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The vibrational properties of ferrimagnetic $\mathrm{Mn_3Si_{2}Te_6}$ single crystals are investigated using Raman spectroscopy and density functional theory calculations. Eighteen Raman-active modes are identified, fourteen of which are…

Intrinsic, two-dimensional (2D) ferromagnetic semiconductors are an important class of materials for spin-charge conversion applications. Cr$_2$Ge$_2$Te$_6$ retains long-range magnetic order in bilayer at cryogenic temperatures and shows…

The presence of spin-polarized charge carriers in metallic magnets provides a mechanism for spin-lattice interactions mediated by electron-phonon coupling. Here, we present a theory of this mechanism used to estimate its effect on the…

Materials Science · Physics 2024-08-20 Danis I. Badrtdinov , Mikhail I. Katsnelson , Alexander N. Rudenko

In Eu2ZnIrO6, effectively two atoms are active i.e. Ir is magnetically active, which results in complex magnetic ordering within the Ir sublattice at low temperature. On the other hand, although Eu is a van-vleck paramagnet, it is active in…

Strongly Correlated Electrons · Physics 2020-11-05 Birender Singh , M. Vogl , S. Wurmehl , S. Aswartham , B. Büchner , Pradeep Kumar

Electronic structure near Fermi level of Pr2CoFeO6 (at 300 K) was investigated by X-ray photoemission spectroscopy (XPS) technique. All three cations, i.e., Pr, Co and Fe were found to be trivalent in nature. XPS analysis also suggested the…

Strongly Correlated Electrons · Physics 2019-05-22 Arkadeb Pal , Surajit Ghosh , Amish G. Joshi , P. K. Gupta , P. Prakash , Amitabh Das , A. K. Ghosh , Sandip Chatterjee

We determine the nature of coupled phonons and magnetic excitations in AlFeO3 using inelastic light scattering from 5 K to 315 K covering a spectral range from 100-2200 cm-1 and complementary first-principles density functional theory-based…

Strongly Correlated Electrons · Physics 2012-05-01 Pradeep Kumar , A. Bera , D. V. S. Muthu , S. N. Shirodkar , R. Saha , A. Shireen , A. Sundaresan , U. V. Waghmare , A. K. Sood , C. N. R. Rao

We perform systematic first-principles calculations to investigate the spin-phonon coupling (SPC) of Cr2Ge2Te6 (CGT) monolayer (ML). It is found that the Eg phonon mode at 211.8 cm^{-1} may have a SPC as large as 3.19 cm^{-1}, as it…

Materials Science · Physics 2020-01-08 B. H. Zhang , Y. S. Hou , Z. Wang , R. Q. Wu

The polycrystalline co-doped samples of Sm0.5Y0.5Fe0.58Mn0.42O3 were prepared by solid-state reaction route and its various physical properties with their correlations have been investigated. The dc magnetization measurements on the sample…

The interplay between lattice distortions, magnetism, and spin-orbit coupling in 5d transition-metal halides offers a fertile platform for exploring correlated spin-lattice dynamics. Here, we investigate the impact of structural symmetry…

Strongly Correlated Electrons · Physics 2026-01-30 S. Bhatia , A. Ahmad , M. Zeeshan , S. Kaur , J. K. Anand , A. Goswami , B. K. Mani , K. Sen

We studied the optical properties of antiferromagnetic ZnCr2Se4 by infrared spectroscopy up to 28,000 cm-1 and for temperatures from 5 to 295 K. At the magnetic phase transition at 21 K, one of the four phonon modes reveals a clear…

Strongly Correlated Electrons · Physics 2009-04-01 T. Rudolf , Ch. Kant , F. Mayr , M. Schmidt , V. Tsurkan , J. Deisenhofer , A. Loidl

We investigate the interplay between lattice symmetry, phonons, and magnetism in the quasi-one-dimensional ladder compound BaFe$_2$S$_3$ by combining polarized synchrotron infrared spectroscopy, hybrid-functional density functional theory…

Strongly Correlated Electrons · Physics 2026-03-20 Y. Oubaid , S. Deng , NS. Dhami , M. Verseils , D. Bounoua , A. Forget , D. Colson , P. Foury-Leylekian , M. B. Lepetit , V. Balédent

The attempt to understand cuprate superconductors is complicated by the presence of multiple strong interactions. While many believe that antiferromagnetism is important for the superconductivity, there has been revived interest in the role…

Superconductivity · Physics 2009-11-11 D. Reznik , L. Pintschovius , M. Ito , S. Iikubo , M. Sato , H. Goka , M. Fujita , K. Yamada , G. D. Gu , J. M. Tranquada

We used polarization-resolved Raman scattering to study the magneto-elastic coupling in the parent compounds of several families of Fe-based superconductors (BaFe2As2, EuFe2As2, NaFeAs, LiFeAs, FeSe and LaFeAsO). We observe an emergent…

Low-dimensional frustrated magnetic square networks feature a variety of unconventional phases with novel emergent excitations. Often these excitations are intertwined and manifest into intriguing phenomena, an area that has remained…

Materials Science · Physics 2024-01-10 Shalini Badola , Aprajita Joshi , Akriti Singh , Surajit Saha

We investigated the magnetic and magnetoelastic properties of MnSc$_2$Se$_4$ single crystals at low temperature under a magnetic field directed along the crystallographic [111] axis. The magnetization data at low temperature show a linear…

Strongly Correlated Electrons · Physics 2024-10-29 J. Sourd , Y. Skourski , L. Prodan , V. Tsurkan , A. Miyata , J. Wosnitza , S. Zherlitsyn

We report measurements of the temperature dependence of phonon densities of states in K0.8Fe1.6Se2 using inelastic neutron scattering technique. While cooling down to 150 K, a phonon peak splitting around 25 meV is observed and a new peak…

Superconductivity · Physics 2015-06-12 R. Mittal , M. K. Gupta , S. L. Chaplot , M. Zbiri , S. Rols , H. Schober , Y. Su , Th. Brueckel , T. Wolf

Multiple structure and symmetry types and their transformations are discovered in quasi-two-dimensional (quasi-2D) Cr2Ge2Te6 crystal in surprisingly very narrow temperature range of 2 K and magnetic field range of 0.07 T using a homebuilt…

Materials Science · Physics 2018-03-22 Tengfei Guo , Zongwei Ma , Gaoting Lin , Xuan Luo , Yubin Hou , Yuping Sun , Zhigao Sheng , Qingyou Lu

The temperature dependence of eigenfrequencies and intensities of the IR active modes has been investigated for the antiferromagnetic chromium spinel compounds CdCr2O4, ZnCr2O4, ZnCr2S4, ZnCr2Se4, and HgCr2S4 by IR spectroscopy for…

Strongly Correlated Electrons · Physics 2007-07-05 T. Rudolf , Ch. Kant , F. Mayr , J. Hemberger , V. Tsurkan , A. Loidl

The coupling between antiferromagnetic spins and infrared-active phonons in solids is responsible for many intriguing phenomena and is a field of intense research with extensive potential applications in the modern devices based on…

While 3$d$-containing materials display strong electron correlations, narrow band widths, and robust magnetism, 5$d$ systems are recognized for strong spin-orbit coupling, increased hybridization, and more diffuse orbitals. Combining these…