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Related papers: Valley Trion Dynamics in Monolayer MoSe$_2$

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Layered two-dimensional (2D) semiconductors such as molybdenum disulfide (MoS2) have recently attracted remarkable attention because of their unique physical properties. Here, we use photoluminescence (PL) and Raman spectroscopy to study…

Monolayer photonic materials offer a tremendous potential for on-chip optoelectronic devices. Their realization requires knowledge of optical coherence properties of excitons and trions that have so far been limited to nonlinear optical…

Mesoscale and Nanoscale Physics · Physics 2017-12-20 Gabriella D. Shepard , Jenny V. Ardelean , Daniel A. Rhodes , X. -Y. Zhu , James C. Hone , Stefan Strauf

We perform photoluminescence experiments at 4K on two different transition metal diselenide monolayers, namely MoSe2 and WSe2 in magnetic fields $B_z$ up to 9T applied perpendicular to the sample plane. In MoSe2 monolayers the valley…

Materials Science · Physics 2015-06-12 G. Wang , L. Bouet , M. M. Glazov , T. Amand , E. L. Ivchenko , E. Palleau , X. Marie , B. Urbaszek

Transition metal dichalcogenide (TMD) monolayers are two-dimensional semiconductors with two valleys in their band structure that can be selectively addressed using circularly polarized light. Their photoluminescence spectrum is…

Mesoscale and Nanoscale Physics · Physics 2020-10-26 Joris J. Carmiggelt , Michael Borst , Toeno van der Sar

Trions, quasi-particles consisting of two electrons combined with one hole or of two holes with one electron, have recently been observed in transition metal dichalcogenides (TMDCs) and drawn increasing attention due to potential…

While valleys (energy extrema) are present in all band structures of solids, their preeminent role in determining exciton resonances and dynamics in atomically thin transition metal dichalcogenides (TMDC) is unique. Using two-dimensional…

We investigate the diffusion process of negatively charged excitons (trions) in WSe2 transition metal dichalcogenide monolayer. We measure time-resolved photoluminescence spatial profiles of these excitonic complexes which exhibit a…

Monolayers of transition metal dichalcogenides present an intriguing platform to investigate the interplay of excitonic complexes in two dimensional semiconductors. Here, we use optical spectroscopy to study light-matter coupling and…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 Jonas Zipfel , Koloman Wagner , Jonas D. Ziegler , Takashi Taniguchi , Kenji Watanabe , Marina A. Semina , Alexey Chernikov

We present a detailed investigation of the exciton and trion dynamics in naturally doped MoSe2 and WSe2 single atomic layers as a function of temperature in the range 10-300K under above band-gap laser excitation. By combining…

Two-dimensional (2D) atomic crystals, such as graphene and transition-metal dichalcogenides, have emerged as a new class of materials with remarkable physical properties. In contrast to graphene, monolayer MoS2 is a non-centrosymmetric…

Materials Science · Physics 2015-06-11 Kin Fai Mak , Keliang He , Changgu Lee , Gwan Hyoung Lee , James Hone , Tony F. Heinz , Jie Shan

Monolayer group VI transition metal dichalcogenides have recently emerged as semiconducting alternatives to graphene in which the true two-dimensionality (2D) is expected to illuminate new semiconducting physics. Here we investigate…

Mesoscale and Nanoscale Physics · Physics 2014-03-05 Jason S Ross , Sanfeng Wu , Hongyi Yu , Nirmal J Ghimire , Aaron M Jones , Grant Aivazian , Jiaqiang Yan , David G. Mandrus , Di Xiao , Wang Yao , Xiaodong Xu

Monolayer transition metal dichalcogenides (TMDs) hold great promise for future information processing applications utilizing a combination of electron spin and valley pseudospin. This unique spin system has led to observation of the valley…

Mesoscale and Nanoscale Physics · Physics 2019-05-30 T. P. Lyons , S. Dufferwiel , M. Brooks , F. Withers , T. Taniguchi , K. Watanabe , K. S. Novoselov , G. Burkard , A. I. Tartakovskii

Charged optical excitations (trions) generated by charge carrier injection are crucial for emerging optoelectronic technologies as they can be produced and manipulated by electric fields. Trions and neutral excitons can be efficiently…

Atomic and Molecular Clusters · Physics 2021-12-23 Jiří Doležal , Sofia Canola , Pablo Merino , Martin Švec

Optical and transport properties of doped monolayer semiconductors are dominated by trions, which are three-particle compounds formed by two electrons and one hole or vice versa. In this work, we investigate the trion-phonon interaction on…

Mesoscale and Nanoscale Physics · Physics 2022-09-09 Raul Perea-Causin , Samuel Brem , Ermin Malic

We investigate how many-electron excited states emerge in twisted MoSe2 homobilayers when the lattice reconstructions evolve. Notably, we identify a new trion resonance that arises in the transition regime of lattice reconstruction, where…

We perform absorption and photoluminescence spectroscopy of trions in hBN-encapsulated WSe$_2$, WS$_2$, MoSe$_2$, and MoS$_2$ monolayers, depending on temperature. The different trends for W- and Mo-based materials are excellently…

Trions -- Coulomb-bound three-particle excitations composed of two like-charge carriers and one oppositely charged carrier -- are central quasiparticles in two-dimensional semiconductors. Reduced dielectric screening and quantum confinement…

Mesoscale and Nanoscale Physics · Physics 2026-03-27 Roman Ya. Kezerashvili

The interactions between charges and excitons involve complex many-body interactions at high densities. The exciton-polaron model has been adopted to understand the Fermi sea screening of charged excitons in monolayer transition metal…

Mesoscale and Nanoscale Physics · Physics 2023-09-14 Xin Cong , Parisa Ali Mohammadi , Mingyang Zheng , Kenji Watanabe , Takashi Taniguchi , Daniel Rhodes , Xiao-Xiao Zhang

The valley pseudospin in monolayer transition metal dichalcogenides (TMDs) has been proposed as a new way to manipulate information in various optoelectronic devices. This relies on a large valley polarization that remains stable over long…

Mesoscale and Nanoscale Physics · Physics 2017-12-22 Fahad Mahmood , Zhanybek Alpichshev , Yi-Hsien Lee , Jing Kong , Nuh Gedik

We investigate the transport of excitons and trions in monolayer semiconductor WS$_2$ subjected to controlled non-uniform mechanical strain. We actively control and tune the strain profiles with an AFM-based setup in which the monolayer is…

Mesoscale and Nanoscale Physics · Physics 2020-05-20 Moshe G. Harats , Jan N. Kirchhof , Mengxiong Qiao , Kyrylo Greben , Kirill I. Bolotin