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We suggest a new spin orientation mechanism for localized electrons: $dynamic~electron~spin~polarization~provided~by~nuclear~spin~fluctuations$. The angular momentum for the electrons is gained from the nuclear spin system via the hyperfine…

Mesoscale and Nanoscale Physics · Physics 2020-10-14 D. S. Smirnov , T. S. Shamirzaev , D. R. Yakovlev , M. Bayer

We studied the zero-field dynamic nuclear spin polarization in a single In$_{0.75}$Al$_{0.25}$As/Al$_{0.3}$Ga$_{0.7}$As quantum dot. Even without any external magnetic field, the positive trion excited by the circularly-polarized light…

Mesoscale and Nanoscale Physics · Physics 2017-03-20 Ryosuke Matsusaki , Reina Kaji , Sohta Yamamoto , Hirotaka Sasakura , Satoru Adachi

Single crystal silicon is an excellent system in which to explore dynamic nuclear polarization (DNP), as it exhibits a continuum of properties from metallic to insulating as a function of doping concentration and temperature. At low doping…

Materials Science · Physics 2011-09-09 Anatoly E. Dementyev , David G. Cory , Chandrasekhar Ramanathan

Solid-state quantum registers consisting of optically active electron spins with nearby nuclear spins are promising building blocks for future quantum technologies. For electron spin-1 registers, dynamical decoupling (DD) quantum gates have…

In this work, we devise a fast and effective nuclear spin hyperpolarization scheme, which is in principle magnetic field and temperature independent. We use this scheme to experimentally demonstrate polarizations of up to 66% for phosphorus…

Dynamic nuclear polarization (DNP) is a method of enhancing NMR signals via the transfer of polarization from electron spins to nuclear spins using on-resonance microwave (MW) irradiation. In most cases, monochromatic continuous-wave (MCW)…

Chemical Physics · Physics 2022-11-17 Daphna Shimon , Kelly A. Cantwell , Linta Joseph , Chandrasekhar Ramanathan

Atomic spin sensors are essential for beyond-the-standard-model exploration, biomagnetic measurement, and quantum navigation. While the traditional DC mode spin-exchange relaxation-free (SERF) comagnetometer achieves ultrahigh sensitivity,…

Atomic Physics · Physics 2025-05-27 Xiaofei Huang , Kai Wei , Yang Rui , Dinghui Gong , Saixin Zhou , Jie Zheng , Wei Quan

We show that detuned optical pulse trains with a modest spectral width can polarize nuclear spins in InAs quantum dots. The pulse bandwidth is large enough to excite a coherent superposition of both electron spin eigenstates in these…

Quantum Physics · Physics 2015-05-27 S. G. Carter , Sophia E. Economou , A. Shabaev , A. S. Bracker

We propose a method for the estimation of the initial polarization of spinful nuclei of the 13 C isotope in diamond via a measurement of the evolution of the coherence of an NV center spin qubit. Existing polarization measurement methods…

Quantum Physics · Physics 2025-04-01 Mateusz Kuniej , Katarzyna Roszak

The use of nuclear spins as physical sensing systems is disadvantaged by their low signal responsivity, particularly when compared to sensing techniques based on electron spins. This primarily results from the small nuclear gyromagnetic…

We present an experimental study of the dynamics underlying the buildup and decay of dynamical nuclear spin polarization in a single semiconductor quantum dot. Our experiment shows that the nuclei can be polarized on a time scale of a few…

Optics · Physics 2007-08-02 P. Maletinsky , A. Badolato , A. Imamoglu

$^1$H nuclear spin-lattice relaxation and Dynamic Nuclear Polarization (DNP) have been studied in amorphous samples of trehalose sugar doped with TEMPO radicals by means of mechanical milling, in the 1.6 K $\div$ 4.2 K temperature range.…

We studied the dynamic nuclear spin polarization of nitrogen in negatively charged nitrogen-vacancy (NV) centers in diamond both experimentally and theoretically over a wide range of magnetic fields from 0 to 1100 G covering both the…

Quantum Physics · Physics 2021-01-04 Laima Busaite , Reinis Lazda , Andris Berzins , Marcis Auzinsh , Ruvin Ferber , Florian Gahbauer

We have explored the manifold physical scenario emerging from a model of Dynamic Nuclear Polarization (DNP) via thermal mixing under the hypothesis of highly effective electron-electron interaction. When the electron and nuclear reservoirs…

Statistical Mechanics · Physics 2017-09-13 Sonia Colombo Serra , Alberto Rosso , Fabio Tedoldi

Polarization transfers from an electron spin to a nuclear spin are essential for various physical tasks, such as dynamic nuclear polarization in nuclear magnetic resonance and quantum state transformations on hybrid electron-nuclear spin…

Quantum Physics · Physics 2015-11-11 Haidong Yuan , Robert Zeier , Nikolas Pomplun , Steffen J. Glaser , Navin Khaneja

Optically-pumped color centers in semiconductor powders can potentially induce high levels of nuclear spin polarization in surrounding solids or fluids at or near ambient conditions, but complications stemming from the random orientation of…

The interplay of dynamical nuclear polarization (DNP) and leakage current through a double quantum dot in the spin-blockade regime is analyzed. A finite DNP is built up due to a competition between hyperfine (HF) spin-flip transitions and…

Mesoscale and Nanoscale Physics · Physics 2013-07-30 Anders Mathias Lunde , Carlos López-Monís , Ioanna A. Vasiliadou , Luis L. Bonilla , Gloria Platero

The optically induced polarization of localized electron spins in an ensemble of quantum dots (QDs) dephases due to the interaction with the surrounding nuclear spins. Despite this dephasing, the spins in the QDs can be controlled to…

Mesoscale and Nanoscale Physics · Physics 2022-04-08 P. Schering , G. S. Uhrig

We present a quantum mechanical theory of optically induced dynamic nuclear polarization applicable to quantum dots and other interacting spin systems. The exact steady state of the optically driven coupled electron-nuclear system is…

Mesoscale and Nanoscale Physics · Physics 2019-02-04 Thomas Nutz , Edwin Barnes , Sophia E. Economou

We experimentally investigate the protection of electron spin coherence of nitrogen vacancy (NV) center in diamond by dynamical nuclear polarization. The electron spin decoherence of an NV center is caused by the magnetic ield fluctuation…