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We study strong-field double ionization in a three-electron atom by applying a simplified, reduced-dimensionality model with three active electrons. The influence of the spin-induced symmetry of the spatial part of the wavefunction on the…

Diatomic molecules (e.g., O$_2$) in intense laser field exhibit a peculiar suppressed ionization behavior compared to their companion atoms. Several physical models have been proposed to account for this suppression while no consensus has…

Atomic Physics · Physics 2011-11-15 Z. Lin , X. Y. Jia , C. Wang , Z. Hu , H. Kang , W. Quan , X. Y. Lai , X. Liu , J. Chen , B. Zeng , W. Chu , J. P. Yao , Y. Cheng , Z. Z. Xu

This paper concerns the theory of non-recollisional ionization or detachment of atoms or ions by intense few-cycle pulses. It is shown that in certain conditions of pulse duration, peak intensity and carrier-envelope phase, the ionization…

Atomic Physics · Physics 2014-09-04 C. C. Chirila , R. M. Potvliege

We present a theory illuminating the cross-over from strong-field tunnelling ionization to weak-field multiphoton ionization in the interaction of a classical laser field with a hydrogen atom. A simple formula is derived in which the…

Atomic Physics · Physics 2016-11-23 Michael Klaiber , John S Briggs

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…

Based on a combined quantum-classical treatment, a complete study of the strong field dynamics of H2+, i.e. including all nuclear and electronic DOF as well as dissociation and ionization, is presented. We find that the ro-vibrational…

Atomic and Molecular Clusters · Physics 2011-08-09 J. Handt , S. M. Krause , J. M. Rost , M. Fischer , F. Grossmann , R. Schmidt

The tunneling splitting in biaxial ferrimagnetic particles at excited states with an explicit calculation of the prefactor of exponent is obtained in terms of periodic instantons which are responsible for tunneling at excited states and is…

Condensed Matter · Physics 2019-08-17 Yi-Hang Nie , Yan-Hong Jin , J. -Q Liang , F. -C Pu

Triple-differential cross sections for two-photon double ionization of molecular hydrogen are presented for a central photon energy of 30 eV. The calculations are based on a fully {\it ab initio}, nonperturbative, approach to the…

Atomic Physics · Physics 2016-11-17 Xiaoxu Guan , Klaus Bartschat , Barry I. Schneider

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

Two-photon free-free transitions in elastic laser-assisted electron-hydrogen collisions are studied in the domain of high scattering energies and low or moderate field intensities, in the third order of perturbation theory, taking into…

Atomic Physics · Physics 2013-03-07 Aurelia Cionga , Gabriela Buica

In this work we report ab initio calculations for the $H_2^+$ molecule interacting with ultrashort intense laser pulses. We analyse several observables that can, in principle, be available experimentally, in order to get a deeper…

Atomic Physics · Physics 2017-05-25 R. E. F. Silva

The alignment- and internuclear-distance dependent ionization of H$_2$ exposed to intense, ultrashort laser fields is studied by solving the time-dependent two-electron Schr\"odinger equation. In the regime of perturbative few-photon…

Atomic Physics · Physics 2015-06-23 Johann Förster , Yulian V. Vanne , Alejandro Saenz

We observed electromagnetically induced transparency (EIT) and dark fluorescence in a cascade three-level diatomic Lithium system using Optical-Optical Double Resonance (OODR) spectroscopy. When a strong coupling laser couples the…

Quantum Physics · Physics 2009-11-11 Jianbing Qi , A. Marjatta Lyyra

We have investigated the structural dynamics in photoexcited 1,2-diiodotetrafluoroethane molecules (C2F4I2) in the gas phase experimentally using ultrafast electron diffraction and theoretically using FOMO-CASCI excited state dynamics…

A single-atom 'double-slit' experiment is realized by photo-ionizing Rubidium atoms using two independent low power lasers. The photoelectron wave of well-defined energy recedes to the continuum either from the 5P or 6P states in the same…

Atomic Physics · Physics 2019-01-17 James Pursehouse , Andrew James Murray , Jonas Wätzel , Jamal Berakdar

We investigate the resonance-enhanced few-photon ionization of atomic lithium by linearly polarized light whose frequency is tuned near the 2s-2p transition. Considering the direction of light polarization orthogonal to the quantization…

With a semiclassical quasi-static model we achieve an insight into the complex dynamics of two correlated electrons under the combined influence of a two-center Coulomb potential and an intense laser field. The model calculation is able to…

Atomic and Molecular Clusters · Physics 2009-11-13 J. Liu , D. F. Ye , J. Chen , X. liu

We theoretically study multiphoton ionization of Mg in the circularly as well as the linearly polarized laser fields. Specifically two-, three-, and four-photon ionization cross sections from the ground and first excited states are…

Atomic Physics · Physics 2013-03-07 Gabriela Buica , Takashi Nakajima

We consider tunnel ionization of an atom or molecule in a strong field within an analytical treatment of the R-matrix method, in which an imaginary boundary is set up inside the classically forbidden region that acts as a source of ionized…

Quantum Physics · Physics 2016-11-26 Emilio Pisanty

We review the semiclassical two-step model for strong-field ionization. The semiclassical two-step model describes quantum interference and accounts for the ionic potential beyond the semiclassical perturbation theory. We discuss…

Atomic Physics · Physics 2021-05-05 N. I. Shvetsov-Shilovski