two fiber-based frequency combs phase-locked to each other. This ultra-broad wavelength bandwidth is…