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We demonstrate optically pumped dynamic nuclear polarization of 29-Si nuclear spins that are strongly coupled to paramagnetic color centers in 4H- and 6H-SiC. The 99 +/- 1% degree of polarization at room temperature corresponds to an…

We proposed and demonstrated that the nuclear spins of the host lattice in GaAs double quantum dots can be strongly polarized in either of two opposite directions, parallel or antiparallel to an external magnetic field. The direction is…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Ryo Takahashi , Kimitoshi Kono , Seigo Tarucha , Keiji Ono

Dynamic Nuclear Polarization (DNP) has enabled enormous gains in magnetic resonance signals and led to vastly accelerated NMR/MRI imaging and spectroscopy. Unlike conventional cw-techniques, DNP methods that exploit the full electron…

Applied Physics · Physics 2018-11-27 A. Ajoy , R. Nazaryan , K. Liu , X. Lv , B. Safvati , G. Wang , E. Druga , J. A. Reimer , D. Suter , C. Ramanathan , C. A. Meriles , A. Pines

Hyper-polarization of nuclear spins is crucial for advancing nuclear magnetic resonance (NMR) and quantum information technologies, as nuclear spins typically exhibit extremely low polarization at room temperature due to their small…

Quantum Physics · Physics 2025-05-20 Haiyang Li , Hao Liao , Ping Wang

We report on the dynamic nuclear polarization of a single charge-tunable self-assembled InAs/GaAs quantum dot in a longitudinal magnetic field of $\sim$0.2T. The hyperfine interaction between the optically oriented electron and nuclei spins…

Hybrid quantum registers consisting of different types of qubits offer a range of advantages as well as challenges. The main challenge is that some types of qubits react only slowly to external control fields, thus considerably slowing down…

Quantum Physics · Physics 2019-12-25 Jingfu Zhang , Swathi S. Hegde , Dieter Suter

Dynamic nuclear polarization via contact with electronic spins has emerged as an attractive route to enhance the sensitivity of nuclear magnetic resonance (NMR) beyond the traditional limits imposed by magnetic field strength and…

We reveal an interplay between temperature and radical concentration necessary to establish thermal mixing (TM) as an efficient dynamic nuclear polarization (DNP) mechanism. We conducted DNP experiments by hyperpolarizing widely used DNP…

Quantum Physics · Physics 2024-04-12 Ludovica M. Epasto , Thibaud Maimbourg , Alberto Rosso , Dennis Kurzbach

The hyperpolarization of nuclear spins can enable powerful imaging and sensing techniques provided the hyperpolarization is sufficiently long-lived. Recent experiments on nanodiamond $^{13}$C nuclear spins demonstrate that relaxation times…

Mesoscale and Nanoscale Physics · Physics 2024-02-20 Gargee Sharma , Torsten Gaebel , Ewa Rej , David J. Reilly , Sophia E. Economou , Edwin Barnes

We report a new transport feature in a GaAs lateral double quantum dot that emerges only for magnetic field sweeps and shows hysteresis due to dynamic nuclear spin polarization (DNP). This DNP signal appears in the Coulomb blockade regime…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Takashi Kobayashi , Kenichi Hitachi , Satoshi Sasaki , Koji Muraki

We propose a practical implementation of a two-qubit entanglement engine which denotes a scheme to generate quantum correlations through purely dissipative processes. On a diamond platform, the electron spin transitions of two…

Quantum Physics · Physics 2024-01-17 Shishir Khandelwal , Shashwat Kumar , Nicolas Palazzo , Géraldine Haack , Mayeul Chipaux

Magnetic resonance imaging in ultra-low fields is often limited by mediocre signal-to-noise ratio hindering a higher resolution. Overhauser dynamic nuclear polarisation (O-DNP) using nitroxide radicals has been an efficient solution for…

The electronic and nuclear spin degrees of freedom for donor impurities in semiconductors form ultra coherent two-level systems that are useful for quantum information applications. Spins naturally have magnetic dipoles, so alternating…

Quantum Physics · Physics 2017-01-25 A. J. Sigillito , A. M. Tyryshkin , T. Schenkel , A. A. Houck , S. A. Lyon

The nature of the nano-scale environment presents a major challenge for solid-state implementation of spin-based qubits. In this work, a single electron spin in an optically pumped nanometer-sized III-V semiconductor quantum dot is used to…

We propose a novel scheme to efficiently polarize and manipulate the electron spin in a quantum dot. This scheme is based on the spin-orbit interaction and it possesses following advantages: (1) The direction and the strength of the spin…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Qing-feng Sun , X. C. Xie

Enhancing the polarization of nuclear spins surrounding the nitrogen-vacancy (NV) center in diamond has attracted widespread attention recently due to its various applications. Here we present an analytical theory and comprehensive…

Quantum Physics · Physics 2016-07-15 Ping Wang , Bao Liu , Wen Yang

We study the mechanism of dynamical nuclear spin polarization by hyperfine interaction in spin-blocked double quantum dot system. We calculate the hyperfine transition rates and solve the master equations for the nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Changxue Deng , Xuedong Hu

A broad effort is underway to improve the sensitivity of nuclear magnetic resonance through the use of dynamic nuclear polarization. Nitrogen-vacancy (NV) centers in diamond offer an appealing platform because these paramagnetic defects can…

The electron-nuclei (hyperfine) interaction is central to spin qubits in solid state systems. It can be a severe decoherence source but also allows dynamic access to the nuclear spin states. We study a double quantum dot exposed to an…

Mesoscale and Nanoscale Physics · Physics 2013-06-13 Gunnar Petersen , Eric A. Hoffmann , Dieter Schuh , Werner Wegscheider , Geza Giedke , Stefan Ludwig

Color-center-hosting semiconductors are emerging as promising source materials for low-field dynamic nuclear polarization (DNP) at or near room temperature, but hyperfine broadening, susceptibility to magnetic field heterogeneity, and…

Quantum Physics · Physics 2022-06-01 J. Henshaw , D. Pagliero , P. R. Zangara , B. Franzoni , A. Ajoy , R. Acosta , J. A. Reimer , A. Pines , C. A. Meriles
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