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Evidence for a strong spin-lattice coupling in multiferroic HoMnO_3 is derived from thermal expansion measurements along a- and c-axis. The magnetoelastic effect results in sizable anomalies of the thermal expansivities at the…

Strongly Correlated Electrons · Physics 2009-11-11 C. dela Cruz , F. Yen , B. Lorenz , Y. Q. Wang , Y. Y. Sun , M. M. Gospodinov , C. W. Chu

Magnetic and ferroelectric properties of layered geometrically frustrated cluster compound FeTe$_2$O$_5$Br were investigated with single-crystal neutron diffraction and dielectric measurements. Incommensurate amplitude modulated magnetic…

Materials Science · Physics 2009-10-01 M. Pregelj , O. Zaharko , A. Zorko , Z. Kutnjak , P. Jeglic , P. J. Brown , M. Jagodic , Z. Jaglicic , H. Berger , D. Arcon

The structural, electronic and lattice dielectric properties of multiferroic TbMn$_2$O$_5$ are investigated using density functional theory within the generalized gradient approximation (GGA). We use collinear spin approximations and ignore…

Materials Science · Physics 2009-11-13 Chenjie Wang , Guang-Can Guo , Lixin He

CuFeO_2 is one of the multiferroic materials and is the first case that the electric polarization is not explained by the magnetostriction model or the spin-current model. We have studied this material using soft x-ray resonant diffraction…

We have performed high resolution neutron diffraction and inelastic neutron scattering experiments in the frustrated multiferroic hexagonal compounds RMnO3 (R=Ho, Yb, Sc, Y), which provide evidence of a strong magneto-elastic coupling in…

Strongly Correlated Electrons · Physics 2009-06-01 X. Fabreges , S. Petit , I. Mirebeau , S. Pailhes , L. Pinsard , A. Forget , M. T. Fernandez-Diaz , F. Porcher

While 3$d$-containing materials display strong electron correlations, narrow band widths, and robust magnetism, 5$d$ systems are recognized for strong spin-orbit coupling, increased hybridization, and more diffuse orbitals. Combining these…

The intrinsic noncollinear spin patterns in rare-earth pyrochlore are physically interesting, hosting many emergent properties, e.g. spin ice and monopole-type excitation. Recently, the magnetic monopole excitation of spin ice systems was…

Materials Science · Physics 2015-12-18 Lin Lin , Y. L. Xie , J. -J. Wen , Shuai Dong , Z. B. Yan , J. -M. Liu

Given the paucity of single phase multiferroic materials (with large ferromagnetic moment), composite systems seem an attractive solution in the quest to realize magnetoelectric cou-pling between ferromagnetic and ferroelectric order…

Mesoscale and Nanoscale Physics · Physics 2014-09-15 P. Jain , Q. Wang , M. Roldan , A. Glavic , V. Lauter , C. Urban , Z. Bi , T. Ahmed , J. Zhu , M. Varela , Q. Jia , M. R. Fitzsimmons

We report the results of various measurements, namely magnetization, complex dielectric permittivity and electric polarization (P) on Dy2BaNiO5 as a function of temperature (T) and magnetic-field (H), apart from heat-capacity (C), with the…

Materials Science · Physics 2015-06-15 Kiran Singh , Tathamay Basu , S. Chowki , N. Mahapotra , K. Iyer , P. L. Paulose , E. V. Sampathkumaran

In antiferromagnets, the interplay of spin frustration and spin-lattice coupling has been extensively studied as the source of complex spin patterns and exotic magnetism. Here, we demonstrate that, although neglected in the past, the…

The correlation between static magnetoelectric coupling and magnetic structure was investigated in $TbMn_{0.98}Fe_{0.02}O_{3}$ with magnetic field up to 8 T and down to 2 K. Single-crystal neutron diffraction experiments reveal a…

The olivine compound Mn2GeO4 is shown to feature both a ferroelectric polarization and a ferromagnetic magnetization that are directly coupled and point along the same direction. We show that a spin spiral generates ferroelectricity (FE),…

Materials Science · Physics 2012-08-07 J. S. White , T. Honda , K. Kimura , T. Kimura , Ch. Niedermayer , O. Zaharko , A. Poole , B. Roessli , M. Kenzelmann

We report an unusual canted magnetism due to 3d and 4f electrons, occupying two different crystallographic sites, with its consequence to electric dipole order. This is based on neutron powder diffraction measurements on Tb2BaNiO5…

We have demonstrated magnetodielectric (MD) coupling in an Ising-chain magnet Sr2Ca2CoMn2O9, via detailed investigation of ac susceptibility and dielectric constant as a function of temperature, magnetic field and frequency. Sr2Ca2CoMn2O9…

Strongly Correlated Electrons · Physics 2021-07-23 Tathamay Basu , Nahed Sakly , Alain Pautrat , Fabien Veillon , Olivier Perez , Vincent Caignaert , Bernard Raveau , Vincent Hardy

We combine two aspects of magnetic frustration, multiferroicity and emergent quasi-particles in spin liquids, by studying magneto-electric monopoles. Spin ice offers to couple these emergent topological defects to external fields, and to…

Strongly Correlated Electrons · Physics 2015-06-24 Ludovic D. C. Jaubert , R. Moessner

Observation of ferroelectricity among non-d0 systems, which was believed for a long time an unrealistic concept, led to various proposals for the mechanisms to explain the same (i.e. magnetically induced ferroelectricity) during last…

Spin supersolids and spin superfluids reveal complex canted spin structures with independent order of longitudinal and transverse spin components. This work addresses the question whether these exotic phases can exhibit spin-driven…

We have carried out a first-principles theoretical study of the magnetically induced polarization in orthorhombic TbMnO3, a prototypical material in which a cycloidal spin structure generates an electric polarization via the spin-orbit…

Materials Science · Physics 2009-12-16 Andrei Malashevich , David Vanderbilt

We report the observation of electric polarization in the magnetically ordered state of the Haldane chain compound, Gd$_2$BaNiO$_5$, with strongly correlated magnetic and dielectric properties. The results of dc magnetic susceptibility and…

Materials Science · Physics 2015-06-22 S. Chowki , Tathamay Basu , K. Singh , N. Mohapatra , E. V. Sampathkumaran

From magnetic susceptibility, dielectric permittivity, electric polarization and specific heat measurements, we discover spin-induced ferroelectricity and magnetoelectric coupling in Mn3TeO6 and observe two successive magnetic transitions…

Materials Science · Physics 2015-12-01 L. Zhao , Z. Hu , C. Y. Kuo , T. -W. Pi , M. -K. Wu , L. H. Tjeng , A. C. Komarek