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Using first-principles density functional theory calculations, we find a strong position and thickness dependence of the formation energy of oxygen vacancies in LaAlO3|SrTiO3 (LAO|STO) multilayers and interpret this with an analytical…

Materials Science · Physics 2010-11-01 Zhicheng Zhong , P. X. Xu , Paul J. Kelly

Quantum confinement at complex oxide interfaces establishes an intricate hierarchy of the strongly correlated $d$-orbitals which is widely recognized as a source of emergent physics. The most prominent example is the (001)…

Strongly Correlated Electrons · Physics 2019-05-15 A. M. R. V. L. Monteiro , M. Vivek , D. J. Groenendijk , P. Bruneel , I. Leermakers , U. Zeitler , M. Gabay , A. D. Caviglia

Ultra-thin tri-color (tri-layer) titanate superlattices ([3u.c. LaTiO3/2u.c. SrTiO3/3u.c. YTiO3], u.c. = unit cells) were grown in a layer-by-layer way on single crystal TbScO3 (110) substrates by pulsed laser deposition. High sample…

Strongly Correlated Electrons · Physics 2013-12-11 M. Kareev , Yanwei Cao , Xiaoran Liu , S. Middey , D. Meyers , J. Chakhalian

Novel phenomena appear when two different oxide materials are combined together to form an interface. For example, at the interface of LaAlO3/SrTiO3, two dimensional conductive states form to avoid the polar discontinuity and magnetic…

Materials Science · Physics 2017-02-23 Fang Wang , Zhaohui Ren , He Tian , Shengyuan A. Yang , Yanwu Xie , Yunhao Lu , Jianzhong Jiang , Gaorong Han , Kesong Yang

We have studied the electronic properties of the 2D electron liquid present at the LaAlO$_3$/SrTiO$_3$ interface in series of samples prepared at different growth temperatures. We observe that interfaces fabricated at 650{\deg}C exhibit the…

Materials Science · Physics 2015-03-20 A. Fête , C. Cancellieri , D. Li , D. Stornaiuolo , A. D. Caviglia , S. Gariglio , J. -M. Triscone

Transition metal oxides display a great variety of quantum electronic behaviours where correlations often play an important role. The achievement of high quality epitaxial interfaces involving such materials gives a unique opportunity to…

Understanding the nature of electrical conductivity, superconductivity and magnetism between layers of oxides is of immense importance for the design of electronic devices employing oxide heterostructures. We demonstrate that resonant…

We report on the fabrication of all perovskite Mott insulator/band insulator YTiO3/CaTiO3 superlattices by pulsed laser deposition. The combination of in situ reflection high energy electron diffraction, X-ray diffraction, and X-ray…

Strongly Correlated Electrons · Physics 2015-11-25 Xiaoran Liu , D. Choudhury , Yanwei Cao , M. Kareev , S. Middey , J. Chakhalian

A superconducting phase with an extremely low carrier density of the order of 10^13 cm^-2 is present at LaAlO3-SrTiO3 interfaces. If depleted from charge carriers by means of a gate field, this superconducting phase undergoes a transition…

Superconductivity · Physics 2016-02-17 E. Fillis-Tsirakis , C. Richter , J. Mannhart , H. Boschker

Polar discontinuities occurring at interfaces between two different materials constitute both a challenge and an opportunity in the study and application of a variety of devices. In order to cure the large electric field occurring in such…

The electronic reconstruction at the interface between two insulating oxides can give rise to a highly-conductive interface. In analogy to this remarkable interface-induced conductivity we show how, additionally, magnetism can be induced at…

Strongly Correlated Electrons · Physics 2007-06-13 A. Brinkman , M. Huijben , M. van Zalk , J. Huijben , U. Zeitler , J. C. Maan , W. G. van der Wiel , G. Rijnders , D. H. A. Blank , H. Hilgenkamp

Herein, we reported giant tunability of the physical properties of 2DEGs at the spinel/perovskite interface of {\gamma}-Al2O3/SrTiO3 (GAO/STO). By modulating the carrier density thus the band filling with ionic-liquid gating, the system…

In pursuit of creating cuprate-like electronic and orbital structures, artificial heterostructures based on LaNiO$_3$ have inspired a wealth of exciting experimental and theoretical results. However, to date there is a very limited…

Strongly Correlated Electrons · Physics 2016-02-17 Yanwei Cao , Xiaoran Liu , M. Kareev , D. Choudhury , S. Middey , D. Meyers , J. -W. Kim , P. Ryan , J. W. Freeland , J. Chakhalian

We present a multi-band model for superconductivity at the metallic interface between insulating oxides LaAlO$_3$ and SrTiO$_3$ (001). Using a self-consistent Bogoliubov-de Gennes theory, formulated with the realistic bands at the…

Superconductivity · Physics 2015-12-09 N. Mohanta , A. Taraphder

Surfaces and interfaces offer new possibilities for tailoring the many-body interactions that dominate the electrical and thermal properties of transition metal oxides. Here, we use the prototypical two-dimensional electron liquid (2DEL) at…

Recent reports of superconductivity at KTaO3 (KTO) (110) and (111) interfaces have sparked intense interest due to the relatively high critical temperature as well as other properties that distinguish this system from the more extensively…

Mesoscale and Nanoscale Physics · Physics 2022-10-26 Muqing Yu , Changjiang Liu , Dengyu Yang , Xi Yan , Qianheng Du , Dillon D. Fong , Anand Bhattacharya , Patrick Irvin , Jeremy Levy

Polar crystals composed of charged ionic planes cannot exist in nature without acquiring surface changes to balance an ever-growing dipole. The necessary changes can manifest structurally or electronically. An electronic asymetry has long…

The question of stability against diffusional mixing at the prototypical LaAlO3/SrTiO3(001) interface is explored using a multi-faceted experimental and theoretical approach. We combine analytical methods with a range of sensitivities to…

The introduction of manganite buffer layers, La7/8Sr1/8MnO3 (LSMO) in particular, at the metallic interface between SrTiO3 (STO) and another band insulator suppresses the carrier density of the interfacial two-dimensional electron gas…

Materials Science · Physics 2017-10-24 Y. Z. Chen , M. Döbeli , E. Pomjakushina , Y. L. Gan , N. Pryds , T. Lippert

Novel low dimensional quantum phenomena are expected at (110) LaAlO3/SrTiO3 (LAO/STO) interfaces after the quasi two dimensional electron gas similar to that of (001) LAO/STO interfaces was found [G. Herranz et al., Sci. Rep. 2, 758 (2012)…

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