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Related papers: Ultrafast charge redistribution in small iodine co…

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The double-slit interference in single-photon ionization of the diatomic molecular ion $\mathrm{H}_2^+$ is theoretically studied beyond the dipole approximation. Via simulating and comparing the interactions of the prealigned…

Atomic Physics · Physics 2021-11-24 Kunlong Liu , Yibo Hu , Qingbin Zhang , Peixiang Lu

Experimental charge exchange and energy loss data for the transmission of slow highly charged Xe ions through ultra-thin polymeric carbon membranes are presented. Surprisingly, two distinct exit charge state distributions accompanied by…

Ionization of atoms and molecules in laser fields can lead to various interesting interference structures in the photoelectron spectrum. For the case of a super-intense extreme ultraviolet laser pulse, we identify a novel petal-like…

Atomic Physics · Physics 2022-03-29 Lei Geng , Hao Liang , K. Krajewska , Liang-You Peng , Qihuang Gong

Conical intersections between electronic states often dictate the chemistry of photoexcited molecules. Recently developed sources of ultrashort extreme ultraviolet (XUV) pulses tuned to element-specific transitions in molecules allow for…

We investigate the possibility to monitor the dynamics of autoionizing states in real time and control the yields of different ionization channels in helium by simulating XUV-pump IR-probe experiments focused on the N=2 threshold. The XUV…

Atomic Physics · Physics 2015-05-18 Luca Argenti , Eva Lindroth

The recently proposed Partition Theory (PT) [J.Phys.Chem.A 111, 2229 (2007)] is illustrated on a simple one-dimensional model of a heteronuclear diatomic molecule. It is shown that a sharp definition for the charge of molecular fragments…

Other Condensed Matter · Physics 2016-09-28 Morrel H. Cohen , Adam Wasserman , Roberto Car , Kieron Burke

We analyze the photoelectron angular distribution in two-pathway interference between non\-resonant one-photon and resonant two-photon ionization of neon. We consider a bichromatic femtosecond XUV pulse whose fundamental frequency is tuned…

We study the ionization of atomic hydrogen in the direction of polarization due to a linearly polarized XUV pulse in the presence a strong field IR. We describe the photoelectron spectra as an interference problem in the time domain.…

Atomic Physics · Physics 2016-11-15 Ana Alicia Gramajo , Renata Della Picca , Carlos Roberto Garibotti , Diego Arbó

It is shown that it is feasible to use ultrashort time delay between two XUV femtosecond pulses in order to control two photon resonant ionization. The proposal is demonstrated on the spectrum of Helium, in terms of nonperturbative…

Atomic Physics · Physics 2019-08-22 Theodoros Mercouris , Yannis Komninos , Cleanthes A. Nicolaides

Semi-classical molecular dynamics simulations of small rare gas clusters in short laser pulses of 100 nm wavelength were performed. For comparison, the cluster response to 800 nm laser pulses was investigated as well. The inner ionization…

Atomic and Molecular Clusters · Physics 2009-11-10 D. Bauer

Non-equilibrium processes following the irradiation of atomic clusters with short pulses of vacuum ultraviolet radiation are modelled using kinetic Boltzmann equations. The dependence of the ionization dynamics on the cluster size is…

Plasma Physics · Physics 2009-11-13 B. Ziaja , H. Wabnitz , E. Weckert , T. Möller

We theoretically investigate the role of complex dipole phase in the attosecond probing of charge migration. The iodobromoacetylene ion (ICCBr$^+$) is considered as an example, in which one can probe charge migration by accessing both the…

Chemical Physics · Physics 2022-02-23 Yuki Kobayashi , Daniel M. Neumark , Stephen R. Leone

Sudden ionisation of a relatively large molecule can initiate a correlation-driven process dubbed charge migration, where the electron density distribution is expected to rapidly change. Capturing this few-femtosecond/attosecond charge…

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

We investigate the laser-assisted single XUV photon double ionization of ground state helium. By solving full six-dimensional time-dependent schr{\"o}dinger equation, we study the correlation and angular distribution. The discussion in…

Atomic Physics · Physics 2020-03-24 Fengzheng Zhu , Genliang Li , Aihua Liu

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

Ionization of matter by energetic radiation generally causes complex secondary reactions which are hard to decipher. Using large helium nanodroplets irradiated by XUV photons, we show that the full chain of processes ensuing primary…

Atomic and Molecular Clusters · Physics 2023-07-26 L. Ben Ltaief , K. Sishodia , S. Mandal , S. De , S. R. Krishnan , C. Medina , N. Pal , R. Richter , T. Fennel , M. Mudrich

We study the EUV/soft X-ray emission generated by charge transfer between solar wind heavy ions and interstellar H and He neutral atoms in the inner Heliosphere. We present heliospheric maps and spectra for stationary solar wind, depending…

Phase-shift differences and amplitude ratios of the outgoing $s$ and $d$ continuum wave packets generated by two-photon ionization of helium atoms are determined from the photoelectron angular distributions obtained using velocity map…

The UV photochemistry of small heteroaromatic molecules serves as a testbed for understanding fundamental photoinduced transformations in moderately complex compounds, including isomerization, ring-opening, and molecular dissociation. Here,…