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We have performed sub-Doppler spectroscopy on the narrow intercombination line of cold calcium atoms using the amplified output of a femtosecond laser frequency comb. Injection locking of a 657-nm diode laser with a femtosecond comb allows…

Atomic Physics · Physics 2010-03-19 T. M. Fortier , Y. Le Coq , J. E. Stalnaker , D. Ortega , S. A. Diddams , C. W. Oates , L. Hollberg

The frequency combs characterized by their phase-coherent equidistant spectral modes and precise frequency scales of broadband spectrum, have made them an indispensable part of contemporary physics. A terahertz (THz) frequency comb is a key…

We demonstrate fiber mode-locked dual frequency comb spectroscopy for broadband, high resolution measurements in a rapid compression machine (RCM). We apply an apodization technique to improve the short-term signal-to-noise-ratio (SNR),…

Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…

Optics · Physics 2020-06-04 A. V. Muraviev , D. Konnov , K. L. Vodopyanov

Optical frequency comb synthesizers (FCs) [1] are laser sources covering a broad spectral range with a number of discrete, equally spaced and highly coherent frequency components, fully controlled through only two parameters: the frequency…

Dual-comb spectroscopy has emerged as an indispensable analytical technique in applications that require high resolution and broadband coverage within short acquisition times. Its experimental realization, however, remains hampered by…

Instrumentation and Detectors · Physics 2019-12-02 Łukasz A. Sterczewski , Aleksandra Przewłoka , Wawrzyniec Kaszub , Jarosław Sotor

Frequency-modulated (FM) combs based on active cavities like quantum cascade lasers have recently emerged as promising light sources in many spectral regions. Unlike passive modelocking, which uses amplitude modulation to generate amplitude…

Optics · Physics 2024-08-15 Mithun Roy , Zhenyang Xiao , Sadhvikas Addamane , David Burghoff

We demonstrate fast characterization (~1.4 microseconds) of both the dispersion and dispersion slope of long optical fiber links (~25 km) using dual quadrature spectral interferometry with an optical frequency comb. Compared to previous…

Dual-comb spectroscopy utilizes two sets of comb lines with slightly different comb-tooth-spacings, and optical spectral information is acquired by measuring the radio-frequency beat notes between the sets of comb lines. It holds the…

Optics · Physics 2016-09-13 Xin Zhao , Guoqing Hu , Bofeng Zhao , Cui Li , Yingling Pan , Ya Liu , Takeshi Yasui , Zheng Zheng

The frequency noise power spectral density of a free-running quantum cascade laser frequency comb is investigated. A plateau is observed at high frequencies, attributed to the quantum noise limit set by the Schawlow-Townes formula for the…

Optics · Physics 2015-11-18 Francesco Cappelli , Gustavo Villares , Sabine Riedi , Jerome Faist

Optical frequency combs can potentially provide an efficient light source for multi-terabit-per-second optical superchannels. However, as the bandwidth of these multi-wavelength light sources is increased, it can result in low per-line…

Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…

A four-wave-mixing, frequency-comb-based, hyperspectral imaging technique that is spectrally precise, potentially rapid, and can in principle be applied to any material, is demonstrated in a near-diffraction-limited microscopy application.

Optics · Physics 2021-07-21 Brad C. Smith , Bachana Lomsadze , Steven T. Cundiff

We report an approach for high-resolution spectroscopy using a widely tunable laser emitting in the molecular fingerprint region. The laser is based on difference-frequency generation (DFG) in a nonlinear orientation-patterned GaAs crystal.…

We demonstrate the advantages of THz frequency combs for high-resolution spectroscopy. This benefits from wide spectral coverage and the exact knowledge of the frequency position of each comb component. Heterodyne detection combined with a…

Instrumentation and Detectors · Physics 2024-12-03 Francis Hindle , Alexandra Khabbaz , Anthony Roucou , Jean-Francois Lampin , Gaël Mouret

Frequency combs (FCs) -- spectra containing equidistant coherent peaks -- have enabled researchers and engineers to measure the frequencies of complex signals with high precision thereby revolutionising the areas of sensing, metrology and…

Terahertz (THz) frequency combs are increasingly essential for spectroscopy, metrology, and quantum science. However, generating a dense array of evenly spaced ultra-narrow THz comb lines is challenging. Here, we demonstrate broadband THz…

Optics · Physics 2026-02-10 Min Li , Yu Xia , Yuan Chen , Sinan Tao , Mingyang He , Kun Huang , Hua Li , Ming Yan , Heping Zeng

Reducing the pulse repetition rate of an optical frequency comb increases the pulse energy for a given average power. This enhances the efficiency of nonlinear frequency conversion and it facilitates extending the accessible wavelength…

Optical frequency combs paved the way for fast and compact multi-component optical chemical analysis due to their broadband spectra. Dual-comb spectrometers embody this technology, but their design requires a pair of matched combs, adding…

Optics · Physics 2025-09-25 Ina Heckelmann , Davide Pinto , Uwe Schmitt , Mattias Beck , Jérôme Faist

Two techniques that employ equally spaced trains of optical pulses to map an optical high frequency into a low frequency modulation of the signal that can be detected in real time are compared. The development of phase-stable optical…

Quantum Physics · Physics 2017-08-22 Kochise Bennett , Jeremy Rouxel , Shaul Mukamel
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