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Coherent phonons in single wall carbon nanotubes (SWNTs) are observed as oscillations of the differential absorption coefficient as a function of time by means of pump-probe spectroscopy. For the radial breathing mode (RBM) of a SWNT, the…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 A. R. T. Nugraha , E. H. Hasdeo , G. D. Sanders , C. J. Stanton , R. Saito

We review recent studies of coherent phonons (CPs) corresponding to the radial breathing mode (RBM) and G-mode in single-wall carbon nanotubes (SWCNTs) and graphene. Because of the bandgap-diameter relationship, RBM-CPs cause bandgap…

Mesoscale and Nanoscale Physics · Physics 2013-03-28 J. -H. Kim , A. R. T. Nugraha , L. G. Booshehri , E. H. Hároz , K. Sato , G. D. Sanders , K. -J. Yee , Y. -S. Lim , C. J. Stanton , R. Saito , J. Kono

We have used a femtosecond pump-probe impulsive Raman technique to explore the polarization dependence of coherent optical phonons in highly-purified and aligned semiconducting single-wall carbon nanotubes (SWCNTs). Coherent phonon spectra…

Mesoscale and Nanoscale Physics · Physics 2013-06-11 Yuki Honda , Elizabeth Maret , Atsushi Hirano , Takeshi Tanaka , Kotaro Makino , Muneaki Hase

Using femtosecond pump-probe spectroscopy with pulse shaping techniques, one can generate and detect coherent phonons in chirality-specific semiconducting single-walled carbon nanotubes. The signals are resonantly enhanced when the pump…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 G. D. Sanders , C. J. Stanton , J. -H. Kim , K. -J. Yee , Y. -S. Lim , E. H. Haroz , L. G. Booshehri , J. Kono , R. Saito

We have observed large-amplitude coherent phonon oscillations of radial breathing modes (RBMs) in single-walled carbon nanotubes excited through the lowest-energy (E11) interband transitions. In contrast to the previously-studied coherent…

Mesoscale and Nanoscale Physics · Physics 2010-08-11 Y. -S. Lim , J. -G. Ahn , J. -H. Kim , K. -J. Yee , T. Joo , S. -H. Baik , E. H. Haroz , L. G. Booshehri , J. Kono

We have used a femtosecond pump-probe impulsive Raman technique to explore the ultrafast dynamics of micelle suspended single walled carbon nanotubes (SWNTs) in various pH environments. The structures of coherent phonon spectra of the…

Mesoscale and Nanoscale Physics · Physics 2010-11-17 Kotaro Makino , Atsushi Hirano , Kentaro Shiraki , Yutaka Maeda , Muneaki Hase

The Raman spectra of two G-bands and a radial breathing mode (RBM) of unfilled and filled single-wall semiconducting and metallic carbon nanotubes have been investigated theoretically, in the presence of electron-phonon and phonon-phonon…

Other Condensed Matter · Physics 2009-11-13 S. Gayen , S. N. Behera , S. M. Bose

We have studied the coherent dynamics of G-band phonons in single-walled carbon nanotubes through impulsive stimulated Stokes and anti-Stokes Raman scattering. The probe energy dependence of phonon amplitude as well as preferential…

Mesoscale and Nanoscale Physics · Physics 2012-11-13 J. -H. Kim , K. -J. Yee , Y. -S. Lim , L. G. Booshehri , E. H. Haroz , J. Kono

The radial-breathing-like phonon modes (RBLMs) of the double-walled carbon nanotubes are studied in a simple analytical model, in which the interaction force constants (FCs) can be obtained analytically from the continuous model. The RBLMs…

Mesoscale and Nanoscale Physics · Physics 2007-07-31 Gang Wu , Jian Zhou , Jinming Dong

We have investigated the polarization dependence of the generation and detection of radial breathing mode (RBM) coherent phonons (CP) in highly-aligned single-walled carbon nanotubes. Using polarization-dependent pump-probe…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 L. G. Booshehri , C. L. Pint , G. D. Sanders , L. Ren , C. Sun , E. H. Haroz , J. -H. Kim , K. -J. Yee , Y. -S. Lim , R. H. Hauge , C. J. Stanton , J. Kono

The motion of atoms is at the heart of any chemical or structural transformation in molecules and materials. Upon activation of this motion by an external source, several (usually many) vibrational modes can be coherently coupled, thus…

In terms of lattice dynamics theory, we study the vibrational properties of the oxygen-functionalized single wall carbon nanotubes (O-SWCNs). Due to the C-O and O-O interactions, many degenerate phonon modes are split and even some new…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Z. X. Guo , J. W. Ding , Y. Xiao , D. Y. Xing

Selective enhancement of coherent optical phonons in Bi-Sb mixed crystals has been performed using terahertz (THz) rate pulse trains generated by spatial phase modulation of femtosecond pulse with a liquid-crystal spatial light modulator.…

Materials Science · Physics 2010-11-17 Muneaki Hase , Tetsuya Itano , Kohji Mizoguchi , Shin-ichi Nakashima

A mass and spring model is used to calculate the phonon mode dispersion for single wall carbon nanotubes (SWNTs) of arbitrary chirality. The calculated dispersions are used to determine the chirality dependence of the radial breathing…

Other Condensed Matter · Physics 2007-05-23 A. N. Vamivakas , Y. Yin , A. G. Walsh , M. S. Unlu , B. B. Goldberg , A. K. Swan

Using the first principles calculations we have studied the vibrational modes and Raman spectra of a (10, 10) single-walled carbon nanotube (SWNT) bundle under hydrostatic pressure. Detailed analysis shows that the original radial breathing…

Mesoscale and Nanoscale Physics · Physics 2007-07-31 Gang Wu , Xiaoping Yang , Jinming Dong

The phonon modes at finite temperature in graphene and single-walled carbon nanotubes (SWCNT) are investigated by the mode projection technique combined with molecular dynamics simulation. It is found that the quadratic phonon spectrum of…

Materials Science · Physics 2011-08-31 Jin-Wu Jiang , Jian-Sheng Wang

Using a macroscopic ensemble of highly-enriched (6,5) single-wall carbon nanotubes, combined with high signal-to-noise ratio, time-dependent differential transmission spectroscopy, we have generated vibrational modes in an ultrawide…

We study the optical properties of a single, semiconducting single-walled carbon nanotube (CNT) that is partially suspended across a trench and partially supported by a SiO2-substrate. By tuning the laser excitation energy across the E33…

We use the energy analysis as a perturbative method to study the effect of electron-radial breathing mode (RBM) phonon interaction on the electrical conductivity of long metallic zigzag carbon nanotubes (CNTs). The band structure of zigzag…

Mesoscale and Nanoscale Physics · Physics 2018-05-29 Reyhaneh Taj , Afshin Namiranian

We have developed a microscopic theory for the generation and detection of coherent phonons in armchair and zigzag carbon nanoribbons using an extended tight-binding model for the electronic states and a valence force field model for the…

Mesoscale and Nanoscale Physics · Physics 2012-05-03 G. D. Sanders , A. R. T. Nugraha , R. Saito , C. J. Stanton
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