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Achieving long-range ferrimagnetic order in purely organic systems remains a major challenge in molecular magnetism. Here we report the synthesis and characterization of heterospin-coupling motifs, formed by covalently linking spin-1/2 and…

Mesoscale and Nanoscale Physics · Physics 2026-04-10 Elia Turco , Fupeng Wu , Annika Bernhardt , Nils Krane , Ji Ma , Roman Fasel , Michal Juriček , Xinliang Feng , Pascal Ruffieux

The problem of interacting electrons moving under the influence of a strong magnetic field in two dimensions on a finite disk is reconsidered. First, the results of exact diagonalizations for up to $N=9$ electrons for Coulomb as well as for…

Condensed Matter · Physics 2009-10-22 M. Kasner , W. Apel

Nanomagnets form the building blocks for a gamut of miniaturized energy-efficient devices including data storage, memory, wave-based computing, sensors and biomedical devices. They also offer a span of exotic phenomena and stern challenges.…

Mesoscale and Nanoscale Physics · Physics 2020-12-02 Anjan Barman , Sucheta Mondal , Sourav Sahoo , Anulekha De

The computation of strongly correlated quantum systems is challenging because of its potentially exponential scaling in the number of electron configurations. Variational calculation of the two-electron reduced density matrix (2-RDM)…

Quantum Physics · Physics 2021-04-01 David A. Mazziotti

The calculation of interaction integrals is a bottleneck for the treatment of many-body quantum systems due to its high numerical cost. We conduct configuration interaction calculations of the few-electron states confined in III-V…

Computational Physics · Physics 2020-08-13 Alina Mreńca-Kolasińska , Krzysztof Kolasiński , Bartłomiej Szafran

The ground state structure of few-electron concentric double quantum rings is investigated within the local spin density approximation. Signatures of inter-ring coupling in the addition energy spectrum are identified and discussed. We show…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. I. Climente , J. Planelles , M. Barranco , F. Malet , M. Pi

We present a theoretical approach to determine the electronic properties of nanoscale systems exhibiting strong electron-electron and electron-phonon interactions and coupled to metallic electrodes. This approach is based on an…

Strongly Correlated Electrons · Physics 2009-11-13 A. Martin-Rodero , A. Levy Yeyati , F Flores , R. C. Monreal

We study the formation of molecular states in a two-electron quantum dot as a function of the barrier potential dividing the dot. The increasing barrier potential drives the two electron system from an artificial helium atom to an…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. Dybalski , P. Hawrylak

Laterally localized electronic states are identified on a single layer of graphene on ruthenium. The individual states are separated by 3 nm and comprise regions of about 90 carbon atoms. This constitutes a quantum dot array, evidenced by…

Materials Science · Physics 2010-07-08 H. G. Zhang , H. Hu , Y. Pan , J. H. Mao , M. Gao , H. M. Guo , S. X. Du , T. Greber , H. -J. Gao

Understanding how the orbital motion of electrons is coupled to the spin degree of freedom in nanoscale systems is central for applications in spin-based electronics and quantum computation. We demonstrate this coupling of spin and orbit in…

The exact study of small systems can guide us toward measures for extracting information about many-body physics as we move to more complex systems capable of quantum information processing or quantum analog simulation. We use exact…

Mesoscale and Nanoscale Physics · Physics 2021-06-10 Emily Townsend , Tomáš Neuman , Alex Debrecht , Javier Aizpurua , Garnett W. Bryant

We review recent theoretical developments about the role of spins, electron-electron interactions, and spin-orbit coupling in metal nanoparticles and semiconductor quantum dots. For a closed system, in the absence of spin-orbit coupling or…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yuval Oreg , P. W. Brouwer , X. Waintal , Bertrand I. Halperin

Two-electron states bound to donors in silicon are important for both two qubit gates and spin readout. We present a full configuration interaction technique in the atomistic tight-binding basis to capture multi-electron exchange and…

We discuss advantages and limitations of the spin noise spectroscopy for characterization of interacting quantum dot systems on specific examples of individual singly and doubly charged quantum dot molecules (QDMs). It is shown that all the…

Mesoscale and Nanoscale Physics · Physics 2013-07-29 Dibyendu Roy , Yan Li , Alex Greilich , Yuriy V. Pershin , Avadh Saxena , Nikolai A. Sinitsyn

We study a system in which electrons in a two-dimensional electron gas are confined by a nonhomogeneous nuclear spin polarization. The system consists of a heterostructure that has non-zero nuclei spins. We show that in this system…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yu. V. Pershin

By measuring electron tunneling between a ferromagnet and individual energy levels in an aluminum quantum dot, we show how spin-resolved quantum states can be used as filters to determine spin-dependent tunneling rates. We also observe…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Mandar M. Deshmukh , D. C. Ralph

We study the superradiance dynamics in a dense system of atoms each of which can be generally a spin-$j$ particle with $j$ an arbitrary half-integer. We generalize Dicke's superradiance point of view to multiple-level systems, and compare…

Quantum Physics · Physics 2012-05-28 G. -D. Lin , S. F. Yelin

Spin properties of two interacting electrons in a quantum dot (QD) embedded in a nanowire with controlled aspect ratio and longitudinal magnetic fields are investigated by using a configuration interaction (CI) method and exact…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Yan-Ting Chen , Shun-Jen Cheng , Chi-Shung Tang

We show here the existence of the indirect coupling of electron and magnetic or nuclear ion spins in self-assembled quantum dots mediated by electron-electron interactions. With a single localized spin placed in the center of the dot, only…

Mesoscale and Nanoscale Physics · Physics 2016-11-25 Udson C. Mendes , Marek Korkusinski , Pawel Hawrylak

Nanoscale quantum dots in microwave cavities can be used as a laboratory for exploring electron-electron interactions and their spin in the presence of quantized light and a magnetic field. We show how a simple theoretical model of this…

Mesoscale and Nanoscale Physics · Physics 2023-11-16 S. S. Beltrán-Romero , F. J. Rodríguez , L. Quiroga , N. F. Johnson