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Related papers: Angular anisotropy of time delay in XUV/IR photoio…

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We solve the time-dependent Schr\"odinger equation describing a water molecule driven by a superposition of the XUV and IR pulses typical for a RABBITT experiment. This solution is obtained by a combination of the time-dependent coordinate…

Atomic Physics · Physics 2018-01-17 Vladislav V. Serov , A. S. Kheifets

We study orientation and two-center interference effects in attosecond time-resolved photoionization of the H$_2$ molecule. Time resolution of XUV ionization of H$_2$ is gained through the phase retrieval capability of attosecond angular…

Atomic Physics · Physics 2026-03-03 Vladislav V. Serov , Anatoli S. Kheifets

We demonstrate an accurate phase retrieval of XUV atomic ionization by streaking the photoelectron in a circularly polarized IR laser field. The streaking phase can then be converted to the atomic time delay containing the Wigner and…

A new theoretical approach to the description of the attosecond streaking measurements of atomic photoionization is presented. It is a fully quantum mechanical description based on numerical solving of the time-dependent Schroedinger…

Atomic Physics · Physics 2007-05-23 A. K. Kazansky , N. M. Kabachnik

Time delays of electrons emitted from an isotropic initial state and leaving behind an isotropic ion are assumed to be angle-independent. Using an interferometric method involving XUV attosecond pulse trains and an IR probe field in…

Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…

Measured photoionization time delays may exhibit large variations as a function of the emission angles, even for spherically symmetric targets, as shown in recent RABBITT (reconstruction of attosecond beating by interference of two-photon…

Atomic Physics · Physics 2022-12-29 D. I. R. Boll , L. Martini , A. Palacios , O. A. Fojón

We describe in detail how attosecond delays in laser-assisted photoionization can be computed using perturbation theory based on two-photon matrix elements. Special emphasis is laid on above-threshold ionization, where the electron…

Atomic Physics · Physics 2015-06-19 J. M. Dahlström , E. Lindroth

We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets , I. A. Ivanov , Igor. Bray

Attosecond streaking of atomic photoemission holds the promise to provide unprecedented information on the release time of the photoelectron. We show that attosecond streaking phase shifts indeed contain timing (or spectral phase)…

We apply a recently proposed theoretical concept and numerical approach to obtain time delays in extreme ultraviolet (XUV) photoionization of an electron in a short- or long-range potential. The results of our numerical simulations on a…

Atomic Physics · Physics 2015-06-12 Jing Su , Hongcheng Ni , Andreas Becker , Agnieszka Jaron-Becker

We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…

Atomic Physics · Physics 2022-05-03 Jakub Benda , Zdeněk Mašín , Jimena D. Gorfinkiel

Recent angle-resolved RABBITT experiments have shown that the photoionization time delay depends on the emission angle of the photoelectron. In this work we demonstrate that for photoemission from helium accompanied by shake-up (correlation…

Atomic Physics · Physics 2020-09-30 Stefan Donsa , Manuel Ederer , Renate Pazourek , Joachim Burgdörfer , Iva Březinová

We revisit the time-resolved photoemission in neon atoms as probed by attosecond streaking. We calculate streaking time shifts for the emission of 2p and 2s electrons and compare the relative delay as measured in a recent experiment by…

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

We analyze the time delay between emission of photoelectrons from the outer valence $ns$ and $np$ sub-shells in noble gas atoms following absorption of an attosecond XUV pulse. By solving the time dependent Schr\"odinger equation and…

Atomic Physics · Physics 2010-12-07 A. S. Kheifets , I. A. Ivanov

We investigate an angular dependence of the photoemission time delay in helium as measured by the RABBITT (Reconstruction of Attosecond Beating By Interference of Two-photon Transitions) technique. The measured time delay $…

Atomic Physics · Physics 2016-05-17 I A Ivanov , J M Dahlström , E Lindroth , A S Kheifets

Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…

We explore how the spectral phase of atto\-second pulse trains influences the optical cross section in transient absorption (TA) spectroscopy. The interaction of extreme ultraviolet (XUV) and time-delayed near-infrared (NIR) fields with an…

Atomic Physics · Physics 2025-06-12 J. Jakob , C. Bauer , M. -J. Ilhan , D. Bharti , C. Ott , T. Pfeifer , K. Bartschat , A. Harth

We simulate angular resolved RABBITT (Reconstruction of Attosecond Beating By Interference of Two-photon Transitions) measurements on valence shells of noble gas atoms (Ne, Ar, Kr, and Xe). Our non-perturbative numerical simulation is based…

Atomic Physics · Physics 2018-06-13 Alexander W. Bray , Faiza Naseem , Anatoli S. Kheifets
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