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Symmetry adaptation techniques are applied to the determination of the intensity of two-photon absorption transitions, between Stark levels of configurations with opposite parities, for transition ions in finite symmetry environments. The…

Atomic and Molecular Clusters · Physics 2007-05-23 M. Daoud , M. Kibler

Unravelling the main initial dynamics responsible for chiral recognition is a key stepin the understanding of many biological processes. However this challenging task requires a sensitive enantiospecic probe to investigate molecular…

We investigate the characteristic effects of nuclear motion on attosecond transient absorption spectra in molecules by calculating the spectrum for different model systems. Two models of the hydrogen molecular ion are considered: one where…

Atomic Physics · Physics 2015-04-16 Jens E. Bækhøj , Lun Yue , Lars Bojer Madsen

A new type of disorder-driven electronic percolation transition is found for two-dimensional electron gas (2DEG), based on a quantum cellular automaton model. This transition is shown to be accompanied with a metal-insulator transition, as…

Statistical Mechanics · Physics 2018-10-17 M. N. Najafi

The systematic shifts of the transition frequencies in the molecular hydrogen ions are of relevance to ultra-high-resolution radio-frequency, microwave and optical spectroscopy of these systems, performed in ion traps. We develop the…

Atomic Physics · Physics 2015-06-16 Dimitar Bakalov , Stephan Schiller

Liquid crystals (LCs) play a fundamental and significant role in modern technology. Recently, they have also been used in active switching, adaptive optics, and next-generation displays for augmented and virtual reality. This is due to the…

Optics · Physics 2022-08-18 N. Madadi , M. Amiri

Specific heat and linear thermal expansivity are fundamental thermal dynamics and have been proven as interesting relaxing quantities to investigate in glass transition and glassy state. However, their possibility has much less been…

Soft Condensed Matter · Physics 2021-09-06 Pengfei Zhang , Marco Gandolfi , Francesco Banfi , Christ Glorieux , Liwang Liu

The objective of this article is to study the behavior of electromagnetic field under X-ray diffraction by time-dependent deformed crystals. Derived system of differential equations looks like the Takagi equations in the case of…

Computational Physics · Physics 2007-05-23 Svetlana Sytova

We find that transparent conducting oxides (TCOs) exhibit oscillatory (sign-reversing) dynamics on a few optical cycle timescale under extreme electron temperatures. We demonstrate a mechanism for such transient dynamics and present an…

We present a theoretical study of the shaping of the time-evolution of field-free orientation of linear molecules. We show the extend to which the degree of orientation can be steered along a desired periodic time-dependent signal. The…

Quantum Physics · Physics 2019-05-15 R. Tehini , K. Hamraoui , D. Sugny

Broadband dielectric spectroscopy was used to study the molecular orientational dynamics of the glass-forming, thioether-linked cyanobiphenyl liquid crystal dimers. As was expected theoretically, two different relaxation processes that…

Soft Condensed Matter · Physics 2023-04-18 M. Czarnecka , Y. Arakawa , A. Kocot , K. Merkel

Temperature-induced phase transition in BaTiO3 has been explored using the machine learning analysis of domain morphologies visualized via variable-temperature scanning transmission electron microscopy (STEM) imaging data. This approach is…

Materials Science · Physics 2020-11-20 Mani Valleti , Reinis Ignatans , Sergei V. Kalinin , Vasiliki Tileli

Antiferroelectric liquid crystals can be considered as a promising alternative to nematic mixtures in the area of microdisplays. Switching behaviour of the molecules has been modelled as two adjacent smectic layers. However, some studies…

Soft Condensed Matter · Physics 2007-05-23 P. L. del Castillo , P. L. Lucas , N. Bennis , A. Spadlo , D. Rodriguez-Perez

Optical microscopy is without a doubt an essential component of life science research, but many objects of interest in biology are transparent. Chemical or immunological dyes, which can often be toxic, fluorescent transgenes, which require…

Optics · Physics 2012-09-11 Quintin Tyrell Davis

In an attempt to quantitatively characterize the recently observed slow dynamics in the isotropic and nematic phase of liquid crystals, we investigate the single-particle orientational dynamics of rodlike molecules across the…

Soft Condensed Matter · Physics 2009-11-13 Biman Jana , Dwaipayan Chakrabarti , Biman Bagchi

We study the relaxation dynamics and intersystem-crossing to the metastable state in laser-pumped tetra and hexa-coordinated nickel porphyrins. We use a ligand-field model which takes into account the crystal field created by the porphyrin…

Strongly Correlated Electrons · Physics 2015-11-29 Javier Fernandez-Rodriguez , Jun Chang , Arthur J. Fedro , Michel van Veenendaal

Two-dimensional infrared (2DIR) spectroscopy is widely used to study molecular dynamics but it is typically restricted to solid and liquid phase samples and modest spectral resolution. Only recently, its potential to study gas-phase…

Optics · Physics 2022-11-01 Grzegorz Kowzan , Thomas K. Allison

We report on time-resolved broadband transient reflectivity (tr-bb-TR) measurements performed on a bulk single crystal of T$_d$-MoTe$_2$ as a function of the incident pump fluence (F). Tr-bb-TR data unveil photoinduced electronic changes…

This paper presents an analytical framework for the analysis of time-varying metal-based metamaterials. Concretely, we particularize the study to time-modulated metal-air interfaces embedded between two different semi-infinite media that…

We apply a time-dependent perturbation theory based on unitary transformations combined with averaging techniques, on molecular orientation dynamics by ultrashort pulses. We test the validity and the accuracy of this approach on LiCl…

Quantum Physics · Physics 2007-05-23 D. Sugny , A. Keller , O. Atabek , D. Daems , S. Guérin , H. R. Jauslin