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High-harmonic generation (HHG) in two-dimensional materials offers a compelling route toward compact extreme ultraviolet sources and probing electron dynamics on the attosecond scale. However, achieving precise control over the emission and…

Computational Physics · Physics 2026-05-19 Zhenjiang Zhao , Zhihua Zheng , Zhiyi Xu , Xing Ran , Xiaolong Yao , Fangping Ouyang

We establish time-resolved high harmonic generation (tr-HHG) as a powerful spectroscopy for photoinduced dynamics in strongly correlated materials through a detailed investigation of the insulator-to-metal transitions in vanadium dioxide.…

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…

Atomic Physics · Physics 2025-03-31 Xinhua Xie

We propose a novel amplification mechanism for high harmonic generation (HHG) in solids by leveraging bandgap engineering with momentum k-gaps. By constructing a simple diatomic lattice featuring balanced, alternating gain and loss…

Optics · Physics 2025-03-28 Yiming Pan , Danni Chen , Xiaoxi Xu , Zhaopin Chen , Huaiqiang Wang

Since the discovery of high-order harmonic generation (HHG) in solids, much effort has been devoted to understanding its generation mechanism and both interband and intraband transitions are known to be essential. However, intraband…

Optical coherence encodes information about the correlations of the electromagnetic field. In combination with quantum optical approaches, it allows for the study of the correlations between photons. Since the pioneering papers of Glauber,…

Quantum Physics · Physics 2025-04-21 Philipp Stammer , Javier Rivera-Dean , Maciej Lewenstein

High-harmonic generation (HHG), which is generation of multiple optical harmonic light, is an unconventional nonlinear optical phenomenon beyond perturbation regime. HHG, which was initially observed in gaseous media, has recently been…

High harmonic spectra generated in condensed matter carry the fingerprints of sub-cycle electronic motion and the energy structure of the studied system. Here we show that tailoring the waveform of mid-infrared driving light by using a…

A theoretical model for high-order harmonic generation (HHG) in bulk solids is considered. Our approach treats laser-induced inter- and intraband currents on an equal footing. The sum of these currents is the source of the high-order…

Quantum Physics · Physics 2017-07-12 Peter Foldi

Several correlation and interference effects in strong-field physics are investigated. We show that the interference of continuum wave packets can be the dominant mechanism of high-harmonic generation (HHG) in the over-the-barrier regime.…

Using real-space view of high harmonic generation (HHG) in solids, we develop a physically transparent and gauge-invariant approach for distinguishing intraband and interband HHG mechanisms. Our approach relies on resolving the harmonic…

High harmonic generation (HHG) takes place in all phases of matter. In gaseous atomic and molecular media, it has been extensively studied and is very well-understood. In solids research is ongoing, but a consensus is forming for the…

Chemical Physics · Physics 2022-06-22 Ofer Neufeld , Zahra Nourbakhsh , Nicolas Tancogne-Dejean , Angel Rubio

High-harmonic generation has emerged as a pivotal process in strong-field physics, yielding extreme ultraviolet radiation and attosecond pulses with a wide range of applications. Furthermore, its emergent connection with the field of…

High harmonic generation (HHG) in crystals has revealed a wealth of perspectives such as all-optical mapping of the electronic band structure, ultrafast quantum information and the creation of novel all-solid-state attosecond sources.…

Since the new millennium coherent extreme ultra-violet and soft x-ray radiation has revolutionized the understanding of dynamical physical, chemical and biological systems at the electron's natural timescale. Unfortunately, coherent…

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

High-harmonic generation (HHG) in solids is an emerging method to probe ultrafast electron dynamics in solids at attosecond timescale. In this work, we study HHG from monolayer and bilayer graphene. Bilayer graphenes with AA and AB stacking…

Optics · Physics 2021-03-26 M. S. Mrudul , Gopal Dixit

Symmetries essentially provide conservation rules in nonlinear light-matter interactions, that facilitate control and understanding of photon conversion processes or electron dynamics. Since anisotropic solids have rich symmetries, they are…

Light beams carrying orbital angular momentum (OAM) have led to stunning applications in various fields from quantum information to microscopy. In this letter, we examine OAM from the recently discovered high-harmonic generation (HHG) in…