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Related papers: Herbertsmithite and the Search for the Quantum Spi…

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The effect of the quenched bond-randomness on the ordering of the $S=1/2$ antiferromagnetic Heisenberg model on the kagome lattice is investigated by means of an exact-diagonalization method. When the randomness exceeds a critical value,…

Strongly Correlated Electrons · Physics 2015-08-18 Hikaru Kawamura , Ken Watanabe , Tokuro Shimokawa

The kagome Heisenberg antiferromagnet formed by frustrated spins arranged in a lattice of corner-sharing triangles is a prime candidate for hosting a quantum spin liquid (QSL) ground state consisting of entangled spin singlets. But the…

Strongly Correlated Electrons · Physics 2022-03-09 Jiaming Wang , Weishi Yuan , Philip M. Singer , Rebecca W. Smaha , Wei He , Jiajia Wen , Young S. Lee , Takashi Imai

The spin-1/2 kagome lattice antiferromagnet herbertsmithite, ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, is a candidate material for a quantum spin liquid ground state. We show that the magnetic response of this material displays an unusual scaling…

Strongly Correlated Electrons · Physics 2010-04-07 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Qiu , D. G. Nocera , Y. S. Lee

The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…

We report measurements of the specific heat and magnetization of single crystal samples of the spin-1/2 kagome compound ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ (herbertsmithite), a promising quantum spin-liquid candidate, in high magnetic fields and…

In solid materials, nontrivial topological states, electron correlations, and magnetism are central ingredients for realizing quantum properties, including unconventional superconductivity, charge and spin density waves, and quantum spin…

Strongly Correlated Electrons · Physics 2023-10-10 Yaojia Wang , Heng Wu , Gregory T. McCandless , Julia Y. Chan , Mazhar N. Ali

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

The structural-magnetic models of 25 AFM kagome cuprates similar to herbertsmithite (ZnCu3(OH)6Cl2) - a perspective spin liquid - have been calculated and analyzed. Main correlations between the structure and magnetic properties of these…

Materials Science · Physics 2021-08-13 L. M. Volkova , D. V. Marinin

Spin-1/2 kagome-lattice Heisenberg antiferromagnet is theoretically known to have a quantum spin liquid ground state, one of the frontiers of condensed matter physics. The search for the model substances has been continued for a long time,…

Strongly Correlated Electrons · Physics 2024-08-21 Hidekazu Tanaka

Magnetic properties of the spin-1/2 kagome-like compound volborthite are studied using a high-quality polycrystalline sample. It is evidenced from magnetization and specific heat measurements that the spins on the kagome lattice still…

Condensed matter physicists have long sought a realistic two-dimensional (2D) magnetic system whose ground state is a {\it spin liquid}---a zero temperature state in which quantum fluctuations have melted away any form of magnetic order.…

Strongly Correlated Electrons · Physics 2012-08-16 Simeng Yan , David A. Huse , Steven R. White

The kagome lattice sits at the crossroad of present research efforts in quantum spin liquids, chiral phases, emergent skyrmion excitations and anomalous Hall effects to name but a few. In light of this diversity, our goal in this paper is…

Strongly Correlated Electrons · Physics 2016-02-17 K. Essafi , Owen Benton , Ludovic D. C. Jaubert

Quantum spin liquids are exotic quantum phases of matter that do not order even at zero temperature. While there are several toy models and simple Hamiltonians that could host a quantum spin liquid as their ground state, it is very rare to…

Strongly Correlated Electrons · Physics 2020-09-02 A. Kshetrimayum , C. Balz , B. Lake , J. Eisert

In recent work, we argued that a particular algebraic spin liquid (ASL) may be the ground state of the S = 1/2 kagome lattice Heisenberg antiferromagnet. This state, which lacks a spin gap, is appealing in light of recent experiments on…

Strongly Correlated Electrons · Physics 2008-06-10 Michael Hermele , Ying Ran , Patrick A. Lee , Xiao-Gang Wen

Actively shought since the turn of the century, two-dimensional quantum spin liquids (QSLs) are exotic phases of matter where magnetic moments remain disordered even at extremely low temperatures. Despite ongoing searches, QSLs remain…

Strongly Correlated Electrons · Physics 2015-07-22 Juan Carrasquilla , Zhihao Hao , Roger G. Melko

On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

Low energy inelastic neutron scattering on single crystals of the kagome spin liquid compound ZnCu3(OD)6Cl2 (Herbertsmithite) reveals antiferromagnetic correlations between impurity spins for energy transfers E < 0.8 meV (~J/20). The…

Strongly Correlated Electrons · Physics 2016-08-24 Tian-Heng Han , M. R. Norman , J. -J. Wen , Jose A. Rodriguez-Rivera , Joel S. Helton , Collin Broholm , Young S. Lee

The quantum spin liquid material herbertsmithite is described by an antiferromagnetic Heisenberg model on the kagome lattice with non-negligible Dzyaloshinskii-Moriya interaction~(DMI). A well established phase transition to the $\mathbf…

Strongly Correlated Electrons · Physics 2017-07-04 Laura Messio , Samuel Bieri , Claire Lhuillier , Bernard Bernu

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

Strongly Correlated Electrons · Physics 2019-07-02 A. Zorko , M. Pregelj , M. Klanjšek , M. Gomilšek , Z. Jagličić , J. S. Lord , J. A. T. Verezhak , T. Shang , W. Sun , J. -X. Mi

The study of quantum spin-liquid states (QSL) with lattice dimension $>1$ has proven an enduring problem in solid state physics. Key candidate materials are the $S=\frac{1}{2}$ kagome magnets due to their ability to host quantum…

Materials Science · Physics 2016-10-04 E Connolly , P Reeves , D Boldrin , A S Wills