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The interaction between carbon nanostructures like quantum dots and radiation can generate different effects inside the nanomaterial, with the use of computational methods such effects can be predicted and optimize the material allowing a…

Mesoscale and Nanoscale Physics · Physics 2022-05-10 Alexander Leon , Juan E. Gomez , Freddy R. Perez

This paper derives and demonstrates a new, purely density-based ab initio approach for calculation of the energies and properties of many-electron systems. It is based upon the discovery of relationships that govern the "mechanics" of the…

Chemical Physics · Physics 2024-09-04 James C. Ellenbogen

Once the periodic properties of elements were unveiled, chemical bonds could be understood in terms of the valence of atoms. Ideally, this rationale would extend to quantum dots, often termed artificial atoms, and quantum computation could…

The significant electron-electron interactions that characterize the {\pi}-electrons of graphene nanoribbons (GNRs) necessitate going beyond one-electron tight-binding description. Existing theories of electron-electron interactions in GNRs…

Strongly Correlated Electrons · Physics 2016-07-27 V. M. L. Durga Prasad Goli , Suryoday Prodhan , Sumit Mazumdar , S. Ramasesha

We review recent theoretical and experimental advances toward understanding the effects of nuclear spins in confined nanostructures. These systems, which include quantum dots, defect centers, and molecular magnets, are particularly…

Mesoscale and Nanoscale Physics · Physics 2009-09-15 W. A. Coish , J. Baugh

Nanowire double quantum dots occupied by an even number of electrons are investigated in the context of energy level structure revealed by electric dipole spin resonance measurements. We use numerically exact configuration interaction…

Mesoscale and Nanoscale Physics · Physics 2015-03-05 M. P. Nowak , B. Szafran

Graphene nanoribbons (GNRs) are one-dimensional nanostructures predicted to display a rich variety of electronic behaviors. Depending on their structure, GNRs realize metallic and semiconducting electronic structures with band gaps that can…

Mesoscale and Nanoscale Physics · Physics 2013-10-16 Oleg V. Yazyev

The one-- and two-- particle densities of up to four interacting electrons with spin, confined within a quasi one--dimensional ``quantum dot'' are calculated by numerical diagonalization. The transition from a dense homogeneous charge…

Condensed Matter · Physics 2009-10-22 K. Jauregui , W. Haeusler , B. Kramer , PTB Braunschweig

Multi-dimensional direct numerical simulation (DNS) of the Schr\"odinger equation is needed for design and analysis of quantum nanostructures that offer numerous applications in biology, medicine, materials, electronic/photonic devices,…

Computational Engineering, Finance, and Science · Computer Science 2023-04-25 Martin Veresko , Ming-Cheng Cheng

The low-lying eigenstates of a system of two electrons confined within a two-dimensional quantum dot with a hard polygonal boundary are obtained by means of exact diagonalization. The transition from a weakly correlated charge distribution…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 C E Creffield , Wolfgang Haeusler , J H Jefferson , Sarben Sarkar

The quantum molecule consisting of three quantum dots that forms a triangle with its centers is studied. The electron wave function in the nanosystem is written using the linear combination of orbital quantum wells. The dispersion equation…

Mesoscale and Nanoscale Physics · Physics 2020-03-05 I. V. Bilynskyi , V. B. Hols'kyi , R. Ya. Leshko

In this perspective, the various measures of electron correlation used in wavefunction theory, density functional theory and quantum information theory are briefly reviewed. We then focus on a more traditional metric based on dominant…

Chemical Physics · Physics 2023-04-07 Róbert Izsák , Aleksei V Ivanov , Nick S. Blunt , Nicole Holzmann , Frank Neese

Quantum dots are nanoscopic systems, where carriers are confined in all three spatial directions. Such nanoscopic systems are suitable for fundamental studies of quantum mechanics and are candidates for applications such as quantum…

Mesoscale and Nanoscale Physics · Physics 2016-03-16 Bahareh Goldozian , Fikeraddis A. Damtie , Gediminas Kiršanskas , Andreas Wacker

This document provides detailed descriptions of data acquisition and data analysis in support of the accompanying Article, cond-mat/0610721: Observation of the two-channel Kondo effect. Some of the most intriguing problems in solid state…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 R. M. Potok , I. G. Rau , Hadas Shtrikman , Yuval Oreg , D. Goldhaber-Gordon

The exponential computational cost of describing strongly correlated electrons can be mitigated by adopting a reduced density-matrix (RDM)-based description of the electronic structure. While variational two-electron RDM (v2RDM) methods can…

Chemical Physics · Physics 2026-01-06 Grier M. Jones , Run. R. Li , A. Eugene DePrince , Konstantinos D. Vogiatzis

Properly regularized second-order degenerate perturbation theory is applied to compute the contribution of higher Landau levels to the low-energy spectrum of interacting electrons in a disk-shaped quantum dot. At ``filling factor'' near…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Augusto Gonzalez , Juan David Serna , Roberto Capote , Guillermo Avendaño

The self consistent version of the density functional theory (DFT) is presented, which allows to calculate the ground state and dynamic properties of finite multi-electron systems such as atoms, molecules and clusters. The exact functional…

Condensed Matter · Physics 2007-05-23 M. Ya. Amusia , V. R. Shaginyan

We analyze a model problem representing a multi-electronic molecule sitting on a metal surface. Working with a reduced configuration interaction Hamiltonian, we show that one can extract very accurate ground state wavefunctions as compared…

Chemical Physics · Physics 2020-09-24 Junhan Chen , Zuxin Jin , Wenjie Dou , Joseph Subotnik

We consider a quantum dot embedded in a three-dimensional nanowire with tunable aspect ratio a. A configuration interaction theory is developed to calculate the energy spectra of the finite 1D quantum dot systems charged with two electrons…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Y. T. Chen , C. C. Chao , S. Y. Huang , C. S. Tang , S. J. Cheng

The electronic properties of semiconductor, vertical, double quantum dot systems with few electrons are investigated by means of analytic, configuration-interaction, and mean-field methods. The combined effect of a high magnetic field,…

Condensed Matter · Physics 2009-10-22 Juan Jose Palacios , Pawel Hawrylak