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The physics of excitons, electron-hole pairs that are bound together by their mutual Coulomb attraction, can to great extent be understood in the framework of the quantum-mechanical hydrogen model. This model has recently been challenged by…

Mesoscale and Nanoscale Physics · Physics 2017-09-15 Maxim Trushin , Mark Oliver Goerbig , Wolfgang Belzig

Excitons in Transition Metal Dichalcogenides (TMDs) acquire a spin-like quantum number, a pseudospin, originating from the crystal's discrete rotational symmetry. Here, we break this symmetry using a tunable uniaxial strain, effectively…

Heterostructures of layered transition metal dichalcogenides (TMDs) host long-lived, tunable excitons, making them intriguing candidates for material-based quantum information applications. Light absorption in these systems induces a…

Materials Science · Physics 2023-08-25 Tomer Amit , Sivan Refaely-Abramson

We calculate the binding energy, transition energies, oscillator strength, and absorption coefficient of indirect excitons in transition metal dichalcogenide (TMDC) double layers separated by an integer number of hexagonal boron nitride…

Mesoscale and Nanoscale Physics · Physics 2018-09-19 Matthew N. Brunetti , Oleg L. Berman , Roman Ya. Kezerashvili

In this paper, we study the third-order nonlinear optical response due to transitions between excitonic levels in two-dimensional transition metal dichalcogeniedes. To accomplish this, we use methods not applied to the description of…

Mesoscale and Nanoscale Physics · Physics 2021-06-14 J. C. G. Henriques , Høgni C. Kamban , Thomas G. Pedersen , N. M. R. Peres

Rich valleytronics and diverse defect-induced or interlayer pre-bandgap excitonics have been extensively studied in transition metal dichalcogenides (TMDCs), a system with fascinating optical physics. However, more intense high-energy…

Materials Science · Physics 2021-04-02 Jinhua Hong , Masanori Koshino , Ryosuke Senga , Thomas Pichler , Hua Xu , Kazu Suenaga

When transition-metal dichalcogenide monolayers lack inversion symmetry, their low-energy single particle spectrum can described by tilted massive Dirac Hamiltonians. The so-called Janus materials fall into that category. Inversion symmetry…

Mesoscale and Nanoscale Physics · Physics 2022-09-15 M. F. C. Martins Quintela , A. T. Costa , N. M. R. Peres

We propose a continuum model for the theoretical study of hybridized moir\'e excitons in transition metal dichalcogenides heterobilayers, and we use a variational method to solve the exciton wavefunction and calculate the optical absorption…

Mesoscale and Nanoscale Physics · Physics 2023-10-23 Yao-Wen Chang

In monolayer transition metal dichalcogenides, tightly bound excitons have been discovered with a valley pseudospin that can be optically addressed through polarization selection rules. Here, we show that this valley pseudospin is strongly…

Mesoscale and Nanoscale Physics · Physics 2014-05-20 Hongyi Yu , Guibin Liu , Pu Gong , Xiaodong Xu , Wang Yao

Recent results on the optical properties of mono- and few-layers of semiconducting transition metal dichalcogenides are reviewed. Experimental observations are presented and discussed in the frame of existing models, highlighting the limits…

Mesoscale and Nanoscale Physics · Physics 2017-09-19 M. Koperski , M. R. Molas , A. Arora , K. Nogajewski , A. O. Slobodeniuk , C. Faugeras , M. Potemski

Semiconducting transition metal dichalcogenides (STMDC) are two-dimensional (2D) crystals characterized by electron volt size band gaps, spin-orbit coupling (SOC), and d-orbital character of its valence and conduction bands. We show that…

Mesoscale and Nanoscale Physics · Physics 2014-08-28 A. S. Rodin , A. H. Castro Neto

Optically generated excitons dictate the absorption and emission spectrum of doped semiconductor transition metal dichalcogenide monolayers. We show that upon increasing the electron density, the elementary optical excitations develop a…

Mesoscale and Nanoscale Physics · Physics 2020-05-20 Ovidiu Cotlet , Dominik S. Wild , Mikhail D. Lukin , Atac Imamoglu

Excitons in monolayer transition-metal dichalcogenides (TMDs) have garnered significant attention because of their large binding energies due to weakly screened Coulomb interaction, and direct bandgap at the K/K$^\prime$ point in the…

Starting from the single-particle Dirac Hamiltonian for charge carriers in monolayer transition metal dichalcogenides (TMDs), we construct a four-band Hamiltonian describing interlayer excitons consisting of an electron in one TMD layer and…

Mesoscale and Nanoscale Physics · Physics 2018-09-05 M. Van der Donck , F. M. Peeters

In order to discuss the exciton fine-structure of transition-metal dichalcogenides mono-layers, excitons are first defined in the subspace of electron- and hole states, including the lowest conduction band (LCB) and the uppermost valence…

Mesoscale and Nanoscale Physics · Physics 2019-06-25 Pierre Gilliot , Mathieu Gallart , Bernd Hönerlage

Semiconducting Transition Metal Dichalcogenides (TMDs) have significant nonlinear optical effects. In this work we have used second-harmonic generation (SHG) and the four-wave mixing (FWM) spectroscopy in resonance with the excitons in…

Even the best quality 2D materials have non-negligible concentrations of vacancies and impurities. It is critical to understand and quantify how defects change intrinsic properties, and use this knowledge to generate functionality. This…

Other Condensed Matter · Physics 2020-10-22 Pedro Miguel M. C. de Melo , Zeila Zanolli , Matthieu Jean Verstraete

We present a unified description of the excitonic properties of four monolayer transition-metal dichalcogenides (TMDC's) using an equation of motion method for deriving the Bethe-Salpeter equation in momentum space. Our method is able to…

Mesoscale and Nanoscale Physics · Physics 2017-08-08 A. J. Chaves , R. M. Ribeiro , T. Frederico , N. M. R. Peres

We develop an analytical model to describe sub-bandgap optical absorption in two-dimensional semiconducting transition metal dichalcogenide (s-TMD) nanoflakes. The material system represents an array of few-layer molybdenum disulfide…

Mesoscale and Nanoscale Physics · Physics 2016-10-11 Maxim Trushin , Edmund J. R. Kelleher , Tawfique Hasan

Excitons in van der Waals heterostructures based on atomically thin transition metal dichalcogenides are considered as potential candidates for the formation of a superfluid state in two-dimensional systems. A number of studies reported…

Mesoscale and Nanoscale Physics · Physics 2024-06-27 M. M. Glazov , R. A. Suris
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