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Mid-infrared Quantum Cascade Lasers (QCLs) are compact and efficient sources ideal for molecular spectroscopy applications, such as dual-comb spectroscopy. However, despite over a decade of active developments of QCL frequency comb devices,…

Applied Physics · Physics 2022-07-20 Martin Franckie

Chip-scale optical frequency combs can provide broadband spectroscopy for diagnosing complex organic molecules. They are also promising as miniaturized laser spectrometers in applications ranging from atmospheric chemistry to geological…

A fieldable dual-comb spectrometer is described based on a "bootstrapped" frequency referencing scheme in which short-term optical phase coherence between combs is attained by referencing each to a free-running diode laser, whilst high…

We present homogeneous quantum cascade lasers (QCLs) emitting around 3 THz which display bandwidths up to 950 GHz with a single stable beatnote. Devices are spontaneously operating in a harmonic comb state, and when in a dense mode regime…

The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multi-heterodyne spectroscopy. We measure the absorption and phase shift experienced by…

Optics · Physics 2009-11-13 Ian Coddington , William C. Swann , Nathan R. Newbury

Broadband dual-comb spectroscopy has attracted increasing interests due to its unique advantages in high spectral resolution, fast detection, and so on. Although the dual-comb technique is relatively mature in the infrared wavelengths, it…

Precise astronomical spectroscopic analyses routinely assume that individual pixels in charge-coupled devices (CCDs) have uniform sensitivity to photons. Intra-pixel sensitivity (IPS) variations may already cause small systematic errors in,…

Instrumentation and Methods for Astrophysics · Physics 2015-06-04 Michael T. Murphy , Clayton R. Locke , Philip S. Light , Andre N. Luiten , Jon S. Lawrence

Laser frequency combs are coherent light sources that emit a broad spectrum consisting of discrete, evenly spaced narrow lines, each having an absolute frequency measurable within the accuracy of an atomic clock. Their development, a decade…

Optics · Physics 2017-06-13 Albert Schliesser , Nathalie Picqué , Theodor W. Hänsch

We propose a new approach to near-infrared molecular spectroscopy, harnessing advanced concepts of optical telecommunications and supercontinuum photonics. We generate, without mode-locked lasers, two frequency combs of slightly different…

We present a monolithic solution to extract efficiently light from terahertz quantum cascade lasers with metal-metal waveguides suitable for broadband frequency comb applications. The design is optimized for a bandwidth of 500 GHz around a…

The search for earth-like exoplanets with the Doppler radial velocity technique is an extremely challenging and multifaceted precision spectroscopy problem. Currently, one of the limiting instrumental factors in reaching the required…

Cavity-enhanced direct frequency comb spectroscopy combines broad spectral bandwidth, high spectral resolution, precise frequency calibration, and ultrahigh detection sensitivity, all in one experimental platform based on an optical…

Optics · Physics 2009-11-13 Michael J. Thorpe , Jun Ye

In this work, control over the precise state emitted by quantum cascade laser frequency combs through strong radio-frequency current modulation close to their repetition frequency is demonstrated. In particular, broadening of the spectrum…

We demonstrate simple optical frequency combs based on semiconductor quantum well laser diodes. The frequency comb spectrum can be tailored by choice of material properties and quantum-well widths, providing spectral flexibility. Finally,…

Optics · Physics 2020-07-21 Mark Dong , Matthew W. Day , Herbert G. Winful , Steven T. Cundiff

The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…

Quantum cascade lasers are proving to be instrumental in the development of compact frequency comb sources at mid-infrared and terahertz frequencies. Here we demonstrate a heterogeneous terahertz quantum cascade laser with two active…

Multiheterodyne techniques using frequency combs -- light sources whose lines are perfectly evenly-spaced -- have revolutionized optical science. By beating an unknown signal with the many lines of a comb, its spectrum is recovered.…

Optics · Physics 2020-04-23 David Burghoff

We report on the first direct measurement of the emission character of quantum cascade laser based frequency combs, using intensity autocorrelation. The correlation technique is based on fast electro-optic sampling, with a bandwidth…

Instrumentation and Detectors · Physics 2017-09-20 Ileana-Cristina Benea-Chelmus , Markus Rösch , Giacomo Scalari , Mattias Beck , Jérôme Faist

We describe the cavity-enhancement of frequency combs over a wide tuning range of 450-700 nm (> 7900 cm$^{-1}$), covering nearly the entire visible spectrum. Tunable visible frequency combs from a synchronously-pumped optical parametric…

Due to its fast and high resolution characteristics, dual-comb spectroscopy has attracted an increasing amount of interest since its first demonstration. In the terahertz frequency range where abundant absorption lines (finger prints) of…