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The dynamics of polymer-nanoparticle (NP) mixtures, which involves multiple scales and system-specific variables, has posed a long-standing challenge on its theoretical description. In this paper, we construct a microscopic theory for…

Soft Condensed Matter · Physics 2021-06-15 Bokai Zhang , Jian Li , Juan-mei Hu , Lei Liu

Over the past two decades polymer nanocomposites have received tremendous interest from industry and academia due to their advanced properties comparative to polymer blends. Many computational studies have revealed that the macroscopic…

Materials Science · Physics 2015-04-07 Argyrios Karatrantos

The equilibrium properties of block copolymer micelles confined in polymer thin films are investigated using self-consistent field theory. The theory is based on a model system consisting of AB diblock copolymers and A homopolymers. Two…

Soft Condensed Matter · Physics 2014-01-16 Jiajia Zhou , An-Chang Shi

The effect of ring stiffness and pressure on the glassy dynamics of a thermal assembly of two-dimensional ring polymers is investigated using extensive coarse-grained molecular dynamics simulations. In all cases, dynamical slowing down is…

Soft Condensed Matter · Physics 2023-06-06 Sayantan Ghosh , Satyavani Vemparala , Pinaki Chaudhuri

Twist grain boundaries are widely observed in lamellar phases of block copolymers. A mesoscopic model of the copolymer is used to obtain stationary configurations that include a twist grain boundary, and to analyze their stability against…

Soft Condensed Matter · Physics 2008-04-15 Xusheng Zhang , Zhi-Feng Huang , Jorge Viñals

We present a braided circuit topology framework for investigating topology and structural phase transitions in aggregates of semiflexible polymers. In the conventional approach to circuit topology, which specifically applies to single…

Soft Condensed Matter · Physics 2024-02-27 Jonas Berx , Alireza Mashaghi

We propose and study a model for the equilibrium statistical mechanics of a pressurised semiflexible polymer ring. The Hamiltonian has a term which couples to the algebraic area of the ring and a term which accounts for bending…

Statistical Mechanics · Physics 2009-11-13 Mithun K. Mitra , Gautam I. Menon , R. Rajesh

The mean area of a two-dimensional Gaussian ring of $N$ monomers is known to diverge when the ring is subject to a critical pressure differential, $p_c \sim N^{-1}$. In a recent publication [Eur. Phys. J. E 19, 461 (2006)] we have shown…

Soft Condensed Matter · Physics 2008-04-27 Emir Haleva , Haim Diamant

The structure and function of polymers in confined environments, e.g., biopolymers in the cytoplasm of a cell, are strongly affected by macromolecular crowding. To explore the influence of solvent quality on conformations of crowded…

Soft Condensed Matter · Physics 2018-09-27 Wyatt J. Davis , Alan R. Denton

The excluded volume effects of randomly branched polymers are investigated. To approach this problem we assume the Gaussian distribution of segments around the center of gravity. Once this approximation is introduced, we can make use of the…

Soft Condensed Matter · Physics 2017-09-27 Kazumi Suematsu

We determine the depletion-induced phase-behavior of hard sphere colloids and interacting polymers by large-scale Monte Carlo simulations using very accurate coarse-graining techniques. A comparison with standard Asakura-Oosawa model…

Soft Condensed Matter · Physics 2009-11-07 P. G. Bolhuis , A. A. Louis , J-P Hansen

A self consistent field theory for compressible polymer mixtures is developed by introducing elements of classical density functional theory into the framework of the Helfand theory. It is then applied to study free surfaces of binary (A,B)…

Condensed Matter · Physics 2009-10-28 F. Schmid

Effects of multi-gradient fields on the transport of a polymer chain have been investigated by using generalized Langevin dynamics simulations. We observe that the natural frequency of tumbling follows $Wi^{0.66}$ scaling, where $Wi$ is the…

Soft Condensed Matter · Physics 2019-01-30 Sadhana Singh , Sanjay Kumar

The aim of this paper is to investigate the distribution of a continuous polymer in the presence of an attractive finitely supported potential. The most intricate behavior can be observed if we simultaneously and independently vary two…

Mathematical Physics · Physics 2020-12-04 L. Koralov , S. Molchanov , B. Vainberg

During the life cycle of bacterial cells the non-mixing of the two ring-shaped daughter genomes is an important prerequisite for the cell division process. Mimicking the environments inside highly crowded biological cells, we study the…

Soft Condensed Matter · Physics 2014-12-24 Jaeoh Shin , Andrey G Cherstvy , Ralf Metzler

The conformational statistics of ring polymers in melts or dense solutions is strongly affected by their quenched microscopic topological state. The effect is particularly strong for non-concatenated unknotted rings, which are known to…

Soft Condensed Matter · Physics 2015-06-17 Angelo Rosa , Ralf Everaers

Theoretical aspects of polymers in mixed solvents are considered using the Edwards Hamiltonian formalism. Thermodynamic and structural properties are investigated and some predictions are made when the mixed solvent approaches criticality.…

Soft Condensed Matter · Physics 2007-05-23 A. Negadi , A. Sans-Penninckx , M. Bemouna , T. A. Vilgis

We consider a mean-field model of a polymer with a spherically-symmetric finitely supported potential. We describe how the typical size of the polymer depends on the two parameters: the temperature, which approaches the critical value, and…

Mathematical Physics · Physics 2020-08-12 L. Koralov , S. Molchanov , B. Vainberg

We consider a biopolymer bundle consisting of filaments that are crosslinked together. The crosslinks are reversible: they can dynamically bind and unbind adjacent filament pairs as controlled by a binding enthalpy. The bundle is subjected…

Soft Condensed Matter · Physics 2012-01-19 Richard L. C. Vink , Claus Heussinger

The endpoint distribution and dynamics of semiflexible fibers is studied by numerical simulation. A brief overview is given over the analytical theory of flexible and semiflexible polymers. In particular, a closed expression is given for…

Soft Condensed Matter · Physics 2013-06-13 Robert D. Groot